, volume 328 , pages 111446

Synthesis of ZSM-5 catalysts via microwave-assisted heating method for military jet fuel cracking into petroleum gas

Sungtak Kim ¹

Jochen Lauterbach ²

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Department of Chemical Engineering & Applied Chemistry Chungnam National University Daejeon 34134 Republic of Korea |

Smartstate Center for Strategic Approaches to the Generation of Electricity (SAGE), Department of Chemical Engineering, University of South Carolina, Columbia, SC 29201, USA |

Publication type: Journal Article

Publication date: 2021-12-01

Elsevier

Microporous and Mesoporous Materials

scimago Q1

wos Q2

SJR: 1.003

CiteScore: 11.0

Impact factor: 4.7

ISSN: 13871811, 18733093

DOI: 10.1016/j.micromeso.2021.111446

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General Chemistry

Condensed Matter Physics

General Materials Science

Mechanics of Materials

Abstract

Hydrothermal synthesis of ZSM-5 zeolites with different Si/Al ratios was conducted by using a microwave-assisted heating method. Their characteristics, such as morphology, porosity, acidity, and the catalytic performance for the cracking reaction of military jet fuel JP-8, were compared with ZSM-5 zeolites obtained via a conventional heating synthesis method. The microwave-assisted heating method contributed to bigger crystal sizes of the ZSM-5 zeolite as well as broader mesopore size distribution in the zeolite crystal with the same Si/Al ratio. Acidity analysis revealed ZSM-5 zeolites with similar acid properties could be produced with both heating methods. As the different heating methods attributed to different crystal sizes and roughness of the synthesized ZSM-5 zeolite, which are influenced by the fast crystal growth and consumption of silicon and aluminum precursor during the hydrothermal synthesis, different petroleum gas yields, and paraffinic product selectivity were observed from the ZSM-5 zeolite produced via microwave-assisted heating method. • Microwave-assisted heating method for hydrothermal synthesis (MH) of ZSM-5 zeolites were investigated. • MH method exhibited the same acidic properties but bigger and fairer surface of crystal due to fast crystallization. • Catalytic cracking reaction of military jet fuel was firstly explored with the ZSM-5 catalyst synthesized from MH method.

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Kim S., Lauterbach J. Synthesis of ZSM-5 catalysts via microwave-assisted heating method for military jet fuel cracking into petroleum gas // Microporous and Mesoporous Materials. 2021. Vol. 328. p. 111446.

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RIS Copy

TY - JOUR

DO - 10.1016/j.micromeso.2021.111446

UR - https://doi.org/10.1016/j.micromeso.2021.111446

TI - Synthesis of ZSM-5 catalysts via microwave-assisted heating method for military jet fuel cracking into petroleum gas

T2 - Microporous and Mesoporous Materials

AU - Kim, Sungtak

AU - Lauterbach, Jochen

PY - 2021

DA - 2021/12/01

PB - Elsevier

SP - 111446

VL - 328

SN - 1387-1811

SN - 1873-3093

ER -

BibTex

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BibTex (up to 50 authors) Copy

@article{2021_Kim,

author = {Sungtak Kim and Jochen Lauterbach},

title = {Synthesis of ZSM-5 catalysts via microwave-assisted heating method for military jet fuel cracking into petroleum gas},

journal = {Microporous and Mesoporous Materials},

year = {2021},

volume = {328},

publisher = {Elsevier},

month = {dec},

url = {https://doi.org/10.1016/j.micromeso.2021.111446},

pages = {111446},

doi = {10.1016/j.micromeso.2021.111446}

}

Publisher

Elsevier

Journal

Microporous and Mesoporous Materials

scimago Q1

wos Q2

SJR

1.003

CiteScore

11.0

Impact factor

4.7

ISSN

13871811 (Print)

18733093