Applied Catalysis B: Environmental, volume 255, pages 117771

Urchin-like hierarchical CoZnAl-LDH/RGO/g-C3N4 hybrid as a Z-scheme photocatalyst for efficient and selective CO2 reduction

Yong Yang ^{1, 2}

Jiajia Wu ³

Tingting Xiao ³

Zheng Tang ³

Jinyou Shen ³

HAIJIN LI ⁴

Yong Zhou ⁴

Zhigang Zou ⁴

Hide authors affiliations Show authors affiliations: 4 affiliations

Eco-Materials and Renewable Energy Research Centre (ERERC), Jiangsu Key Laboratory for Nano Technology, School of Physics, Nanjing University, Nanjing 210093, PR China |

Key Laboratory of Soft Chemistry and Functional Materials, Ministry of Education, Nanjing University of Science and Technology, Nanjing, 210094, PR China |

Key Laboratory of Soft Chemistry and Functional Materials, Ministry of Education, Nanjing University of Science and Technology, Nanjing 210094, PR China |

⁴

Eco-Materials and Renewable Energy Research Centre (ERERC), Jiangsu Key Laboratory for Nano Technology, School of Physics, Nanjing University, Nanjing, 210093, PR China |

Publication type: Journal Article

Publication date: 2019-10-01

Elsevier

Journal: Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor: 22.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2019.117771

Copy DOI

Catalysis

Process Chemistry and Technology

General Environmental Science

Abstract

A unique urchin-like CoZnAl-LDH/RGO/g-C3N4 (LDH/RGO/CN) Z-scheme photocatalyst, which is fabricated by the hydrothermal synthesis of CoZnAl-LDH and the in situ loading of RGO and g-C3N4, is developed for the photocatalytic conversion of CO2. The special spiny external surface and hollow inner cavity endow LDH/RGO/CN with a significantly enhanced light-harvesting capacity. The well-distributed g-C3N4 nanosheets on the CoZnAl-LDH nanoplates, combined with RGO as an electron mediator, constructs an excellent heterosystem with numerous interfaces, efficient charge separation and highly exposed catalytic active sites. The Z-scheme charge-transfer process promotes the oxidizability and reducibility of CoZnAl-LDH and g-C3N4. Furthermore, the synergistic effect among the components contributes to intense adsorption and chemical activation towards CO2, which reduces the reaction barrier for CO2 photoreduction. As a result, the optimized LDH/RGO/CN exhibits highly efficient and selective photocatalytic CO2 conversion to CO. The special 3D urchin-like architecture paves a new way for design of photocatalyst with ideal performance.

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Citations by journals

	2 4 6 8 10 12 14 16 18 20
Chemical Engineering Journal	Chemical Engineering Journal, 19, 8.64% Chemical Engineering Journal 19 publications, 8.64%
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Applied Surface Science	Applied Surface Science, 9, 4.09% Applied Surface Science 9 publications, 4.09%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 9, 4.09% Applied Catalysis B: Environmental 9 publications, 4.09%
Journal of Environmental Chemical Engineering	Journal of Environmental Chemical Engineering, 7, 3.18% Journal of Environmental Chemical Engineering 7 publications, 3.18%
Colloids and Surfaces A: Physicochemical and Engineering Aspects	Colloids and Surfaces A: Physicochemical and Engineering Aspects, 5, 2.27% Colloids and Surfaces A: Physicochemical and Engineering Aspects 5 publications, 2.27%
International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 5, 2.27% International Journal of Hydrogen Energy 5 publications, 2.27%
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Separation and Purification Technology	Separation and Purification Technology, 5, 2.27% Separation and Purification Technology 5 publications, 2.27%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 5, 2.27% Journal of Materials Chemistry A 5 publications, 2.27%
New Journal of Chemistry	New Journal of Chemistry, 5, 2.27% New Journal of Chemistry 5 publications, 2.27%
Energy & Fuels	Energy & Fuels, 4, 1.82% Energy & Fuels 4 publications, 1.82%
Solar RRL	Solar RRL, 4, 1.82% Solar RRL 4 publications, 1.82%
Small	Small, 3, 1.36% Small 3 publications, 1.36%
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Journal of CO2 Utilization	Journal of CO2 Utilization, 3, 1.36% Journal of CO2 Utilization 3 publications, 1.36%
Advanced Functional Materials	Advanced Functional Materials, 3, 1.36% Advanced Functional Materials 3 publications, 1.36%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 1.36% ACS applied materials & interfaces 3 publications, 1.36%
Catalysis Science and Technology	Catalysis Science and Technology, 3, 1.36% Catalysis Science and Technology 3 publications, 1.36%
Nanoscale	Nanoscale, 3, 1.36% Nanoscale 3 publications, 1.36%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 2, 0.91% Coordination Chemistry Reviews 2 publications, 0.91%
Microchimica Acta	Microchimica Acta, 2, 0.91% Microchimica Acta 2 publications, 0.91%
Environmental Science and Pollution Research	Environmental Science and Pollution Research, 2, 0.91% Environmental Science and Pollution Research 2 publications, 0.91%
Solar Energy	Solar Energy, 2, 0.91% Solar Energy 2 publications, 0.91%
Catalysis Letters	Catalysis Letters, 2, 0.91% Catalysis Letters 2 publications, 0.91%
Inorganic Chemistry Communication	Inorganic Chemistry Communication, 2, 0.91% Inorganic Chemistry Communication 2 publications, 0.91%
Journal of Photochemistry and Photobiology A: Chemistry	Journal of Photochemistry and Photobiology A: Chemistry, 2, 0.91% Journal of Photochemistry and Photobiology A: Chemistry 2 publications, 0.91%
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Applied Clay Science	Applied Clay Science, 2, 0.91% Applied Clay Science 2 publications, 0.91%
	2 4 6 8 10 12 14 16 18 20

Citations by publishers

	20 40 60 80 100 120
Elsevier	Elsevier, 116, 52.73% Elsevier 116 publications, 52.73%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 29, 13.18% Royal Society of Chemistry (RSC) 29 publications, 13.18%
Wiley	Wiley, 28, 12.73% Wiley 28 publications, 12.73%
American Chemical Society (ACS)	American Chemical Society (ACS), 16, 7.27% American Chemical Society (ACS) 16 publications, 7.27%
Springer Nature	Springer Nature, 14, 6.36% Springer Nature 14 publications, 6.36%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 6, 2.73% Multidisciplinary Digital Publishing Institute (MDPI) 6 publications, 2.73%
Institution of Chemical Engineers	Institution of Chemical Engineers, 1, 0.45% Institution of Chemical Engineers 1 publication, 0.45%
King Saud University	King Saud University, 1, 0.45% King Saud University 1 publication, 0.45%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.45% Korean Society of Industrial Engineering Chemistry 1 publication, 0.45%
Walter de Gruyter	Walter de Gruyter, 1, 0.45% Walter de Gruyter 1 publication, 0.45%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.45% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.45%
	20 40 60 80 100 120

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Yang Y. et al. Urchin-like hierarchical CoZnAl-LDH/RGO/g-C3N4 hybrid as a Z-scheme photocatalyst for efficient and selective CO2 reduction // Applied Catalysis B: Environmental. 2019. Vol. 255. p. 117771.

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Yang Y., Wu J., Xiao T., Tang Z., Shen J., LI H., Zhou Y., Zou Z. Urchin-like hierarchical CoZnAl-LDH/RGO/g-C3N4 hybrid as a Z-scheme photocatalyst for efficient and selective CO2 reduction // Applied Catalysis B: Environmental. 2019. Vol. 255. p. 117771.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.apcatb.2019.117771

UR - https://doi.org/10.1016/j.apcatb.2019.117771

TI - Urchin-like hierarchical CoZnAl-LDH/RGO/g-C3N4 hybrid as a Z-scheme photocatalyst for efficient and selective CO2 reduction

T2 - Applied Catalysis B: Environmental

AU - Yang, Yong

AU - Wu, Jiajia

AU - Xiao, Tingting

AU - Tang, Zheng

AU - Shen, Jinyou

AU - LI, HAIJIN

AU - Zhou, Yong

AU - Zou, Zhigang

PY - 2019

DA - 2019/10/01 00:00:00

PB - Elsevier

SP - 117771

VL - 255

SN - 0926-3373

SN - 1873-3883

ER -

BibTex

Cite this

BibTex Copy

@article{2019_Yang,

author = {Yong Yang and Jiajia Wu and Tingting Xiao and Zheng Tang and Jinyou Shen and HAIJIN LI and Yong Zhou and Zhigang Zou},

title = {Urchin-like hierarchical CoZnAl-LDH/RGO/g-C3N4 hybrid as a Z-scheme photocatalyst for efficient and selective CO2 reduction},

journal = {Applied Catalysis B: Environmental},

year = {2019},

volume = {255},

publisher = {Elsevier},

month = {oct},

url = {https://doi.org/10.1016/j.apcatb.2019.117771},

pages = {117771},

doi = {10.1016/j.apcatb.2019.117771}

}

Found error?

Publisher

Elsevier

Journal

Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor

22.1

ISSN

09263373 (Print)
18733883 (Electronic)