Open Access

Journal of Colloid and Interface Science, volume 564, pages 406-417

Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance

Qijun Tang

Zhuxing Sun ¹

Shuang Deng ²

Haiqiang Wang ³

Zhongbiao Wu ³

Hide authors affiliations Show authors affiliations: 3 affiliations

School of Environmental Science and Engineering, Shanghai Jiao Tong University, Shanghai, 200240, PR China |

Chinese Research Academy of Environmental Sciences, Beijing 100012, PR China. |

Key Laboratory of Environment Remediation and Ecological Health, Ministry of Education, College of Environmental & Resources Science, Zhejiang University, Hangzhou 310058, PR China |

Publication type: Journal Article

Publication date: 2020-03-01

Elsevier

Journal: Journal of Colloid and Interface Science

Quartile SCImago

Quartile WOS

Impact factor: 9.9

ISSN: 00219797, 10957103

DOI: 10.1016/j.jcis.2019.12.091

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Surfaces, Coatings and Films

Electronic, Optical and Magnetic Materials

Colloid and Surface Chemistry

Biomaterials

Abstract

Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti3C2) was used as a noble metal-free co-catalyst by simply mixing graphitic carbon nitride (g-C3N4) and alkalized Ti3C2. The carbon monoxide evolution rate of the optimized composite (5%TCOH-CN) from photocatalytic reduction of CO2 was 5.9 times higher than that of pure g-C3N4. Alkalized Ti3C2 was responsible for the superior photocatalytic activity due to its excellent electrical conductivity and large CO2 adsorption capacity. Furthermore, the separation of the photo-induced electron-hole pairs was greatly enhanced because of the large Fermi level difference between alkalized Ti3C2 and pure g-C3N4. This work demonstrates the potential of MXenes as noble metal-free co-catalyst for photocatalysis processes such as carbon dioxide reduction reaction and nitrogen reduction reaction.

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Citations by journals

	5 10 15 20 25
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 21, 9.68% Journal of Colloid and Interface Science 21 publications, 9.68%
ACS Symposium Series	ACS Symposium Series, 10, 4.61% ACS Symposium Series 10 publications, 4.61%
Chemical Engineering Journal	Chemical Engineering Journal, 8, 3.69% Chemical Engineering Journal 8 publications, 3.69%
Energy & Fuels	Energy & Fuels, 7, 3.23% Energy & Fuels 7 publications, 3.23%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 6, 2.76% Journal of Materials Chemistry A 6 publications, 2.76%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 5, 2.3% Coordination Chemistry Reviews 5 publications, 2.3%
Journal of CO2 Utilization	Journal of CO2 Utilization, 5, 2.3% Journal of CO2 Utilization 5 publications, 2.3%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 5, 2.3% Journal of Alloys and Compounds 5 publications, 2.3%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 5, 2.3% Applied Catalysis B: Environmental 5 publications, 2.3%
Catalysis Science and Technology	Catalysis Science and Technology, 5, 2.3% Catalysis Science and Technology 5 publications, 2.3%
Colloids and Surfaces A: Physicochemical and Engineering Aspects	Colloids and Surfaces A: Physicochemical and Engineering Aspects, 4, 1.84% Colloids and Surfaces A: Physicochemical and Engineering Aspects 4 publications, 1.84%
Journal of Materials Science and Technology	Journal of Materials Science and Technology, 4, 1.84% Journal of Materials Science and Technology 4 publications, 1.84%
Separation and Purification Technology	Separation and Purification Technology, 4, 1.84% Separation and Purification Technology 4 publications, 1.84%
Journal of Environmental Chemical Engineering	Journal of Environmental Chemical Engineering, 4, 1.84% Journal of Environmental Chemical Engineering 4 publications, 1.84%
Chemistry - A European Journal	Chemistry - A European Journal, 4, 1.84% Chemistry - A European Journal 4 publications, 1.84%
Environmental Science and Pollution Research	Environmental Science and Pollution Research, 3, 1.38% Environmental Science and Pollution Research 3 publications, 1.38%
Materials Science in Semiconductor Processing	Materials Science in Semiconductor Processing, 3, 1.38% Materials Science in Semiconductor Processing 3 publications, 1.38%
Applied Surface Science	Applied Surface Science, 3, 1.38% Applied Surface Science 3 publications, 1.38%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 1.38% ACS applied materials & interfaces 3 publications, 1.38%
Nanoscale	Nanoscale, 3, 1.38% Nanoscale 3 publications, 1.38%
New Journal of Chemistry	New Journal of Chemistry, 3, 1.38% New Journal of Chemistry 3 publications, 1.38%
Sustainable Energy and Fuels	Sustainable Energy and Fuels, 3, 1.38% Sustainable Energy and Fuels 3 publications, 1.38%
Advanced Materials Interfaces	Advanced Materials Interfaces, 2, 0.92% Advanced Materials Interfaces 2 publications, 0.92%
Nano Materials Science	Nano Materials Science, 2, 0.92% Nano Materials Science 2 publications, 0.92%
Journal of Molecular Liquids	Journal of Molecular Liquids, 2, 0.92% Journal of Molecular Liquids 2 publications, 0.92%
Chinese Journal of Catalysis	Chinese Journal of Catalysis, 2, 0.92% Chinese Journal of Catalysis 2 publications, 0.92%
Journal of Energy Chemistry	Journal of Energy Chemistry, 2, 0.92% Journal of Energy Chemistry 2 publications, 0.92%
Chemosphere	Chemosphere, 2, 0.92% Chemosphere 2 publications, 0.92%
Materials Today Energy	Materials Today Energy, 2, 0.92% Materials Today Energy 2 publications, 0.92%
	5 10 15 20 25

Citations by publishers

	20 40 60 80 100 120
Elsevier	Elsevier, 108, 49.77% Elsevier 108 publications, 49.77%
American Chemical Society (ACS)	American Chemical Society (ACS), 30, 13.82% American Chemical Society (ACS) 30 publications, 13.82%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 27, 12.44% Royal Society of Chemistry (RSC) 27 publications, 12.44%
Springer Nature	Springer Nature, 17, 7.83% Springer Nature 17 publications, 7.83%
Wiley	Wiley, 17, 7.83% Wiley 17 publications, 7.83%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 4, 1.84% Multidisciplinary Digital Publishing Institute (MDPI) 4 publications, 1.84%
Taylor & Francis	Taylor & Francis, 2, 0.92% Taylor & Francis 2 publications, 0.92%
EDP Sciences	EDP Sciences, 1, 0.46% EDP Sciences 1 publication, 0.46%
Tianjin Daxue/Tianjin University	Tianjin Daxue/Tianjin University, 1, 0.46% Tianjin Daxue/Tianjin University 1 publication, 0.46%
Institution of Chemical Engineers	Institution of Chemical Engineers, 1, 0.46% Institution of Chemical Engineers 1 publication, 0.46%
KeAi Communications Co.	KeAi Communications Co., 1, 0.46% KeAi Communications Co. 1 publication, 0.46%
Chemical Industry Press	Chemical Industry Press, 1, 0.46% Chemical Industry Press 1 publication, 0.46%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.46% Taiwan Institute of Chemical Engineers 1 publication, 0.46%
IOP Publishing	IOP Publishing, 1, 0.46% IOP Publishing 1 publication, 0.46%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.46% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.46%
	20 40 60 80 100 120

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Tang Q. et al. Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance // Journal of Colloid and Interface Science. 2020. Vol. 564. pp. 406-417.

GOST all authors (up to 50) Copy

Tang Q., Sun Z., Deng S., Wang H., Wu Z. Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance // Journal of Colloid and Interface Science. 2020. Vol. 564. pp. 406-417.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.jcis.2019.12.091

UR - https://doi.org/10.1016/j.jcis.2019.12.091

TI - Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance

T2 - Journal of Colloid and Interface Science

AU - Tang, Qijun

AU - Sun, Zhuxing

AU - Deng, Shuang

AU - Wang, Haiqiang

AU - Wu, Zhongbiao

PY - 2020

DA - 2020/03/01 00:00:00

PB - Elsevier

SP - 406-417

VL - 564

SN - 0021-9797

SN - 1095-7103

ER -

BibTex

Cite this

BibTex Copy

@article{2020_Tang,

author = {Qijun Tang and Zhuxing Sun and Shuang Deng and Haiqiang Wang and Zhongbiao Wu},

title = {Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance},

journal = {Journal of Colloid and Interface Science},

year = {2020},

volume = {564},

publisher = {Elsevier},

month = {mar},

url = {https://doi.org/10.1016/j.jcis.2019.12.091},

pages = {406--417},

doi = {10.1016/j.jcis.2019.12.091}

}

Found error?

Publisher

Elsevier

Journal

Journal of Colloid and Interface Science

Quartile SCImago

Quartile WOS

Impact factor

9.9

ISSN

00219797 (Print)
10957103 (Electronic)