Applied Surface Science, volume 396, pages 1765-1774

Laser-induced damage thresholds of gold, silver and their alloys in air and water

Publication typeJournal Article
Publication date2017-02-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor6.7
ISSN01694332
Surfaces, Coatings and Films
General Chemistry
General Physics and Astronomy
Condensed Matter Physics
Surfaces and Interfaces
Abstract
The nanosecond-laser-induced damage thresholds of gold, silver and gold-silver alloys of various compositions in air and water have been measured for single-shot irradiation conditions. The experimental results are analyzed theoretically by solving the heat flow equation for the samples irradiated in air and in water taking into account vapor nucleation at the solid-water interface. The damage thresholds of Au-Ag alloys are systematically lower than those for pure metals, both in air and water that is explained by lower thermal conductivities of the alloys. The thresholds measured in air agree well with the calculated melting thresholds for all samples. The damage thresholds in water are found to be considerably higher, by a factor of ∼1.5, than the corresponding thresholds in air. This cannot be explained, in the framework of the used model, neither by the conductive heat transfer to water nor by the vapor pressure effect. Possible reasons for the high damage thresholds in water such as scattering of the incident laser light by the vapor-liquid interface and the critical opalescence in the superheated water are suggested. Optical pump-probe measurements have been performed to study the reflectance dynamics of the surface irradiated in air and water. Comparison of the transient reflectance signal with the calculated nucleation dynamics provides evidence that the both suggested scattering mechanisms are likely to occur during metal ablation in water.

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Sulyaeva V., Shukhov Y. G., Bulgakov A. V. Laser-induced damage thresholds of gold, silver and their alloys in air and water // Applied Surface Science. 2017. Vol. 396. pp. 1765-1774.
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Sulyaeva V., Shukhov Y. G., Bulgakov A. V. Laser-induced damage thresholds of gold, silver and their alloys in air and water // Applied Surface Science. 2017. Vol. 396. pp. 1765-1774.
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RIS Copy
TY - JOUR
DO - 10.1016/j.apsusc.2016.11.221
UR - https://doi.org/10.1016%2Fj.apsusc.2016.11.221
TI - Laser-induced damage thresholds of gold, silver and their alloys in air and water
T2 - Applied Surface Science
AU - Sulyaeva, Veronica
AU - Shukhov, Yuri G.
AU - Bulgakov, Alexander V
PY - 2017
DA - 2017/02/01 00:00:00
PB - Elsevier
SP - 1765-1774
VL - 396
SN - 0169-4332
ER -
BibTex
Cite this
BibTex Copy
@article{2017_Sulyaeva,
author = {Veronica Sulyaeva and Yuri G. Shukhov and Alexander V Bulgakov},
title = {Laser-induced damage thresholds of gold, silver and their alloys in air and water},
journal = {Applied Surface Science},
year = {2017},
volume = {396},
publisher = {Elsevier},
month = {feb},
url = {https://doi.org/10.1016%2Fj.apsusc.2016.11.221},
pages = {1765--1774},
doi = {10.1016/j.apsusc.2016.11.221}
}
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