Applied Catalysis B: Environmental, volume 282, pages 119600
Construction of highly efficient Z-scheme ZnxCd1-xS/Au@g-C3N4 ternary heterojunction composite for visible-light-driven photocatalytic reduction of CO2 to solar fuel
Puttaswamy Madhusudan
,
Puttaswamy Madhusudan
1
,
Run Shi
,
Run Shi
2
,
Shengling Xiang
2
,
Mengtian Jin
2
,
Bananakere Nanjegowda Chandrashekar
,
Bananakere Nanjegowda Chandrashekar
2
,
Jingwei Wang
2
,
Jingwei Wang
,
Weijun Wang
2
,
Ouwen Peng
2
,
Abbas Amini
,
Abbas Amini
3
,
Chun Cheng
,
Chun-Hu Cheng
1
Publication type: Journal Article
Publication date: 2021-03-01
Journal:
Applied Catalysis B: Environmental
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 22.1
ISSN: 09263373, 18733883
Catalysis
Process Chemistry and Technology
General Environmental Science
Abstract
Converting CO2 into renewable solar fuel using photocatalysts is one of the most ideal solutions for environmental challenges and energy crises. Here, the solid-solid Z-scheme Zn0.5Cd0.5S/Au@g-C3N4 (ZCS/Au@CN) heterojunction showed improved photocatalytic reduction of CO2 due to the enhanced visible light consumption, fast dissolution of photogenerated electron-hole pairs, quick interfacial transfer process of electrons, and enlarged surface area. Under visible-light irradiation, methanol (CH3OH) was produced at a rate of 1.31 μmol h−1 g−1 over ZCS/Au@CN, roughly 43.6 and 32.7 folds higher than those observed over pure ZCS and CN samples. The analytical characterization results verified the role of AuNPs as an electron mediator, which improved the rapid extraction of photoinduced electrons and enhanced the reduction ability of CO2. This work not only demonstrates a facile photodeposition assisted hydrothermal method for fabrication of ZnxCd1-xS/Au@C3N4 heterojunction composite photocatalysts but also demonstrates the possibility of utilizing ternary composites for enhanced photocatalytic reduction of CO2.
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Citations by publishers
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1 publication, 0.69%
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King Saud University
1 publication, 0.69%
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World Scientific
1 publication, 0.69%
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Madhusudan P. et al. Construction of highly efficient Z-scheme ZnxCd1-xS/Au@g-C3N4 ternary heterojunction composite for visible-light-driven photocatalytic reduction of CO2 to solar fuel // Applied Catalysis B: Environmental. 2021. Vol. 282. p. 119600.
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Madhusudan P., Madhusudan P., Shi R., Shi R., Xiang S., Jin M., Chandrashekar B. N., Chandrashekar B. N., Wang J., Wang J., Wang W., Peng O., Amini A., Amini A., Cheng C., Cheng C. Construction of highly efficient Z-scheme ZnxCd1-xS/Au@g-C3N4 ternary heterojunction composite for visible-light-driven photocatalytic reduction of CO2 to solar fuel // Applied Catalysis B: Environmental. 2021. Vol. 282. p. 119600.
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TY - JOUR
DO - 10.1016/j.apcatb.2020.119600
UR - https://doi.org/10.1016/j.apcatb.2020.119600
TI - Construction of highly efficient Z-scheme ZnxCd1-xS/Au@g-C3N4 ternary heterojunction composite for visible-light-driven photocatalytic reduction of CO2 to solar fuel
T2 - Applied Catalysis B: Environmental
AU - Madhusudan, Puttaswamy
AU - Shi, Run
AU - Xiang, Shengling
AU - Jin, Mengtian
AU - Chandrashekar, Bananakere Nanjegowda
AU - Wang, Jingwei
AU - Wang, Weijun
AU - Peng, Ouwen
AU - Amini, Abbas
AU - Cheng, Chun
AU - Madhusudan, Puttaswamy
AU - Shi, Run
AU - Chandrashekar, Bananakere Nanjegowda
AU - Wang, Jingwei
AU - Amini, Abbas
AU - Cheng, Chun-Hu
PY - 2021
DA - 2021/03/01 00:00:00
PB - Elsevier
SP - 119600
VL - 282
SN - 0926-3373
SN - 1873-3883
ER -
Cite this
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@article{2021_Madhusudan,
author = {Puttaswamy Madhusudan and Run Shi and Shengling Xiang and Mengtian Jin and Bananakere Nanjegowda Chandrashekar and Jingwei Wang and Weijun Wang and Ouwen Peng and Abbas Amini and Chun Cheng and Puttaswamy Madhusudan and Run Shi and Bananakere Nanjegowda Chandrashekar and Jingwei Wang and Abbas Amini and Chun-Hu Cheng},
title = {Construction of highly efficient Z-scheme ZnxCd1-xS/Au@g-C3N4 ternary heterojunction composite for visible-light-driven photocatalytic reduction of CO2 to solar fuel},
journal = {Applied Catalysis B: Environmental},
year = {2021},
volume = {282},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/j.apcatb.2020.119600},
pages = {119600},
doi = {10.1016/j.apcatb.2020.119600}
}