Applied Catalysis B: Environmental, volume 203, pages 633-640

Synthesis of hierarchical bismuth-rich Bi4O5BrxI2-x solid solutions for enhanced photocatalytic activities of CO2 conversion and Cr(VI) reduction under visible light

Yang Bai ¹

Liqun Ye ¹

陈挺 Ting Chen ¹

Pingquan Wang ¹

Li Wang ²

X. Shi ¹

Po-Keung Wong ³

Hide authors affiliations Show authors affiliations: 3 affiliations

State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation, School of Oil & Natural Gas Engineering, Southwest Petroleum University, Chengdu 610500, China |

Key Laboratory of Ecological Security for Water Source Region of Mid-line Project of South-to-North Water Diversion of Henan Province, College of Chemistry and Pharmaceutical Engineering, Nanyang Normal University, Nanyang 473061, China |

School of Life Sciences, The Chinese University of Hong Kong, Shatin, NT, Hong Kong Special Administrative Region, China |

Publication type: Journal Article

Publication date: 2017-04-01

Elsevier

Journal: Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor: 22.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2016.10.066

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Catalysis

Process Chemistry and Technology

General Environmental Science

Abstract

Bismuth oxyhalides (BiOX, X = Br, I) photocatalysts are rarely applied for photocatalytic reduction reaction withthe photo-induced electron, as this is impeded by their low conduction band. As a widely used approach for enhancing the photocatalytic reduction activity, bismuth-rich strategy results the bismuth content of BiOX photocatalysts increasing. In this paper, a solid solutions of bismuth-rich Bi4O5BrxI2-x were prepared applying the molecular precursor method. Bi4O5BrxI2-x were characterized by X-ray diffraction (XRD), field emission scanning electron microscopy (FESEM), transmission electron microscopy (TEM), element mapping, Brunauer–Emmett–Teller surface analysis (BET), UV–vis diffuse reflectance spectroscopy (DRS), and X-ray photoelectron spectroscopy (XPS). The obtained photocatalytic data showed that Bi4O5BrxI2-x solid solutions had higher photocatalytic activities than Bi4O5Br2 and Bi4O5I2. At an optimal ratio of x = 1, the Bi4O5BrI photocatalyst showed the highest photocatalytic reduction activity for CO2 conversion (22.85 μmol h−1 g−1 CO generation, AQE was 0.372 at 400 nm) and Cr(VI) removal (88%). CO2 adsorption data and CO2 temperature programmed desorption (CO2-TPD) revealed that Bi4O5BrI exhibited the highest chemical adsorption ability of CO2 molecules Photocurrent and electrochemical impedance (EIS) spectroscopy demonstrated the enhanced photo-induced carrier separation efficiency of Bi4O5BrI. These mechanistic studies suggest that Bi4O5BrxI2-x solid solutions are excellent photocatalysts for solar fuel generation and environmental remediation.

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Elsevier	Elsevier, 99, 61.49% Elsevier 99 publications, 61.49%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 16, 9.94% Royal Society of Chemistry (RSC) 16 publications, 9.94%
Springer Nature	Springer Nature, 15, 9.32% Springer Nature 15 publications, 9.32%
American Chemical Society (ACS)	American Chemical Society (ACS), 10, 6.21% American Chemical Society (ACS) 10 publications, 6.21%
Wiley	Wiley, 10, 6.21% Wiley 10 publications, 6.21%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 1.24% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 1.24%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 2, 1.24% Taiwan Institute of Chemical Engineers 2 publications, 1.24%
Institution of Engineering and Technology (IET)	Institution of Engineering and Technology (IET), 1, 0.62% Institution of Engineering and Technology (IET) 1 publication, 0.62%
The Electrochemical Society	The Electrochemical Society, 1, 0.62% The Electrochemical Society 1 publication, 0.62%
Pleiades Publishing	Pleiades Publishing, 1, 0.62% Pleiades Publishing 1 publication, 0.62%
IOP Publishing	IOP Publishing, 1, 0.62% IOP Publishing 1 publication, 0.62%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.62% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.62%
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Bai Y. et al. Synthesis of hierarchical bismuth-rich Bi4O5BrxI2-x solid solutions for enhanced photocatalytic activities of CO2 conversion and Cr(VI) reduction under visible light // Applied Catalysis B: Environmental. 2017. Vol. 203. pp. 633-640.

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Bai Y., Ye L., Ting Chen 陈., Wang P., Wang L., Shi X., Wong P. Synthesis of hierarchical bismuth-rich Bi4O5BrxI2-x solid solutions for enhanced photocatalytic activities of CO2 conversion and Cr(VI) reduction under visible light // Applied Catalysis B: Environmental. 2017. Vol. 203. pp. 633-640.

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RIS Copy

TY - JOUR

DO - 10.1016/j.apcatb.2016.10.066

UR - https://doi.org/10.1016/j.apcatb.2016.10.066

TI - Synthesis of hierarchical bismuth-rich Bi4O5BrxI2-x solid solutions for enhanced photocatalytic activities of CO2 conversion and Cr(VI) reduction under visible light

T2 - Applied Catalysis B: Environmental

AU - Bai, Yang

AU - Ye, Liqun

AU - Ting Chen, 陈挺

AU - Wang, Pingquan

AU - Wang, Li

AU - Shi, X.

AU - Wong, Po-Keung

PY - 2017

DA - 2017/04/01 00:00:00

PB - Elsevier

SP - 633-640

VL - 203

SN - 0926-3373

SN - 1873-3883

ER -

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BibTex Copy

@article{2017_Bai,

author = {Yang Bai and Liqun Ye and 陈挺 Ting Chen and Pingquan Wang and Li Wang and X. Shi and Po-Keung Wong},

title = {Synthesis of hierarchical bismuth-rich Bi4O5BrxI2-x solid solutions for enhanced photocatalytic activities of CO2 conversion and Cr(VI) reduction under visible light},

journal = {Applied Catalysis B: Environmental},

year = {2017},

volume = {203},

publisher = {Elsevier},

month = {apr},

url = {https://doi.org/10.1016/j.apcatb.2016.10.066},

pages = {633--640},

doi = {10.1016/j.apcatb.2016.10.066}

}

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Publisher

Elsevier

Journal

Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor

22.1

ISSN

09263373 (Print)
18733883 (Electronic)

	2 4 6 8 10 12 14
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 14, 8.7% Applied Catalysis B: Environmental 14 publications, 8.7%
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Applied Surface Science	Applied Surface Science, 7, 4.35% Applied Surface Science 7 publications, 4.35%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 6, 3.73% Journal of Materials Science: Materials in Electronics 6 publications, 3.73%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 6, 3.73% Journal of Alloys and Compounds 6 publications, 3.73%
Separation and Purification Technology	Separation and Purification Technology, 4, 2.48% Separation and Purification Technology 4 publications, 2.48%
Inorganic Chemistry Communication	Inorganic Chemistry Communication, 4, 2.48% Inorganic Chemistry Communication 4 publications, 2.48%
ACS applied materials & interfaces	ACS applied materials & interfaces, 4, 2.48% ACS applied materials & interfaces 4 publications, 2.48%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 4, 2.48% Journal of Materials Chemistry A 4 publications, 2.48%
Catalysis Science and Technology	Catalysis Science and Technology, 4, 2.48% Catalysis Science and Technology 4 publications, 2.48%
Research on Chemical Intermediates	Research on Chemical Intermediates, 3, 1.86% Research on Chemical Intermediates 3 publications, 1.86%
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Coordination Chemistry Reviews	Coordination Chemistry Reviews, 3, 1.86% Coordination Chemistry Reviews 3 publications, 1.86%
Nano Energy	Nano Energy, 3, 1.86% Nano Energy 3 publications, 1.86%
Science of the Total Environment	Science of the Total Environment, 3, 1.86% Science of the Total Environment 3 publications, 1.86%
ACS Catalysis	ACS Catalysis, 2, 1.24% ACS Catalysis 2 publications, 1.24%
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Materials Science in Semiconductor Processing	Materials Science in Semiconductor Processing, 2, 1.24% Materials Science in Semiconductor Processing 2 publications, 1.24%
Chinese Chemical Letters	Chinese Chemical Letters, 2, 1.24% Chinese Chemical Letters 2 publications, 1.24%
Journal of Photochemistry and Photobiology A: Chemistry	Journal of Photochemistry and Photobiology A: Chemistry, 2, 1.24% Journal of Photochemistry and Photobiology A: Chemistry 2 publications, 1.24%
Journal of Molecular Structure	Journal of Molecular Structure, 2, 1.24% Journal of Molecular Structure 2 publications, 1.24%
Journal of Hazardous Materials	Journal of Hazardous Materials, 2, 1.24% Journal of Hazardous Materials 2 publications, 1.24%
Journal of the Taiwan Institute of Chemical Engineers	Journal of the Taiwan Institute of Chemical Engineers, 2, 1.24% Journal of the Taiwan Institute of Chemical Engineers 2 publications, 1.24%
ACS Sustainable Chemistry and Engineering	ACS Sustainable Chemistry and Engineering, 2, 1.24% ACS Sustainable Chemistry and Engineering 2 publications, 1.24%
CrystEngComm	CrystEngComm, 2, 1.24% CrystEngComm 2 publications, 1.24%
Journal of Environmental Chemical Engineering	Journal of Environmental Chemical Engineering, 2, 1.24% Journal of Environmental Chemical Engineering 2 publications, 1.24%
Micro and Nano Letters	Micro and Nano Letters, 1, 0.62% Micro and Nano Letters 1 publication, 0.62%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 1, 0.62% Journal of the Electrochemical Society 1 publication, 0.62%
	2 4 6 8 10 12 14