Nano Research, volume 13, issue 8, pages 2259-2267
Exploring porous zeolitic imidazolate frame work-8 (ZIF-8) as an efficient filler for high-performance poly(ethyleneoxide)-based solid polymer electrolytes
Zhiwen Lei
1, 2
,
Jinlai Shen
1, 2
,
Weide Zhang
2
,
Qingrong Wang
3
,
Jun Wang
3
,
Yonghong Deng
3
,
Chaoyang Wang
1
2
3
Department of Materials Science and Engineering, Academy for Advanced Interdisciplinary Studies, Guangdong Provincial Key Laboratory of Energy Materials for Electric Power, Shenzhen, China
|
Publication type: Journal Article
Publication date: 2020-06-05
Journal:
Nano Research
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.9
ISSN: 19980124, 19980000
Atomic and Molecular Physics, and Optics
Condensed Matter Physics
General Materials Science
Electrical and Electronic Engineering
Abstract
The incorporation of inorganic fillers into poly(ethyleneoxide)(PEO)-based solid polymer electrolytes (SPEs) is well known as a low-cost and effective method to improve their mechanical and electrochemical properties. Porous zeolitic imidazolate framework-8 (ZIF-8) is firstly used as the filler for PEO-based SPEs in this work. Due to the introduction of ZIF-8, an ionic conductivity of 2.2 × 10−5 S/cm (30 °C) is achieved for the composite SPE, which is one order of magnitude higher than that of the pure PEO. ZIF-8 also accounts for the broader electrochemical stability window and lithium ion transference number (0.36 at 60 °C) of the composite SPE. Moreover, the improved mechanism of ZIF-8 to the composite SPE is investigated by zeta potential and Fourier transform infrared spectrograph characterizations. The stability at the composite SPE/lithium interface is greatly enhanced. The LiFePO4||Li cells using the composite SPE exhibit high capacity and excellent cycling performance at 60 °C, i.e., 85% capacity retention with 111 mA·h/g capacity retained after 350 cycles at 0.5 C. In comparison, the cells using the pure PEO show fast capacity decay to 74 mA·h/g maintaining only 68 capacity. These results indicate that the PEO-based SPEs with ZIF-8 are of great promise for the application in solid-state lithium metal batteries.
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Lei Z. et al. Exploring porous zeolitic imidazolate frame work-8 (ZIF-8) as an efficient filler for high-performance poly(ethyleneoxide)-based solid polymer electrolytes // Nano Research. 2020. Vol. 13. No. 8. pp. 2259-2267.
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Lei Z., Shen J., Zhang W., Wang Q., Wang J., Deng Y., Wang C. Exploring porous zeolitic imidazolate frame work-8 (ZIF-8) as an efficient filler for high-performance poly(ethyleneoxide)-based solid polymer electrolytes // Nano Research. 2020. Vol. 13. No. 8. pp. 2259-2267.
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TY - JOUR
DO - 10.1007/s12274-020-2845-2
UR - https://doi.org/10.1007/s12274-020-2845-2
TI - Exploring porous zeolitic imidazolate frame work-8 (ZIF-8) as an efficient filler for high-performance poly(ethyleneoxide)-based solid polymer electrolytes
T2 - Nano Research
AU - Lei, Zhiwen
AU - Shen, Jinlai
AU - Zhang, Weide
AU - Wang, Qingrong
AU - Wang, Jun
AU - Deng, Yonghong
AU - Wang, Chaoyang
PY - 2020
DA - 2020/06/05 00:00:00
PB - Springer Nature
SP - 2259-2267
IS - 8
VL - 13
SN - 1998-0124
SN - 1998-0000
ER -
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@article{2020_Lei,
author = {Zhiwen Lei and Jinlai Shen and Weide Zhang and Qingrong Wang and Jun Wang and Yonghong Deng and Chaoyang Wang},
title = {Exploring porous zeolitic imidazolate frame work-8 (ZIF-8) as an efficient filler for high-performance poly(ethyleneoxide)-based solid polymer electrolytes},
journal = {Nano Research},
year = {2020},
volume = {13},
publisher = {Springer Nature},
month = {jun},
url = {https://doi.org/10.1007/s12274-020-2845-2},
number = {8},
pages = {2259--2267},
doi = {10.1007/s12274-020-2845-2}
}
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MLA
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Lei, Zhiwen, et al. “Exploring porous zeolitic imidazolate frame work-8 (ZIF-8) as an efficient filler for high-performance poly(ethyleneoxide)-based solid polymer electrolytes.” Nano Research, vol. 13, no. 8, Jun. 2020, pp. 2259-2267. https://doi.org/10.1007/s12274-020-2845-2.