Applied Catalysis B: Environmental, volume 263, pages 118314

Efficient Z-scheme photocatalysts of ultrathin g-C3N4-wrapped Au/TiO2-nanocrystals for enhanced visible-light-driven conversion of CO2 with H2O

Chujun Wang ¹

Yilong Zhao ¹

Hui Xu ²

Yifei Li ¹

Yuechang Wei ¹

Jian Liu ¹

Zhen Zhao ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Chang Ping, Beijing 102249, PR China |

Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China. |

Publication type: Journal Article

Publication date: 2020-04-01

Elsevier

Journal: Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor: 22.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2019.118314

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Catalysis

Process Chemistry and Technology

General Environmental Science

Abstract

Z-scheme-type photocatalysts with two photochemical systems of graphic-C3N4 (g-C3N4) and anatase TiO2 (A-TiO2) nanocrystals combined with Au nanoparticles (NPs) [(Au/A-TiO2)@g-C3N4] were successfully fabricated. The surface heterojunction between coexposed {001} and {101} facets in A-TiO2 nanocrystals improves separation efficiency of photoelectrons and holes. Supported Au NPs gather and transfer the stimulated electrons originated from A-TiO2 to g-C3N4. Wrapped g-C3N4 nanosheets can not only trap the photoelectrons, but also its surface π bond can improve adsorption capabilities for CO2. (Au/A-TiO2)@g-C3N4 catalysts with enriched surface photoelectrons and CO2 exhibit high photocatalytic activity for visible-light-driven conversion of CO2, i.e., the formation rates of CH4 and CO over (Au/A-TiO2)@C3N4-5 catalyst are 37.4 and 21.7 μmol g−1 h−1, respectively. The selectivity for CO2 reduction is higher than 99%, and the selectivity of CH4 product increases from 1.4% to 63.3%. The innovation of Z-scheme-type photocatalysts is expected to provide new inspiration for artificial simulation photosynthesis.

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Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 16, 7.21% Applied Catalysis B: Environmental 16 publications, 7.21%
Chemical Engineering Journal	Chemical Engineering Journal, 13, 5.86% Chemical Engineering Journal 13 publications, 5.86%
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Journal of Environmental Chemical Engineering	Journal of Environmental Chemical Engineering, 4, 1.8% Journal of Environmental Chemical Engineering 4 publications, 1.8%
ACS applied materials & interfaces	ACS applied materials & interfaces, 4, 1.8% ACS applied materials & interfaces 4 publications, 1.8%
Catalysts	Catalysts, 3, 1.35% Catalysts 3 publications, 1.35%
Nanomaterials	Nanomaterials, 3, 1.35% Nanomaterials 3 publications, 1.35%
Molecules	Molecules, 3, 1.35% Molecules 3 publications, 1.35%
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Ceramics International	Ceramics International, 3, 1.35% Ceramics International 3 publications, 1.35%
Chemistry - A European Journal	Chemistry - A European Journal, 3, 1.35% Chemistry - A European Journal 3 publications, 1.35%
Inorganic Chemistry	Inorganic Chemistry, 3, 1.35% Inorganic Chemistry 3 publications, 1.35%
Energy & Fuels	Energy & Fuels, 3, 1.35% Energy & Fuels 3 publications, 1.35%
ACS Catalysis	ACS Catalysis, 3, 1.35% ACS Catalysis 3 publications, 1.35%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 3, 1.35% Journal of Materials Chemistry A 3 publications, 1.35%
Frontiers in Chemistry	Frontiers in Chemistry, 2, 0.9% Frontiers in Chemistry 2 publications, 0.9%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 2, 0.9% Journal of Materials Science: Materials in Electronics 2 publications, 0.9%
Journal of Physics and Chemistry of Solids	Journal of Physics and Chemistry of Solids, 2, 0.9% Journal of Physics and Chemistry of Solids 2 publications, 0.9%
Materials Today Energy	Materials Today Energy, 2, 0.9% Materials Today Energy 2 publications, 0.9%
	2 4 6 8 10 12 14 16

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	20 40 60 80 100 120 140
Elsevier	Elsevier, 126, 56.76% Elsevier 126 publications, 56.76%
American Chemical Society (ACS)	American Chemical Society (ACS), 25, 11.26% American Chemical Society (ACS) 25 publications, 11.26%
Wiley	Wiley, 19, 8.56% Wiley 19 publications, 8.56%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 18, 8.11% Royal Society of Chemistry (RSC) 18 publications, 8.11%
Springer Nature	Springer Nature, 13, 5.86% Springer Nature 13 publications, 5.86%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 12, 5.41% Multidisciplinary Digital Publishing Institute (MDPI) 12 publications, 5.41%
Frontiers Media S.A.	Frontiers Media S.A., 2, 0.9% Frontiers Media S.A. 2 publications, 0.9%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 0.45% American Institute of Physics (AIP) 1 publication, 0.45%
Pleiades Publishing	Pleiades Publishing, 1, 0.45% Pleiades Publishing 1 publication, 0.45%
Walter de Gruyter	Walter de Gruyter, 1, 0.45% Walter de Gruyter 1 publication, 0.45%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.45% OAE Publishing Inc. 1 publication, 0.45%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.45% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.45%
	20 40 60 80 100 120 140

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Wang C. et al. Efficient Z-scheme photocatalysts of ultrathin g-C3N4-wrapped Au/TiO2-nanocrystals for enhanced visible-light-driven conversion of CO2 with H2O // Applied Catalysis B: Environmental. 2020. Vol. 263. p. 118314.

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Wang C., Zhao Y., Xu H., Li Y., Wei Y., Liu J., Zhao Z. Efficient Z-scheme photocatalysts of ultrathin g-C3N4-wrapped Au/TiO2-nanocrystals for enhanced visible-light-driven conversion of CO2 with H2O // Applied Catalysis B: Environmental. 2020. Vol. 263. p. 118314.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.apcatb.2019.118314

UR - https://doi.org/10.1016/j.apcatb.2019.118314

TI - Efficient Z-scheme photocatalysts of ultrathin g-C3N4-wrapped Au/TiO2-nanocrystals for enhanced visible-light-driven conversion of CO2 with H2O

T2 - Applied Catalysis B: Environmental

AU - Wang, Chujun

AU - Zhao, Yilong

AU - Xu, Hui

AU - Li, Yifei

AU - Wei, Yuechang

AU - Liu, Jian

AU - Zhao, Zhen

PY - 2020

DA - 2020/04/01 00:00:00

PB - Elsevier

SP - 118314

VL - 263

SN - 0926-3373

SN - 1873-3883

ER -

BibTex

Cite this

BibTex Copy

@article{2020_Wang,

author = {Chujun Wang and Yilong Zhao and Hui Xu and Yifei Li and Yuechang Wei and Jian Liu and Zhen Zhao},

title = {Efficient Z-scheme photocatalysts of ultrathin g-C3N4-wrapped Au/TiO2-nanocrystals for enhanced visible-light-driven conversion of CO2 with H2O},

journal = {Applied Catalysis B: Environmental},

year = {2020},

volume = {263},

publisher = {Elsevier},

month = {apr},

url = {https://doi.org/10.1016/j.apcatb.2019.118314},

pages = {118314},

doi = {10.1016/j.apcatb.2019.118314}

}

Found error?

Publisher

Elsevier

Journal

Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor

22.1

ISSN

09263373 (Print)
18733883 (Electronic)