Carbon dioxide reforming of methane to synthesis gas over supported Ni catalysts
Тип публикации: Journal Article
Дата публикации: 1994-12-01
scimago Q1
wos Q1
БС1
SJR: 1.05
CiteScore: 11.2
Impact factor: 5.3
ISSN: 09205861, 18734308
General Chemistry
Catalysis
Краткое описание
Carbon dioxide reforming of methane to synthesis gas has been investigated over supported Ni catalysts in the temperature range of 500–850°C. Addition of CaO (10mol%) promoter to the Ni/γ-Al2O3 resulted in an increase of reaction rate and an improvement of catalyst stability, which may be related to enhanced reducibility of the promoted catalyst. The kinetic studies show that the overall reaction can be described by a Langmuir-Hinshelwood mechanistic scheme, assuming that methane dissociation is the rate determining step. In addition to adsorbed CO and formate species, three types of carbonaceous species, Cα, Cβ and Cγ, were found to exist on the Ni catalyst. While the active Cα, species is suggested to be responsible for CO formation, the less active Cβ and Cγ species are attributed to causing catalyst deactivation.
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ГОСТ
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Zhang Z. L., Verykios X. Carbon dioxide reforming of methane to synthesis gas over supported Ni catalysts // Catalysis Today. 1994. Vol. 21. No. 2-3. pp. 589-595.
ГОСТ со всеми авторами (до 50)
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Zhang Z. L., Verykios X. Carbon dioxide reforming of methane to synthesis gas over supported Ni catalysts // Catalysis Today. 1994. Vol. 21. No. 2-3. pp. 589-595.
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RIS
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TY - JOUR
DO - 10.1016/0920-5861(94)80183-5
UR - https://doi.org/10.1016/0920-5861(94)80183-5
TI - Carbon dioxide reforming of methane to synthesis gas over supported Ni catalysts
T2 - Catalysis Today
AU - Zhang, Z. L.
AU - Verykios, X.E.
PY - 1994
DA - 1994/12/01
PB - Elsevier
SP - 589-595
IS - 2-3
VL - 21
SN - 0920-5861
SN - 1873-4308
ER -
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BibTex (до 50 авторов)
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@article{1994_Zhang,
author = {Z. L. Zhang and X.E. Verykios},
title = {Carbon dioxide reforming of methane to synthesis gas over supported Ni catalysts},
journal = {Catalysis Today},
year = {1994},
volume = {21},
publisher = {Elsevier},
month = {dec},
url = {https://doi.org/10.1016/0920-5861(94)80183-5},
number = {2-3},
pages = {589--595},
doi = {10.1016/0920-5861(94)80183-5}
}
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MLA
Скопировать
Zhang, Z. L., and X.E. Verykios. “Carbon dioxide reforming of methane to synthesis gas over supported Ni catalysts.” Catalysis Today, vol. 21, no. 2-3, Dec. 1994, pp. 589-595. https://doi.org/10.1016/0920-5861(94)80183-5.