Surface Science

, том 208 , издание 1-2 , страницы 13-33

Periodic perturbations of the oscillatory CO oxidation on Pt(110)

Тип публикации: Journal Article

Дата публикации: 1989-01-01

Elsevier

Surface Science

scimago Q2

wos Q3

БС2

SJR: 0.419

CiteScore: 3.5

Impact factor: 1.8

ISSN: 00396028, 18792758

DOI: 10.1016/0039-6028(89)90034-4

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Materials Chemistry

Surfaces, Coatings and Films

Condensed Matter Physics

Surfaces and Interfaces

Краткое описание

The catalytic oxidation of CO on a Pt(110) surface at low pressures operated under conditions ( p o 2 , p co, T ) of isothermal, self-sustained kinetic oscillations was subject to periodic perturbations of the oxygen partial pressure with variable frequency and (small) amplitude. The large variety of the effects observed in the response of the system is classified according to the principles of the bifurcation theory for periodically perturbed chemical systems: Besides harmonic resonance, nine bands of subharmonic or superharmonic entrainment could be identified. Quasi-periodic oscillations were obtained between the entrainment bands and showed the effect of frequency pulling. Upon approaching an entrainment edge markedly prolonged relaxation behavior (critical slowing down) was observed. The qualitative differences to previous findings with Pt(100) can be traced back to differences in the mechanisms dominating spatial self-organization.

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Eiswirth M., MOLLER P., Ertl G. Periodic perturbations of the oscillatory CO oxidation on Pt(110) // Surface Science. 1989. Vol. 208. No. 1-2. pp. 13-33.

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Eiswirth M., MOLLER P., Ertl G. Periodic perturbations of the oscillatory CO oxidation on Pt(110) // Surface Science. 1989. Vol. 208. No. 1-2. pp. 13-33.

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TY - JOUR

DO - 10.1016/0039-6028(89)90034-4

UR - https://doi.org/10.1016/0039-6028(89)90034-4

TI - Periodic perturbations of the oscillatory CO oxidation on Pt(110)

T2 - Surface Science

AU - Eiswirth, M.

AU - MOLLER, P

AU - Ertl, G

PY - 1989

DA - 1989/01/01

PB - Elsevier

SP - 13-33

IS - 1-2

VL - 208

SN - 0039-6028

SN - 1879-2758

ER -

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BibTex (до 50 авторов) Скопировать

@article{1989_Eiswirth,

author = {M. Eiswirth and P MOLLER and G Ertl},

title = {Periodic perturbations of the oscillatory CO oxidation on Pt(110)},

journal = {Surface Science},

year = {1989},

volume = {208},

publisher = {Elsevier},

month = {jan},

url = {https://doi.org/10.1016/0039-6028(89)90034-4},

number = {1-2},

pages = {13--33},

doi = {10.1016/0039-6028(89)90034-4}

}

MLA

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MLA Скопировать

Eiswirth, M., et al. “Periodic perturbations of the oscillatory CO oxidation on Pt(110).” Surface Science, vol. 208, no. 1-2, Jan. 1989, pp. 13-33. https://doi.org/10.1016/0039-6028(89)90034-4.

Издатель

Elsevier

Журнал

Surface Science

scimago Q2

wos Q3

БС2

SJR

0.419

CiteScore

3.5

Impact factor

1.8

ISSN

00396028 (Print, Electronic)

18792758