Journal of Alloys and Compounds, volume 852, pages 156955
One-pot synthesis of novel ternary Fe3N/Fe2O3/C3N4 photocatalyst for efficient removal of rhodamine B and CO2 reduction
Publication type: Journal Article
Publication date: 2021-01-01
Journal:
Journal of Alloys and Compounds
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 6.2
ISSN: 09258388
Materials Chemistry
Metals and Alloys
Mechanical Engineering
Mechanics of Materials
Abstract
The novel ternary Fe 3 N/Fe 2 O 3 /C 3 N 4 photocatalyst was prepared by thermal pyrolysis of potassium ferricyanide in melamine. The structural, morphological and physico-chemical properties of the photocatalyst were characterized by a multi-technique approach. Photocatalytic experiments supported that 0.04 g of the photocatalyst was able to totally remove 5 ppm of rhodamine B (RhB) solution under acidic condition with the rate constant of 0.1 min −1 in less than 30 min. According to spin-trapping ESR analysis, • OH radicals play a key role in the RhB photodegradation implying Z-scheme mechanism is applicable to our system. Moreover, the evolution rate of CO and CH 4 over the photocatalyst was 8.03 and 1.6 μmol g −1 h −1 , respectively, which was much higher than the reference photocatalysts under the same conditions. The enhanced photocatalytic performance of this system is attributed to the unique ternary heterojunction between the interfaces of g-C 3 N 4 , Fe 3 N and Fe 2 O 3 , which effectively suppressed the charge carriers recombination. • A novel ternary Fe 3 N/Fe 2 O 3 /C 3 N 4 photocatalyst was prepared from cheap raw materials. • The interfacial Fe 3 N regions act as electron mediator and bandgap modifier. • The mechanism of RhB photodegradation was well discussed based on EPR experiments. • The ternary Fe 3 N/Fe 2 O 3 /C 3 N 4 photocatalyst showed efficient photocatalytic CH 4 evolution performance.
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Padervand M. et al. One-pot synthesis of novel ternary Fe3N/Fe2O3/C3N4 photocatalyst for efficient removal of rhodamine B and CO2 reduction // Journal of Alloys and Compounds. 2021. Vol. 852. p. 156955.
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Padervand M., Rhimi B., Wang C. One-pot synthesis of novel ternary Fe3N/Fe2O3/C3N4 photocatalyst for efficient removal of rhodamine B and CO2 reduction // Journal of Alloys and Compounds. 2021. Vol. 852. p. 156955.
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TY - JOUR
DO - 10.1016/j.jallcom.2020.156955
UR - https://doi.org/10.1016/j.jallcom.2020.156955
TI - One-pot synthesis of novel ternary Fe3N/Fe2O3/C3N4 photocatalyst for efficient removal of rhodamine B and CO2 reduction
T2 - Journal of Alloys and Compounds
AU - Padervand, Mohsen
AU - Rhimi, Baker
AU - Wang, Chuanyi
PY - 2021
DA - 2021/01/01 00:00:00
PB - Elsevier
SP - 156955
VL - 852
SN - 0925-8388
ER -
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@article{2021_Padervand,
author = {Mohsen Padervand and Baker Rhimi and Chuanyi Wang},
title = {One-pot synthesis of novel ternary Fe3N/Fe2O3/C3N4 photocatalyst for efficient removal of rhodamine B and CO2 reduction},
journal = {Journal of Alloys and Compounds},
year = {2021},
volume = {852},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/j.jallcom.2020.156955},
pages = {156955},
doi = {10.1016/j.jallcom.2020.156955}
}