Chinese Chemical Letters

, volume 36 , issue 3 , pages 109717

A novel square-shaped Zr-substituted polyoxotungstate for the efficient catalytic oxidation of sulfide to sulfone

Dongsheng Yang ¹

Zixin Li ¹

Yaoyao Lian ¹

Zhenqian Fu ¹

Ziyao Fu ¹

Tianjiao Li ¹

Peng-Tao Ma ¹

Guo Ping Yang ²

Hide authors affiliations Show authors affiliations: 2 affiliations

Henan Key Laboratory of Polyoxometalate Chemistry, College of Chemistry and Molecular Sciences, Henan University, Kaifeng 475004, China |

School of Chemistry and Materials Science, Jiangxi Key Laboratory for Mass Spectrometry and Instrumentation, East China University of Technology, Nanchang 330013, China |

Publication type: Journal Article

Publication date: 2025-03-01

Elsevier

Chinese Chemical Letters

scimago Q1

wos Q1

SJR: 1.677

CiteScore: 15.7

Impact factor: 8.9

ISSN: 10018417, 18785964

DOI: 10.1016/j.cclet.2024.109717

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General Chemistry

Abstract

By introduction of hydrogen peroxide into the reaction system of ZrOCl2·8H2O and K14[As2W19O67(H2O)], a novel polyoxometalate K8Na19.5H0.5[Zr2(O2)2(β-AsVW10O38)]4·68H2O (1) has been successfully obtained via one-pot method and systematically characterized by IR, XPS, solid UV spectra, PXRD pattern, and TGA analysis. The analysis of X-ray crystallography exhibits that compound 1 crystallizes in the triclinic space group P-1 and presents a novel square-shaped Zr-substituted tetrameric polyoxometalate. The catalytic oxidation of sulfides by 1 are carried out, which demonstrate that 1 exhibits a good performance for the catalytic oxidation of sulfides to sulfones with high conversion (100%) and high selectivity (100%).

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GOST |

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GOST Copy

Yang D. et al. A novel square-shaped Zr-substituted polyoxotungstate for the efficient catalytic oxidation of sulfide to sulfone // Chinese Chemical Letters. 2025. Vol. 36. No. 3. p. 109717.

GOST all authors (up to 50) Copy

Yang D., Li Z., Lian Y., Fu Z., Fu Z., Li T., Li T., Ma P., Yang G. P. A novel square-shaped Zr-substituted polyoxotungstate for the efficient catalytic oxidation of sulfide to sulfone // Chinese Chemical Letters. 2025. Vol. 36. No. 3. p. 109717.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.cclet.2024.109717

UR - https://linkinghub.elsevier.com/retrieve/pii/S1001841724002365

TI - A novel square-shaped Zr-substituted polyoxotungstate for the efficient catalytic oxidation of sulfide to sulfone

T2 - Chinese Chemical Letters

AU - Yang, Dongsheng

AU - Li, Zixin

AU - Lian, Yaoyao

AU - Fu, Zhenqian

AU - Fu, Ziyao

AU - Li, Tianjiao

AU - Ma, Peng-Tao

AU - Yang, Guo Ping

PY - 2025

DA - 2025/03/01

PB - Elsevier

SP - 109717

IS - 3

VL - 36

SN - 1001-8417

SN - 1878-5964

ER -

BibTex |

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BibTex (up to 50 authors) Copy

@article{2025_Yang,

author = {Dongsheng Yang and Zixin Li and Yaoyao Lian and Zhenqian Fu and Ziyao Fu and Tianjiao Li and Tianjiao Li and Peng-Tao Ma and Guo Ping Yang},

title = {A novel square-shaped Zr-substituted polyoxotungstate for the efficient catalytic oxidation of sulfide to sulfone},

journal = {Chinese Chemical Letters},

year = {2025},

volume = {36},

publisher = {Elsevier},

month = {mar},

url = {https://linkinghub.elsevier.com/retrieve/pii/S1001841724002365},

number = {3},

pages = {109717},

doi = {10.1016/j.cclet.2024.109717}

}

MLA

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MLA Copy

Yang, Dongsheng, et al. “A novel square-shaped Zr-substituted polyoxotungstate for the efficient catalytic oxidation of sulfide to sulfone.” Chinese Chemical Letters, vol. 36, no. 3, Mar. 2025, p. 109717. https://linkinghub.elsevier.com/retrieve/pii/S1001841724002365.

Publisher

Elsevier

Journal

Chinese Chemical Letters

scimago Q1

wos Q1

SJR

1.677

CiteScore

15.7

Impact factor

8.9

ISSN

10018417 (Print)

18785964