Applied Catalysis B: Environmental, volume 243, pages 566-575

Controlled assemble of hollow heterostructured g-C3N4@CeO2 with rich oxygen vacancies for enhanced photocatalytic CO2 reduction

Mengfang Liang ¹

Timur Borjigin ¹

Yuhao Zhang ¹

Beihong Liu ¹

Hui Liu ¹

Hong Guo ¹

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School of Materials Science and Engineering, Yunnan University, No. 2, Green Lake North Road, Kunming 650091, China |

Publication type: Journal Article

Publication date: 2019-04-01

Elsevier

Journal: Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor: 22.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2018.11.010

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Catalysis

Process Chemistry and Technology

General Environmental Science

Abstract

Hollow heterostructured g-C3N4@CeO2 photocatalysts with rich oxygen vacancies are controllable designed by a facile strategy. The synergetic effect and oxygen vacancies of g-C3N4@CeO2 play the major role in the process of CO2 reduction, leading to CH4 generating much earlier and higher concentration than that of the pristine g-C3N4 and CeO2 alone. Meanwhile, the unique hollow structures can make multiple reflections of light in the cavity, and thus enhance the utilization efficiency of light. Moreover, the L-cysteine offers amine groups and meanwhile is anchored on the surface of g-C3N4 during the synthesis process, and thus contributes greatly to the enhanced CO2 adsorption capability. Additionally, the large CO2 adsorption capability is also beneficial for the enhanced photocatalytic activity. Therefore, the novel photocatalysts exhibit a remarkable reduction performance for CO2 reduction under visible light irradiation. The g-C3N4@CeO2 (CeO2 49.7 wt %) shows the highest yields of CH4 (3.5 μmol g−1), CH3OH (5.2 μmol g−1) and CO (16.8 μmol g−1), which are higher than most of other latest reported g-C3N4 based photocatalysts for CO2 photoreduction, including coupled with semiconductors and noble metal cocatalysts. This strategy might represent a novel way for the effective conversion of CO2 to clean fuels and can also be great potential used in the energy and environmental science.

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ACS Applied Nano Materials	ACS Applied Nano Materials, 3, 0.99% ACS Applied Nano Materials 3 publications, 0.99%
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Citations by publishers

	20 40 60 80 100 120 140 160 180
Elsevier	Elsevier, 172, 56.95% Elsevier 172 publications, 56.95%
Wiley	Wiley, 30, 9.93% Wiley 30 publications, 9.93%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 28, 9.27% Royal Society of Chemistry (RSC) 28 publications, 9.27%
American Chemical Society (ACS)	American Chemical Society (ACS), 22, 7.28% American Chemical Society (ACS) 22 publications, 7.28%
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Pleiades Publishing	Pleiades Publishing, 2, 0.66% Pleiades Publishing 2 publications, 0.66%
University of Science and Technology Beijing	University of Science and Technology Beijing, 1, 0.33% University of Science and Technology Beijing 1 publication, 0.33%
Tsinghua University Press	Tsinghua University Press, 1, 0.33% Tsinghua University Press 1 publication, 0.33%
Chinese Society of Rare Earths	Chinese Society of Rare Earths, 1, 0.33% Chinese Society of Rare Earths 1 publication, 0.33%
Chemical Industry Press	Chemical Industry Press, 1, 0.33% Chemical Industry Press 1 publication, 0.33%
King Saud University	King Saud University, 1, 0.33% King Saud University 1 publication, 0.33%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.33% Taiwan Institute of Chemical Engineers 1 publication, 0.33%
KeAi Communications Co.	KeAi Communications Co., 1, 0.33% KeAi Communications Co. 1 publication, 0.33%
Cambridge University Press	Cambridge University Press, 1, 0.33% Cambridge University Press 1 publication, 0.33%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.33% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.33%
	20 40 60 80 100 120 140 160 180

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Liang M. et al. Controlled assemble of hollow heterostructured g-C3N4@CeO2 with rich oxygen vacancies for enhanced photocatalytic CO2 reduction // Applied Catalysis B: Environmental. 2019. Vol. 243. pp. 566-575.

GOST all authors (up to 50) Copy

Liang M., Borjigin T., Zhang Y., Liu B., Liu H., Guo H. Controlled assemble of hollow heterostructured g-C3N4@CeO2 with rich oxygen vacancies for enhanced photocatalytic CO2 reduction // Applied Catalysis B: Environmental. 2019. Vol. 243. pp. 566-575.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.apcatb.2018.11.010

UR - https://doi.org/10.1016/j.apcatb.2018.11.010

TI - Controlled assemble of hollow heterostructured g-C3N4@CeO2 with rich oxygen vacancies for enhanced photocatalytic CO2 reduction

T2 - Applied Catalysis B: Environmental

AU - Liang, Mengfang

AU - Borjigin, Timur

AU - Zhang, Yuhao

AU - Liu, Beihong

AU - Liu, Hui

AU - Guo, Hong

PY - 2019

DA - 2019/04/01 00:00:00

PB - Elsevier

SP - 566-575

VL - 243

SN - 0926-3373

SN - 1873-3883

ER -

BibTex

Cite this

BibTex Copy

@article{2019_Liang,

author = {Mengfang Liang and Timur Borjigin and Yuhao Zhang and Beihong Liu and Hui Liu and Hong Guo},

title = {Controlled assemble of hollow heterostructured g-C3N4@CeO2 with rich oxygen vacancies for enhanced photocatalytic CO2 reduction},

journal = {Applied Catalysis B: Environmental},

year = {2019},

volume = {243},

publisher = {Elsevier},

month = {apr},

url = {https://doi.org/10.1016/j.apcatb.2018.11.010},

pages = {566--575},

doi = {10.1016/j.apcatb.2018.11.010}

}

Found error?

Publisher

Elsevier

Journal

Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor

22.1

ISSN

09263373 (Print)
18733883 (Electronic)