volume 280 issue 3 pages 629-634

Evolution of actinide partitioning with colloidal matter collected at PA "mayak" site as studied by sequential extraction

E V Kuzovkina 1
B. F. Myasoedov 1
K. Fujiwara 3
A. FUJIWARA 3
Publication typeJournal Article
Publication date2009-04-27
scimago Q2
wos Q3
SJR0.388
CiteScore2.9
Impact factor1.6
ISSN02365731, 15882780
Spectroscopy
Analytical Chemistry
Health, Toxicology and Mutagenesis
Public Health, Environmental and Occupational Health
Pollution
Radiology Nuclear Medicine and imaging
Nuclear Energy and Engineering
Abstract
Evolution of actinide partitioning to colloids upon subsurface migration in the vicinity of Karachay Lake (PA “Mayak”, Russia) was studied by micro- and ultrafiltration and sequential extraction. Colloidal matter was characterized by SEM-EDX, TEM and photon-correlation spectroscopy. Samples were collected from wells with different redox conditions i.e. from higly oxic to rather reducing. Under oxidizing conditions uranium and neptunium is readily washed out from colloids. Plutonium and americium are present in colloidal matter mainly as hard-soluble species. Under oxidizing conditions plutonium and americium are predominantly bound to organic/mineral fractions (carbonates, oxides and organically bound). Under reducing conditions plutonium and americium are present in immobile refractory fraction. It was also established that uranium and neptunium under reducing conditions behave similarly to plutonium. This phenomenon may be explained by the fact that under reducing conditions and at considerable concentrations of uranium and nitrite-ions these elements form low-soluble An(IV) forms.
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Novikov A. P. et al. Evolution of actinide partitioning with colloidal matter collected at PA "mayak" site as studied by sequential extraction // Journal of Radioanalytical and Nuclear Chemistry. 2009. Vol. 280. No. 3. pp. 629-634.
GOST all authors (up to 50) Copy
Novikov A. P., Kalmykov S. N., Kuzovkina E. V., Myasoedov B. F., Fujiwara K., FUJIWARA A. Evolution of actinide partitioning with colloidal matter collected at PA "mayak" site as studied by sequential extraction // Journal of Radioanalytical and Nuclear Chemistry. 2009. Vol. 280. No. 3. pp. 629-634.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1007/s10967-008-7397-y
UR - https://doi.org/10.1007/s10967-008-7397-y
TI - Evolution of actinide partitioning with colloidal matter collected at PA "mayak" site as studied by sequential extraction
T2 - Journal of Radioanalytical and Nuclear Chemistry
AU - Novikov, A. P.
AU - Kalmykov, St N
AU - Kuzovkina, E V
AU - Myasoedov, B. F.
AU - Fujiwara, K.
AU - FUJIWARA, A.
PY - 2009
DA - 2009/04/27
PB - Springer Nature
SP - 629-634
IS - 3
VL - 280
SN - 0236-5731
SN - 1588-2780
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2009_Novikov,
author = {A. P. Novikov and St N Kalmykov and E V Kuzovkina and B. F. Myasoedov and K. Fujiwara and A. FUJIWARA},
title = {Evolution of actinide partitioning with colloidal matter collected at PA "mayak" site as studied by sequential extraction},
journal = {Journal of Radioanalytical and Nuclear Chemistry},
year = {2009},
volume = {280},
publisher = {Springer Nature},
month = {apr},
url = {https://doi.org/10.1007/s10967-008-7397-y},
number = {3},
pages = {629--634},
doi = {10.1007/s10967-008-7397-y}
}
MLA
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MLA Copy
Novikov, A. P., et al. “Evolution of actinide partitioning with colloidal matter collected at PA "mayak" site as studied by sequential extraction.” Journal of Radioanalytical and Nuclear Chemistry, vol. 280, no. 3, Apr. 2009, pp. 629-634. https://doi.org/10.1007/s10967-008-7397-y.