Phase equilibria in SO2 + H2O: the sulfur dioxide gas hydrate, two liquid phases, and the gas phase in the temperature range 273 to 400 K and at pressures up to 400 MPa
Тип публикации: Journal Article
Дата публикации: 1979-04-01
scimago Q2
wos Q2
БС2
SJR: 0.47
CiteScore: 5.5
Impact factor: 2.2
ISSN: 00219614, 10963626
Physical and Theoretical Chemistry
Atomic and Molecular Physics, and Optics
General Materials Science
Краткое описание
The H + L 1 + L 2 phase relations, where L 1 and L 2 stand for the liquid phases rich in hydrate former (sulfur dioxide) and water respectively and H for the gas hydrate, in sulfur dioxide + water have been investigated in the pressure range 1 to 400 MPa. The threephase line shows a maximum temperature at (293.68 ± 0.1) K at (3072 ± 20) atm. It can be concluded that the system shows a congruent melting line of the gas hydrate from (2100 ± 10) atm, up to higher pressures showing a temperature maximum at (294.05 ± 0.05) K and (3450 ± 20) atm. The critical mixing curve L 1 = L 2 has been partly determined. From the experimental results it is not certain whether or not this curve shows a temperature minimum. In addition the L 1 + L 2 + G relations in the temperature range 285 to 395 K have been investigated. Finally the solubility of sulfur dioxide in liquid water as a function of temperature has been determined in the presence of the second liquid and gas.
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Van Berkum J. G., Diepen G. A. M. Phase equilibria in SO2 + H2O: the sulfur dioxide gas hydrate, two liquid phases, and the gas phase in the temperature range 273 to 400 K and at pressures up to 400 MPa // Journal of Chemical Thermodynamics. 1979. Vol. 11. No. 4. pp. 317-334.
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Van Berkum J. G., Diepen G. A. M. Phase equilibria in SO2 + H2O: the sulfur dioxide gas hydrate, two liquid phases, and the gas phase in the temperature range 273 to 400 K and at pressures up to 400 MPa // Journal of Chemical Thermodynamics. 1979. Vol. 11. No. 4. pp. 317-334.
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TY - JOUR
DO - 10.1016/0021-9614(79)90053-3
UR - https://doi.org/10.1016/0021-9614(79)90053-3
TI - Phase equilibria in SO2 + H2O: the sulfur dioxide gas hydrate, two liquid phases, and the gas phase in the temperature range 273 to 400 K and at pressures up to 400 MPa
T2 - Journal of Chemical Thermodynamics
AU - Van Berkum, J G
AU - Diepen, G A M
PY - 1979
DA - 1979/04/01
PB - Elsevier
SP - 317-334
IS - 4
VL - 11
SN - 0021-9614
SN - 1096-3626
ER -
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@article{1979_Van Berkum,
author = {J G Van Berkum and G A M Diepen},
title = {Phase equilibria in SO2 + H2O: the sulfur dioxide gas hydrate, two liquid phases, and the gas phase in the temperature range 273 to 400 K and at pressures up to 400 MPa},
journal = {Journal of Chemical Thermodynamics},
year = {1979},
volume = {11},
publisher = {Elsevier},
month = {apr},
url = {https://doi.org/10.1016/0021-9614(79)90053-3},
number = {4},
pages = {317--334},
doi = {10.1016/0021-9614(79)90053-3}
}
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Van Berkum, J. G., and G A M Diepen. “Phase equilibria in SO2 + H2O: the sulfur dioxide gas hydrate, two liquid phases, and the gas phase in the temperature range 273 to 400 K and at pressures up to 400 MPa.” Journal of Chemical Thermodynamics, vol. 11, no. 4, Apr. 1979, pp. 317-334. https://doi.org/10.1016/0021-9614(79)90053-3.