Extraction of actinides with heterocyclic dicarboxamides
M Alyapyshev
1
,
V Babain
1
,
L Tkachenko
2
,
E Kenf
2
,
I Voronaev
2
,
D Darin
3
,
P Matveev
4
,
V. Petrov
4
,
S. Kalmykov
4
,
Y Ustynyuk
4
Publication type: Journal Article
Publication date: 2018-03-01
scimago Q2
wos Q3
SJR: 0.388
CiteScore: 2.9
Impact factor: 1.6
ISSN: 02365731, 15882780
Spectroscopy
Analytical Chemistry
Health, Toxicology and Mutagenesis
Public Health, Environmental and Occupational Health
Pollution
Radiology Nuclear Medicine and imaging
Nuclear Energy and Engineering
Abstract
Extraction of actinides from aqueous nitric acid by three different heterocyclic dicarboxamides (2,6-pyridinedicarboxamide, 2,2′-bipyridine-6,6′-dicarboxamide and 1,10-phenanthroline-2,9-dicarboxamides) was studied. It was shown that all studied ligands extract actinides at different oxidation states (U(VI), Np(V), Pu(IV), Am(III), Cm(III)) from acidic solutions. All studied diamides extract Am(III) better than Cm(III). Et(pHexPh)ClPhen contains electron-withdrawing chlorine atoms at the positions 4 and 7 of the phenanthroline moiety (SFAm/Cm = 4–6) and possesses the highest separation factor Am(III)/Cm(III). The studied ligands possess high extraction ability to all actinides present in HLW and therefore they could be used for simultaneous extraction of actinides in the GANEX-type process.
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GOST
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Alyapyshev M. et al. Extraction of actinides with heterocyclic dicarboxamides // Journal of Radioanalytical and Nuclear Chemistry. 2018. Vol. 316. No. 2. pp. 419-428.
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Alyapyshev M., Babain V., Tkachenko L., Kenf E., Voronaev I., Darin D., Matveev P., Petrov V., Kalmykov S., Ustynyuk Y. Extraction of actinides with heterocyclic dicarboxamides // Journal of Radioanalytical and Nuclear Chemistry. 2018. Vol. 316. No. 2. pp. 419-428.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1007/s10967-018-5775-7
UR - https://doi.org/10.1007/s10967-018-5775-7
TI - Extraction of actinides with heterocyclic dicarboxamides
T2 - Journal of Radioanalytical and Nuclear Chemistry
AU - Alyapyshev, M
AU - Babain, V
AU - Tkachenko, L
AU - Kenf, E
AU - Voronaev, I
AU - Darin, D
AU - Matveev, P
AU - Petrov, V.
AU - Kalmykov, S.
AU - Ustynyuk, Y
PY - 2018
DA - 2018/03/01
PB - Springer Nature
SP - 419-428
IS - 2
VL - 316
SN - 0236-5731
SN - 1588-2780
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Alyapyshev,
author = {M Alyapyshev and V Babain and L Tkachenko and E Kenf and I Voronaev and D Darin and P Matveev and V. Petrov and S. Kalmykov and Y Ustynyuk},
title = {Extraction of actinides with heterocyclic dicarboxamides},
journal = {Journal of Radioanalytical and Nuclear Chemistry},
year = {2018},
volume = {316},
publisher = {Springer Nature},
month = {mar},
url = {https://doi.org/10.1007/s10967-018-5775-7},
number = {2},
pages = {419--428},
doi = {10.1007/s10967-018-5775-7}
}
Cite this
MLA
Copy
Alyapyshev, M., et al. “Extraction of actinides with heterocyclic dicarboxamides.” Journal of Radioanalytical and Nuclear Chemistry, vol. 316, no. 2, Mar. 2018, pp. 419-428. https://doi.org/10.1007/s10967-018-5775-7.