Journal of Nuclear Materials, volume 385, issue 1, pages 25-27

69Ga NMR and magnetic susceptibility in δ-phase of Pu1−xGax (x=0.05, x=0.08) alloys

Publication typeJournal Article
Publication date2009-03-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor3.1
ISSN00223115
General Materials Science
Nuclear and High Energy Physics
Nuclear Energy and Engineering
Abstract
69Ga nuclear magnetic resonance spectra, line shifts (69K) and nuclear spin-lattice relaxation rate 69 T 1 - 1 have been measured in the 20 years aged Pu0.95Ga0.05 and in fresh prepared Pu0.92Ga0.08 alloys, stabilized δ-phase, at magnetic field of 9.4 T in the temperature range (10–500) K. The line shift and 69 T 1 - 1 are determined correspondingly by the static and fluctuating-in-time parts of the local magnetic field that originates in transferred hyperfine coupling the Ga nuclear spin with the nearest f-electron environment of more magnetic Pu. Temperature behavior of the resonance properties is found the same in fresh Pu0.92Ga0.08 and aged Pu0.95Ga0.05 alloy. The NMR results are in favor that δ-phase of Pu1−xGax alloys represents at T > 200 K the Kondo lattice, in which the localized electronic spins fluctuate independently from each other without any macroscopic coherence. The coherent state like in heavy-fermion liquids emerges in Pu0.95Ga0.05 below T∗ = 200 K. A little bit higher estimate of crossover temperature T∗ = 250 K was founded for Pu0.92Ga0.08.

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Piskunov Y. et al. 69Ga NMR and magnetic susceptibility in δ-phase of Pu1−xGax (x=0.05, x=0.08) alloys // Journal of Nuclear Materials. 2009. Vol. 385. No. 1. pp. 25-27.
GOST all authors (up to 50) Copy
Piskunov Y., Mikhalev K., Buzlukov A., Gerashenko A., Verkhovskii S., Ogloblichev V., Arkhipov V., Korolev A., Zouev Y., Svyatov I., Mikhalev K., Ogloblichev V. V. 69Ga NMR and magnetic susceptibility in δ-phase of Pu1−xGax (x=0.05, x=0.08) alloys // Journal of Nuclear Materials. 2009. Vol. 385. No. 1. pp. 25-27.
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TY - JOUR
DO - 10.1016/j.jnucmat.2008.09.047
UR - https://doi.org/10.1016%2Fj.jnucmat.2008.09.047
TI - 69Ga NMR and magnetic susceptibility in δ-phase of Pu1−xGax (x=0.05, x=0.08) alloys
T2 - Journal of Nuclear Materials
AU - Piskunov, Yu.
AU - Mikhalev, K
AU - Buzlukov, A.
AU - Gerashenko, A.
AU - Verkhovskii, Stanislav
AU - Ogloblichev, V
AU - Arkhipov, V.
AU - Korolev, A.
AU - Zouev, Yu.
AU - Svyatov, I
AU - Mikhalev, Konstantin
AU - Ogloblichev, V. V.
PY - 2009
DA - 2009/03/01 00:00:00
PB - Elsevier
SP - 25-27
IS - 1
VL - 385
SN - 0022-3115
ER -
BibTex |
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@article{2009_Piskunov,
author = {Yu. Piskunov and K Mikhalev and A. Buzlukov and A. Gerashenko and Stanislav Verkhovskii and V Ogloblichev and V. Arkhipov and A. Korolev and Yu. Zouev and I Svyatov and Konstantin Mikhalev and V. V. Ogloblichev},
title = {69Ga NMR and magnetic susceptibility in δ-phase of Pu1−xGax (x=0.05, x=0.08) alloys},
journal = {Journal of Nuclear Materials},
year = {2009},
volume = {385},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016%2Fj.jnucmat.2008.09.047},
number = {1},
pages = {25--27},
doi = {10.1016/j.jnucmat.2008.09.047}
}
MLA
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MLA Copy
Piskunov, Yu., et al. “69Ga NMR and magnetic susceptibility in δ-phase of Pu1−xGax (x=0.05, x=0.08) alloys.” Journal of Nuclear Materials, vol. 385, no. 1, Mar. 2009, pp. 25-27. https://doi.org/10.1016%2Fj.jnucmat.2008.09.047.
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