Applied Catalysis B: Environmental, volume 334, pages 122861
The in-situ formation of supported hydrous ruthenium oxide in aqueous phase during HDO of lignin-derived fractions
Publication type: Journal Article
Publication date: 2023-10-01
Journal:
Applied Catalysis B: Environmental
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 22.1
ISSN: 09263373, 18733883
Catalysis
Process Chemistry and Technology
General Environmental Science
Abstract
The in-situ formation of supported hydrous ruthenium oxide (HRO) from RuO2 over micro-mesoporous materials is reported for the selective hydrogenation of bio-oil under mild reaction conditions (200 °C, 20 bar H2) in an aqueous medium. For the first time, the phase composition of HRO was determined using a variety of characterization techniques. Using synchrotron radiation and in-situ X-ray absorption spectroscopy (XAS), we demonstrated that HRO was generated during the hydrodeoxygenation process. The hydrodeoxygenation (HDO) of real bio-oil was successfully performed at 200 °C, 20 bar H2 on RuO2-containing catalysts. The approximate composition of HRO after 3 h of catalytic hydrogenation, consisted of in approximately equal ratios metallic Ru, RuO2, and RuOOH phases.
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Citations by publishers
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Elsevier
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Multidisciplinary Digital Publishing Institute (MDPI)
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1 publication, 14.29%
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Wiley
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Wiley
1 publication, 14.29%
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Springer Nature
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Springer Nature
1 publication, 14.29%
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1
2
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Naranov E. R. et al. The in-situ formation of supported hydrous ruthenium oxide in aqueous phase during HDO of lignin-derived fractions // Applied Catalysis B: Environmental. 2023. Vol. 334. p. 122861.
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Naranov E. R., Sadovnikov A. A., Arapova O. V., Kuchinskaya T. S., Usoltsev O. A., Bugaev A. L., Janssens K., De Vos D. E., Maximov A. The in-situ formation of supported hydrous ruthenium oxide in aqueous phase during HDO of lignin-derived fractions // Applied Catalysis B: Environmental. 2023. Vol. 334. p. 122861.
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TY - JOUR
DO - 10.1016/j.apcatb.2023.122861
UR - https://doi.org/10.1016%2Fj.apcatb.2023.122861
TI - The in-situ formation of supported hydrous ruthenium oxide in aqueous phase during HDO of lignin-derived fractions
T2 - Applied Catalysis B: Environmental
AU - Naranov, Evgeny R
AU - Sadovnikov, A. A.
AU - Arapova, O V
AU - Kuchinskaya, T S
AU - Usoltsev, Oleg A.
AU - Bugaev, Aram L.
AU - Janssens, Kwinten
AU - De Vos, Dirk E.
AU - Maximov, Anton
PY - 2023
DA - 2023/10/01 00:00:00
PB - Elsevier
SP - 122861
VL - 334
SN - 0926-3373
SN - 1873-3883
ER -
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@article{2023_Naranov,
author = {Evgeny R Naranov and A. A. Sadovnikov and O V Arapova and T S Kuchinskaya and Oleg A. Usoltsev and Aram L. Bugaev and Kwinten Janssens and Dirk E. De Vos and Anton Maximov},
title = {The in-situ formation of supported hydrous ruthenium oxide in aqueous phase during HDO of lignin-derived fractions},
journal = {Applied Catalysis B: Environmental},
year = {2023},
volume = {334},
publisher = {Elsevier},
month = {oct},
url = {https://doi.org/10.1016%2Fj.apcatb.2023.122861},
pages = {122861},
doi = {10.1016/j.apcatb.2023.122861}
}