Chemical Engineering Journal, volume 396, pages 125347

Multifunctional 2D porous g-C3N4 nanosheets hybridized with 3D hierarchical TiO2 microflowers for selective dye adsorption, antibiotic degradation and CO2 reduction

Wang Qiang ^{1, 2}

Ling-Xia Zhang ²

Yangkun Guo ²

Meng Shen ²

Min Wang ²

Bing Li ^{1, 3}

Jianlin Shi ²

Hide authors affiliations Show authors affiliations: 3 affiliations

School of Mechanical and Power Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai 200237, PR China |

State Key Lab of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 1295 Dingxi Road, Shanghai 200050, PR China |

Collaborative Innovation Center of Clean Energy, Longyan University, 1 North Dongxiao Road, Longyan 364012, PR China |

Publication type: Journal Article

Publication date: 2020-09-01

Elsevier

Journal: Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor: 15.1

ISSN: 13858947, 03009467

DOI: 10.1016/j.cej.2020.125347

Copy DOI

General Chemistry

General Chemical Engineering

Industrial and Manufacturing Engineering

Environmental Chemistry

Abstract

Seeking effective strategy to design multifunctional materials for pollutant removal and solar fuel production is of great significance for solving the worldwide environment and energy problems. In this work, two-dimensional porous graphite-like carbon nitride (p-g-C3N4) nanosheets (NSs) decorated with three-dimensional (3D) hierachical TiO2 microflowers (MFs) were constructed through a facile acid hydrothermal route. 3D TiO2 MFs originating from K2Ti6O13 nanobelts were combined with p-g-C3N4 NSs via solid interfacial connections. By chemical exfoliation and etching, the surface area of g-C3N4 was significantly increased along with the formation of porous structures and C vacancies. Interestingly, the hydrothermally produced two-dimensional (2D) p-g-C3N4 NSs showed extraordinarily selective adsorption towards anionic methyl orange via strong electrostatic attraction. More importantly, such 3D/2D TiO2/p-g-C3N4 micro-nano heteroarchitectures exhibited remarkably improved visible-light photocatalytic properties for antibiotic degradation and CO2 reduction, mainly attributed to the enlarged surface areas and pore volumes, increased adsorption/active sites, improved light absorption and higher separation efficiency of photogenerated charge carriers. This one-pot synthesis method opens new possibilities for rational design of multifunctional g-C3N4-based photocatalysts towards environmental purification and solar energy conversion.

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Citations by journals

	2 4 6 8 10 12 14
Chemical Engineering Journal	Chemical Engineering Journal, 14, 9.72% Chemical Engineering Journal 14 publications, 9.72%
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International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 6, 4.17% International Journal of Hydrogen Energy 6 publications, 4.17%
RSC Advances	RSC Advances, 4, 2.78% RSC Advances 4 publications, 2.78%
Environmental Science and Pollution Research	Environmental Science and Pollution Research, 4, 2.78% Environmental Science and Pollution Research 4 publications, 2.78%
Applied Surface Science	Applied Surface Science, 4, 2.78% Applied Surface Science 4 publications, 2.78%
Journal of Environmental Chemical Engineering	Journal of Environmental Chemical Engineering, 4, 2.78% Journal of Environmental Chemical Engineering 4 publications, 2.78%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 4, 2.78% Journal of Colloid and Interface Science 4 publications, 2.78%
Materials Science in Semiconductor Processing	Materials Science in Semiconductor Processing, 4, 2.78% Materials Science in Semiconductor Processing 4 publications, 2.78%
Catalysts	Catalysts, 3, 2.08% Catalysts 3 publications, 2.08%
Polymers	Polymers, 3, 2.08% Polymers 3 publications, 2.08%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 3, 2.08% Applied Catalysis B: Environmental 3 publications, 2.08%
Journal of Cleaner Production	Journal of Cleaner Production, 3, 2.08% Journal of Cleaner Production 3 publications, 2.08%
Solar RRL	Solar RRL, 3, 2.08% Solar RRL 3 publications, 2.08%
ChemistrySelect	ChemistrySelect, 3, 2.08% ChemistrySelect 3 publications, 2.08%
Advanced Functional Materials	Advanced Functional Materials, 3, 2.08% Advanced Functional Materials 3 publications, 2.08%
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Inorganic Chemistry Communication	Inorganic Chemistry Communication, 2, 1.39% Inorganic Chemistry Communication 2 publications, 1.39%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 2, 1.39% Journal of Alloys and Compounds 2 publications, 1.39%
Nanotechnology	Nanotechnology, 2, 1.39% Nanotechnology 2 publications, 1.39%
Processes	Processes, 2, 1.39% Processes 2 publications, 1.39%
Energy & Fuels	Energy & Fuels, 2, 1.39% Energy & Fuels 2 publications, 1.39%
New Journal of Chemistry	New Journal of Chemistry, 2, 1.39% New Journal of Chemistry 2 publications, 1.39%
Chemical Communications	Chemical Communications, 2, 1.39% Chemical Communications 2 publications, 1.39%
Catalysis Science and Technology	Catalysis Science and Technology, 2, 1.39% Catalysis Science and Technology 2 publications, 1.39%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 2, 1.39% Physical Chemistry Chemical Physics 2 publications, 1.39%
Optical Materials	Optical Materials, 2, 1.39% Optical Materials 2 publications, 1.39%
Chemosphere	Chemosphere, 1, 0.69% Chemosphere 1 publication, 0.69%
Journal of Analytical Science and Technology	Journal of Analytical Science and Technology, 1, 0.69% Journal of Analytical Science and Technology 1 publication, 0.69%
	2 4 6 8 10 12 14

Citations by publishers

	10 20 30 40 50 60 70 80
Elsevier	Elsevier, 76, 52.78% Elsevier 76 publications, 52.78%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 17, 11.81% Royal Society of Chemistry (RSC) 17 publications, 11.81%
Wiley	Wiley, 13, 9.03% Wiley 13 publications, 9.03%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 12, 8.33% Multidisciplinary Digital Publishing Institute (MDPI) 12 publications, 8.33%
Springer Nature	Springer Nature, 10, 6.94% Springer Nature 10 publications, 6.94%
American Chemical Society (ACS)	American Chemical Society (ACS), 5, 3.47% American Chemical Society (ACS) 5 publications, 3.47%
IOP Publishing	IOP Publishing, 3, 2.08% IOP Publishing 3 publications, 2.08%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.69% Taiwan Institute of Chemical Engineers 1 publication, 0.69%
SAGE	SAGE, 1, 0.69% SAGE 1 publication, 0.69%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.69% Frontiers Media S.A. 1 publication, 0.69%
Taylor & Francis	Taylor & Francis, 1, 0.69% Taylor & Francis 1 publication, 0.69%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.69% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.69%
	10 20 30 40 50 60 70 80

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Qiang W. et al. Multifunctional 2D porous g-C3N4 nanosheets hybridized with 3D hierarchical TiO2 microflowers for selective dye adsorption, antibiotic degradation and CO2 reduction // Chemical Engineering Journal. 2020. Vol. 396. p. 125347.

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Qiang W., Zhang L., Guo Y., Shen M., Wang M., Li B., Shi J. Multifunctional 2D porous g-C3N4 nanosheets hybridized with 3D hierarchical TiO2 microflowers for selective dye adsorption, antibiotic degradation and CO2 reduction // Chemical Engineering Journal. 2020. Vol. 396. p. 125347.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.cej.2020.125347

UR - https://doi.org/10.1016/j.cej.2020.125347

TI - Multifunctional 2D porous g-C3N4 nanosheets hybridized with 3D hierarchical TiO2 microflowers for selective dye adsorption, antibiotic degradation and CO2 reduction

T2 - Chemical Engineering Journal

AU - Qiang, Wang

AU - Zhang, Ling-Xia

AU - Guo, Yangkun

AU - Shen, Meng

AU - Wang, Min

AU - Li, Bing

AU - Shi, Jianlin

PY - 2020

DA - 2020/09/01 00:00:00

PB - Elsevier

SP - 125347

VL - 396

SN - 1385-8947

SN - 0300-9467

ER -

BibTex

Cite this

BibTex Copy

@article{2020_Qiang,

author = {Wang Qiang and Ling-Xia Zhang and Yangkun Guo and Meng Shen and Min Wang and Bing Li and Jianlin Shi},

title = {Multifunctional 2D porous g-C3N4 nanosheets hybridized with 3D hierarchical TiO2 microflowers for selective dye adsorption, antibiotic degradation and CO2 reduction},

journal = {Chemical Engineering Journal},

year = {2020},

volume = {396},

publisher = {Elsevier},

month = {sep},

url = {https://doi.org/10.1016/j.cej.2020.125347},

pages = {125347},

doi = {10.1016/j.cej.2020.125347}

}

Found error?

Publisher

Elsevier

Journal

Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor

15.1

ISSN

13858947 (Print)
03009467 (Print)