Applied Catalysis B: Environmental, volume 294, pages 120257
Advantageous roles of phosphate decorated octahedral CeO2 {111}/g-C3N4 in boosting photocatalytic CO2 reduction: Charge transfer bridge and Lewis basic site
Publication type: Journal Article
Publication date: 2021-10-01
Journal:
Applied Catalysis B: Environmental
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 22.1
ISSN: 09263373, 18733883
Catalysis
Process Chemistry and Technology
General Environmental Science
Abstract
• Phosphate modified octahedral CeO 2 {111} surface with g-C 3 N 4 were synthesized. • PO 4 3− modification improved more Lewis base sites for CO 2 adsorption/activation. • PO 4 3− acted as interfacial bridge for built-in electric field and Z-scheme formation. • P-CeO 2 /g-C 3 N 4 had excellent activity for fast charge transfer and rich active sites. For photocatalytic CO 2 reduction, directional charge-transfer channel and abundant active sites are of significance. Herein, we designed and fabricated phosphate modified octahedral CeO 2 {111} surface coupling with g-C 3 N 4 (P-CeO 2 /g-C 3 N 4 ) for photocatalytic CO 2 reduction, which had superior activity than others, i.e., P-CeO 2 , g-C 3 N 4 , CeO 2 /g-C 3 N 4 . The characterization results revealed the coordination environment of P species, as well as, the presence of hydrogen bond between phosphate and amino. Through the PO 4 3− bridge, the interfacial electrons donated from g-C 3 N 4 to CeO 2 , leading to the Z-scheme formation and fast photo-generated charge transfer. Furthermore, PO 4 3− modification increased more oxygen-containing functional groups on surface, which acted as Lewis basic sites for CO 2 reactant adsorption and activation. Therefore, under the synergistic interaction of charge-transfer channel and abundant active sites, P-CeO 2 /g-C 3 N 4 is a potential photocatalyst for CO 2 reduction.
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Li W. et al. Advantageous roles of phosphate decorated octahedral CeO2 {111}/g-C3N4 in boosting photocatalytic CO2 reduction: Charge transfer bridge and Lewis basic site // Applied Catalysis B: Environmental. 2021. Vol. 294. p. 120257.
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Li W., Li J., Gao F., Wan H., PU Y., Wei X., Chen C., Zou W., Zhu C., Dong L. Advantageous roles of phosphate decorated octahedral CeO2 {111}/g-C3N4 in boosting photocatalytic CO2 reduction: Charge transfer bridge and Lewis basic site // Applied Catalysis B: Environmental. 2021. Vol. 294. p. 120257.
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TY - JOUR
DO - 10.1016/j.apcatb.2021.120257
UR - https://doi.org/10.1016/j.apcatb.2021.120257
TI - Advantageous roles of phosphate decorated octahedral CeO2 {111}/g-C3N4 in boosting photocatalytic CO2 reduction: Charge transfer bridge and Lewis basic site
T2 - Applied Catalysis B: Environmental
AU - Li, Wanqin
AU - Li, Jin
AU - Gao, Fei
AU - Wan, Haiqin
AU - PU, YU
AU - Wei, Xiaoqian
AU - Chen, Chong
AU - Zou, Weixin
AU - Zhu, Chengzhang
AU - Dong, Lin
PY - 2021
DA - 2021/10/01 00:00:00
PB - Elsevier
SP - 120257
VL - 294
SN - 0926-3373
SN - 1873-3883
ER -
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@article{2021_Li,
author = {Wanqin Li and Jin Li and Fei Gao and Haiqin Wan and YU PU and Xiaoqian Wei and Chong Chen and Weixin Zou and Chengzhang Zhu and Lin Dong},
title = {Advantageous roles of phosphate decorated octahedral CeO2 {111}/g-C3N4 in boosting photocatalytic CO2 reduction: Charge transfer bridge and Lewis basic site},
journal = {Applied Catalysis B: Environmental},
year = {2021},
volume = {294},
publisher = {Elsevier},
month = {oct},
url = {https://doi.org/10.1016/j.apcatb.2021.120257},
pages = {120257},
doi = {10.1016/j.apcatb.2021.120257}
}