Applied Catalysis B: Environmental, volume 241, pages 528-538

All-solid-state artificial Z-scheme porous g-C3N4/Sn2S3-DETA heterostructure photocatalyst with enhanced performance in photocatalytic CO2 reduction

Yao Huo ¹

Jinfeng Zhang ¹

Qiang Li ¹

Jiali Lv ^{2, 3}

Guangping Zhu ¹

Changhao Liang ^{2, 3}

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College of Physics and Electronic Information, Anhui Key Laboratory of Energetic Materials, Huaibei Normal University, Huaibei 235000, PR China |

Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, PR China |

Key Laboratory of Materials Physics and Anhui Key Laboratory of Nanomaterials and Nanotechnology, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, 230021, PR China |

Publication type: Journal Article

Publication date: 2019-02-01

Elsevier

Journal: Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor: 22.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2018.09.073

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Catalysis

Process Chemistry and Technology

General Environmental Science

Abstract

• Novel porous g-C 3 N 4 /Sn 2 S 3 -DETA composites were obtained. • The composites exhibited excellent photocatalytic CO 2 reduction and stability. • Direct Z-scheme photocatalytic mechanism used to explain activity enhancement. • DFT calculation further confirms the presence of direct Z-scheme mechanism. Nowadays, the increasing CO 2 emissions have attracted widespread attentions and it is necessary to reduce CO 2 emissions to solve the global warming problem. So photocatalytic reduction of CO 2 into chemical fuels is a promising strategy. Here, a Z-scheme porous g-C 3 N 4 /Sn 2 S 3 -diethylenetriamine (Pg-C 3 N 4 /Sn 2 S 3 -DETA) composite without an electron intermediary is designed. Photocatalytic performance of the as-fabricated samples is investigated on the basis of photocatalytic CO 2 reduction (PCR) to form CH 4 and CH 3 OH. We find that the Z-scheme heterostructure photocatalysts show a higher PCR performance than Pg-C 3 N 4 and Sn 2 S 3 -DETA. An optimized Pg-C 3 N 4 /Sn 2 S 3 -DETA heterostructure sample displays high CH 4 production rate of 4.84 μmol h −1 g −1 and CH 3 OH-production rate of 1.35 μmol h −1 g −1 with 5% Pg-C 3 N 4 content. The superior PCR performance could be ascribed to the special structure of a direct Z-scheme Pg-C 3 N 4 /Sn 2 S 3 -DETA photocatalyst, which is beneficial to efficient separation of electron-hole pairs. Density functional theory (DFT) calculation further confirms the presence of direct Z-scheme mechanism. This Z-scheme heterostructure photocatalyst with superior performance may inaugurate the perspective on a new promising hierarchy of materials on CO 2 photoreduction.

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Nanoscale	Nanoscale, 4, 1.15% Nanoscale 4 publications, 1.15%
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Solid State Sciences	Solid State Sciences, 3, 0.86% Solid State Sciences 3 publications, 0.86%
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Journal of Industrial and Engineering Chemistry	Journal of Industrial and Engineering Chemistry, 3, 0.86% Journal of Industrial and Engineering Chemistry 3 publications, 0.86%
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Citations by publishers

	50 100 150 200 250
Elsevier	Elsevier, 224, 64.37% Elsevier 224 publications, 64.37%
Wiley	Wiley, 35, 10.06% Wiley 35 publications, 10.06%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 32, 9.2% Royal Society of Chemistry (RSC) 32 publications, 9.2%
American Chemical Society (ACS)	American Chemical Society (ACS), 27, 7.76% American Chemical Society (ACS) 27 publications, 7.76%
Springer Nature	Springer Nature, 11, 3.16% Springer Nature 11 publications, 3.16%
IOP Publishing	IOP Publishing, 4, 1.15% IOP Publishing 4 publications, 1.15%
Frontiers Media S.A.	Frontiers Media S.A., 3, 0.86% Frontiers Media S.A. 3 publications, 0.86%
World Scientific	World Scientific, 2, 0.57% World Scientific 2 publications, 0.57%
KeAi Communications Co.	KeAi Communications Co., 2, 0.57% KeAi Communications Co. 2 publications, 0.57%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 2, 0.57% Korean Society of Industrial Engineering Chemistry 2 publications, 0.57%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 2, 0.57% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 2 publications, 0.57%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 0.29% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 0.29%
King Saud University	King Saud University, 1, 0.29% King Saud University 1 publication, 0.29%
IOS Press	IOS Press, 1, 0.29% IOS Press 1 publication, 0.29%
Chinese Ceramic Society	Chinese Ceramic Society, 1, 0.29% Chinese Ceramic Society 1 publication, 0.29%
	50 100 150 200 250

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Huo Y. et al. All-solid-state artificial Z-scheme porous g-C3N4/Sn2S3-DETA heterostructure photocatalyst with enhanced performance in photocatalytic CO2 reduction // Applied Catalysis B: Environmental. 2019. Vol. 241. pp. 528-538.

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Huo Y., Zhang J., Li Q., Lv J., Zhu G., Liang C. All-solid-state artificial Z-scheme porous g-C3N4/Sn2S3-DETA heterostructure photocatalyst with enhanced performance in photocatalytic CO2 reduction // Applied Catalysis B: Environmental. 2019. Vol. 241. pp. 528-538.

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RIS Copy

TY - JOUR

DO - 10.1016/j.apcatb.2018.09.073

UR - https://doi.org/10.1016/j.apcatb.2018.09.073

TI - All-solid-state artificial Z-scheme porous g-C3N4/Sn2S3-DETA heterostructure photocatalyst with enhanced performance in photocatalytic CO2 reduction

T2 - Applied Catalysis B: Environmental

AU - Huo, Yao

AU - Zhang, Jinfeng

AU - Liang, Changhao

AU - Li, Qiang

AU - Lv, Jiali

AU - Zhu, Guangping

PY - 2019

DA - 2019/02/01 00:00:00

PB - Elsevier

SP - 528-538

VL - 241

SN - 0926-3373

SN - 1873-3883

ER -

BibTex

Cite this

BibTex Copy

@article{2019_Huo,

author = {Yao Huo and Jinfeng Zhang and Changhao Liang and Qiang Li and Jiali Lv and Guangping Zhu},

title = {All-solid-state artificial Z-scheme porous g-C3N4/Sn2S3-DETA heterostructure photocatalyst with enhanced performance in photocatalytic CO2 reduction},

journal = {Applied Catalysis B: Environmental},

year = {2019},

volume = {241},

publisher = {Elsevier},

month = {feb},

url = {https://doi.org/10.1016/j.apcatb.2018.09.073},

pages = {528--538},

doi = {10.1016/j.apcatb.2018.09.073}

}

Found error?

Publisher

Elsevier

Journal

Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor

22.1

ISSN

09263373 (Print)
18733883 (Electronic)