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Nano-Micro Letters, volume 15, issue 1, publication number 74

The Critical Role of Fillers in Composite Polymer Electrolytes for Lithium Battery

Yang Xueying 1
Jiaxiang Liu 1
Nanbiao Pei 1
Zhiqiang Chen 1
Ruiyang Li 2
Lijun Fu 3
Peng Zhang 1
Jinbao Zhao 2
Publication typeJournal Article
Publication date2023-03-28
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor26.6
ISSN23116706, 21505551
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Electrical and Electronic Engineering
Abstract

With excellent energy densities and highly safe performance, solid-state lithium batteries (SSLBs) have been hailed as promising energy storage devices. Solid-state electrolyte is the core component of SSLBs and plays an essential role in the safety and electrochemical performance of the cells. Composite polymer electrolytes (CPEs) are considered as one of the most promising candidates among all solid-state electrolytes due to their excellent comprehensive performance. In this review, we briefly introduce the components of CPEs, such as the polymer matrix and the species of fillers, as well as the integration of fillers in the polymers. In particular, we focus on the two major obstacles that affect the development of CPEs: the low ionic conductivity of the electrolyte and high interfacial impedance. We provide insight into the factors influencing ionic conductivity, in terms of macroscopic and microscopic aspects, including the aggregated structure of the polymer, ion migration rate and carrier concentration. In addition, we also discuss the electrode–electrolyte interface and summarize methods for improving this interface. It is expected that this review will provide feasible solutions for modifying CPEs through further understanding of the ion conduction mechanism in CPEs and for improving the compatibility of the electrode–electrolyte interface.

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GOST |
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GOST Copy
Xueying Y. et al. The Critical Role of Fillers in Composite Polymer Electrolytes for Lithium Battery // Nano-Micro Letters. 2023. Vol. 15. No. 1. 74
GOST all authors (up to 50) Copy
Xueying Y., Liu J., Pei N., Chen Z., Li R., Fu L., Zhang P., Zhao J. The Critical Role of Fillers in Composite Polymer Electrolytes for Lithium Battery // Nano-Micro Letters. 2023. Vol. 15. No. 1. 74
RIS |
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RIS Copy
TY - JOUR
DO - 10.1007/s40820-023-01051-3
UR - https://doi.org/10.1007/s40820-023-01051-3
TI - The Critical Role of Fillers in Composite Polymer Electrolytes for Lithium Battery
T2 - Nano-Micro Letters
AU - Xueying, Yang
AU - Liu, Jiaxiang
AU - Pei, Nanbiao
AU - Chen, Zhiqiang
AU - Li, Ruiyang
AU - Fu, Lijun
AU - Zhang, Peng
AU - Zhao, Jinbao
PY - 2023
DA - 2023/03/28 00:00:00
PB - Springer Nature
IS - 1
VL - 15
SN - 2311-6706
SN - 2150-5551
ER -
BibTex
Cite this
BibTex Copy
@article{2023_Xueying,
author = {Yang Xueying and Jiaxiang Liu and Nanbiao Pei and Zhiqiang Chen and Ruiyang Li and Lijun Fu and Peng Zhang and Jinbao Zhao},
title = {The Critical Role of Fillers in Composite Polymer Electrolytes for Lithium Battery},
journal = {Nano-Micro Letters},
year = {2023},
volume = {15},
publisher = {Springer Nature},
month = {mar},
url = {https://doi.org/10.1007/s40820-023-01051-3},
number = {1},
doi = {10.1007/s40820-023-01051-3}
}
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