Russian Chemical Bulletin

, том 64 , издание 9 , страницы 2062-2068

Selective deoxygenation of vegetable oils in the presence of Pt–Sn/Al2O3 catalyst

M V Tsodikov ^{1, 2}

A. V. Chistyakov ^{1, 2}

M A Gubanov ^{1, 2}

P A Zharova ^{1, 2}

S S Shapovalov ³

A A Pasynskii ³

V.V. Kriventsov ⁴

I. I. Moiseev ^{1, 3}

Скрыть аффилиации авторов Показать аффилиации авторов: 4 аффилиации

A. V. Topchiev Institute of Petrochemical Synthesis, Russian Academy of Sciences, Moscow, Russian Federation |

Moscow Institute of Physics and Technology, Dolgoprudny, Moscow Region, Russian Federation |

Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences, Moscow, Russian Federation |

⁴

Boreskov Institute of Catalysis, Siberian Branch of the Russian Academy of Sciences, Novosibirsk, Russian Federation |

Тип публикации: Journal Article

Дата публикации: 2015-09-01

Springer Nature

Russian Chemical Bulletin

scimago Q3

БС2

SJR: 0.305

CiteScore: 2.8

Impact factor: —

ISSN: 10665285, 15739171

DOI: 10.1007/s11172-015-1118-9

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General Chemistry

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We studied deoxygenation of individual fatty esters and fatty acid triglycerides from vegetable oils and lipid extracts from microalgae in the presence of catalysts prepared by deposition of Pt–Sn-containing compounds onto the γ-aluminum oxide surface. Using individual esters as an example, selective reduction of oxygen into water was demonstrated for the first time to proceed on a catalytic system at the 5 : 1 molar ratio of Sn and Pt active components to afford hydrocarbon components of substrates in virtually quantitative yield. Transformation of vegetable oil in the presence of this catalyst affords the C3–C18 hydrocarbon fraction in yield up to 99% at the content of C3 and C18 hydrocarbons up to 90%. The fraction of C1 and C2 hydrocarbons and carbon oxides is not higher than 0.5%. The possibility of carbon weight loss minimization during transformation of lipids was shown for the first time.

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Tsodikov M. V. et al. Selective deoxygenation of vegetable oils in the presence of Pt–Sn/Al2O3 catalyst // Russian Chemical Bulletin. 2015. Vol. 64. No. 9. pp. 2062-2068.

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Tsodikov M. V., Chistyakov A. V., Gubanov M. A., Zharova P. A., Shapovalov S. S., Pasynskii A. A., Kriventsov V., Moiseev I. I. Selective deoxygenation of vegetable oils in the presence of Pt–Sn/Al2O3 catalyst // Russian Chemical Bulletin. 2015. Vol. 64. No. 9. pp. 2062-2068.

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TY - JOUR

DO - 10.1007/s11172-015-1118-9

UR - https://doi.org/10.1007/s11172-015-1118-9

TI - Selective deoxygenation of vegetable oils in the presence of Pt–Sn/Al2O3 catalyst

T2 - Russian Chemical Bulletin

AU - Tsodikov, M V

AU - Chistyakov, A. V.

AU - Gubanov, M A

AU - Zharova, P A

AU - Shapovalov, S S

AU - Pasynskii, A A

AU - Kriventsov, V.V.

AU - Moiseev, I. I.

PY - 2015

DA - 2015/09/01

PB - Springer Nature

SP - 2062-2068

IS - 9

VL - 64

SN - 1066-5285

SN - 1573-9171

ER -

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@article{2015_Tsodikov,

author = {M V Tsodikov and A. V. Chistyakov and M A Gubanov and P A Zharova and S S Shapovalov and A A Pasynskii and V.V. Kriventsov and I. I. Moiseev},

title = {Selective deoxygenation of vegetable oils in the presence of Pt–Sn/Al2O3 catalyst},

journal = {Russian Chemical Bulletin},

year = {2015},

volume = {64},

publisher = {Springer Nature},

month = {sep},

url = {https://doi.org/10.1007/s11172-015-1118-9},

number = {9},

pages = {2062--2068},

doi = {10.1007/s11172-015-1118-9}

}

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Tsodikov, M. V., et al. “Selective deoxygenation of vegetable oils in the presence of Pt–Sn/Al2O3 catalyst.” Russian Chemical Bulletin, vol. 64, no. 9, Sep. 2015, pp. 2062-2068. https://doi.org/10.1007/s11172-015-1118-9.