Surface Science

, том 201 , издание 1-2 , страницы 195-210

XPS and UPS studies of oxygen adsorption over clean and carbon-modified silver surfaces

Andrei Boronin ¹

V I Bukhityarov ¹

A.L. VISHNEVSKII ¹

G. K. Boreskov ¹

V.I Savchenko ¹

Скрыть аффилиации авторов Показать аффилиации авторов: 1 аффилиация

Institute of Catalysis, Novosibirsk 630090, USSR | |

Тип публикации: Journal Article

Дата публикации: 1988-01-01

Elsevier

Surface Science

scimago Q2

wos Q3

БС2

SJR: 0.419

CiteScore: 3.5

Impact factor: 1.8

ISSN: 00396028, 18792758

DOI: 10.1016/0039-6028(88)90606-1

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Materials Chemistry

Surfaces, Coatings and Films

Condensed Matter Physics

Surfaces and Interfaces

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Oxygen adsorption over clean and carbon-modified silver surfaces has been studied by XPS and UPS in the temperature range 300–700 K under O 2 pressures from 10 −3 to 10 Pa. Adsorption over a clean silver surface at T >420 K leads to the appearance of atomically adsorbed oxygen on the surface, which is characterized by E B (O 1s) = 528.5 eV, high reactivity towards CO and a heat of adsorption of 100 kJ/mol. Subsurface oxygen is formed in small amounts. Increasing the O 2 pressure to 10 Pa does not lead to the formation of new adsorption forms. At T E B (C 1s)=287.8 eV and E B (O 1s)=530.6 eV are formed on the surface. During interaction of O 2 with the silver surface containing dissolved carbon in the bulk, the surface is modified by O and C due to CO bond formation in the subsurface region. The O 2 adsorption at high pressures (10 Pa) on the modified surface is characterized by the formation of a new oxygen state with E B =530.3 eV. Based on UPS spectra characteristics (the peak at E B θ 9.5 eV), this state is supposed to be of molecular form.

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Водянкина Ольга

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Гетерогенный катализ

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Свинцицкий Дмитрий

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Boronin A. et al. XPS and UPS studies of oxygen adsorption over clean and carbon-modified silver surfaces // Surface Science. 1988. Vol. 201. No. 1-2. pp. 195-210.

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Boronin A., Bukhityarov V. I., VISHNEVSKII A., Boreskov G. K., Savchenko V. XPS and UPS studies of oxygen adsorption over clean and carbon-modified silver surfaces // Surface Science. 1988. Vol. 201. No. 1-2. pp. 195-210.

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TY - JOUR

DO - 10.1016/0039-6028(88)90606-1

UR - https://doi.org/10.1016/0039-6028(88)90606-1

TI - XPS and UPS studies of oxygen adsorption over clean and carbon-modified silver surfaces

T2 - Surface Science

AU - Boronin, Andrei

AU - Bukhityarov, V I

AU - VISHNEVSKII, A.L.

AU - Boreskov, G. K.

AU - Savchenko, V.I

PY - 1988

DA - 1988/01/01

PB - Elsevier

SP - 195-210

IS - 1-2

VL - 201

SN - 0039-6028

SN - 1879-2758

ER -

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@article{1988_Boronin,

author = {Andrei Boronin and V I Bukhityarov and A.L. VISHNEVSKII and G. K. Boreskov and V.I Savchenko},

title = {XPS and UPS studies of oxygen adsorption over clean and carbon-modified silver surfaces},

journal = {Surface Science},

year = {1988},

volume = {201},

publisher = {Elsevier},

month = {jan},

url = {https://doi.org/10.1016/0039-6028(88)90606-1},

number = {1-2},

pages = {195--210},

doi = {10.1016/0039-6028(88)90606-1}

}

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Boronin, Andrei, et al. “XPS and UPS studies of oxygen adsorption over clean and carbon-modified silver surfaces.” Surface Science, vol. 201, no. 1-2, Jan. 1988, pp. 195-210. https://doi.org/10.1016/0039-6028(88)90606-1.