Chemical Engineering Journal, volume 425, pages 131402

Photocatalytic carbon dioxide reduction: Exploring the role of ultrathin 2D graphitic carbon nitride (g-C3N4)

Maansi Aggarwal ¹

Haripada Bhunia ¹

Nagaraj P. Shetti ²

Mallikarjuna N. Nadagouda ³

Eilhann E. Kwon ⁴

Young-Kwon Park ⁵

Tejraj M. Aminabhavi ^{6, 7}

Hide authors affiliations Show authors affiliations: 7 affiliations

School of Chemistry and Biochemistry Thapar Institute of Engineering and Technology Patiala 147004 India |

School of Advanced Sciences, KLE Technological University, Vidyanagar, Hubballi - 580031, Karnataka, India. |

Department of Mechanical and Materials Engineering Wright State University Dayton, Ohio 45435, USA |

⁴

Department of Environment and Energy Sejong University Seoul 05006 South Korea |

⁵

School of Environmental Engineering, University of Seoul, Seoul, 02504, South Korea. |

⁶

Department of Chemistry, Karnatak University, Dharwad 580 003, India |

⁷

School of Advanced Sciences, KLE Technological University, Vidyanagar, Hubballi-580031, Karnataka, India |

Publication type: Journal Article

Publication date: 2021-12-01

Elsevier

Journal: Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor: 15.1

ISSN: 13858947, 03009467

DOI: 10.1016/j.cej.2021.131402

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General Chemistry

General Chemical Engineering

Industrial and Manufacturing Engineering

Environmental Chemistry

Abstract

• Effect of critical parameters of 2D g-C 3 N 4 on CO 2 reduction is discussed. • Effective charge separation for high selectivity and activity with 2D g-C 3 N 4 in solar fuels is necessary. • Impact of crystal design on 2D g-C 3 N 4 , which controls the fate of reaction intermediates, is reviewed. • Strategic approaches to improve photocatalytic CO 2 reduction with 2D g-C 3 N 4 are suggested. Photocatalytic CO 2 reduction is the key strategic factor to mitigate the detrimental consequences arising from greenhouse gases (predominantly anthropogenic CO 2 ). Products (CH 4 , C 2 H 6 , CH 3 OH, C 2 H 5 OH, etc.,) that are derived from the reduction of CO 2 could be promising alternatives to petro-derived fuel/chemicals. Even though a great deal of efforts has been devoted to increase the conversion efficiency of CO 2 , the technical readiness level (TRL) has not yet been fully matured. This review emphasizes on the emerging functional material ultrathin two-dimensional (2D) nanosheet graphitic carbon nitride (g-C 3 N 4 ) for the reduction of CO 2 into value-added products. Physico-chemical properties of 2D-cabon nitride (sizeable surface-to-volume ratio, supplementary active sites onto the surface, shorter diffusion length, bandgap tuning, atomic thickness, and bulk to surface charge transportation) governing the photocatalytic activity are discussed. This review provides recent advances in 2D-carbon nitride photocatalysts to highlight the ongoing challenges and new strategies to optimize their functionality for improved selectivity for CO 2 conversion.

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Citations by publishers

	5 10 15 20 25 30 35 40 45
Elsevier	Elsevier, 42, 55.26% Elsevier 42 publications, 55.26%
Wiley	Wiley, 11, 14.47% Wiley 11 publications, 14.47%
Springer Nature	Springer Nature, 5, 6.58% Springer Nature 5 publications, 6.58%
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Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 4, 5.26% Royal Society of Chemistry (RSC) 4 publications, 5.26%
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The Electrochemical Society	The Electrochemical Society, 1, 1.32% The Electrochemical Society 1 publication, 1.32%
Frontiers Media S.A.	Frontiers Media S.A., 1, 1.32% Frontiers Media S.A. 1 publication, 1.32%
Asian Journal of Chemistry	Asian Journal of Chemistry, 1, 1.32% Asian Journal of Chemistry 1 publication, 1.32%
IWA Publishing	IWA Publishing, 1, 1.32% IWA Publishing 1 publication, 1.32%
Pleiades Publishing	Pleiades Publishing, 1, 1.32% Pleiades Publishing 1 publication, 1.32%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.32% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.32%
	5 10 15 20 25 30 35 40 45

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Aggarwal M. et al. Photocatalytic carbon dioxide reduction: Exploring the role of ultrathin 2D graphitic carbon nitride (g-C3N4) // Chemical Engineering Journal. 2021. Vol. 425. p. 131402.

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Aggarwal M., Bhunia H., Shetti N. P., Nadagouda M. N., Kwon E. E., Park Y., Aminabhavi T. M. Photocatalytic carbon dioxide reduction: Exploring the role of ultrathin 2D graphitic carbon nitride (g-C3N4) // Chemical Engineering Journal. 2021. Vol. 425. p. 131402.

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Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.cej.2021.131402

UR - https://doi.org/10.1016/j.cej.2021.131402

TI - Photocatalytic carbon dioxide reduction: Exploring the role of ultrathin 2D graphitic carbon nitride (g-C3N4)

T2 - Chemical Engineering Journal

AU - Aggarwal, Maansi

AU - Bhunia, Haripada

AU - Shetti, Nagaraj P.

AU - Nadagouda, Mallikarjuna N.

AU - Kwon, Eilhann E.

AU - Park, Young-Kwon

AU - Aminabhavi, Tejraj M.

PY - 2021

DA - 2021/12/01 00:00:00

PB - Elsevier

SP - 131402

VL - 425

SN - 1385-8947

SN - 0300-9467

ER -

BibTex

Cite this

BibTex Copy

@article{2021_Aggarwal,

author = {Maansi Aggarwal and Haripada Bhunia and Nagaraj P. Shetti and Mallikarjuna N. Nadagouda and Eilhann E. Kwon and Young-Kwon Park and Tejraj M. Aminabhavi},

title = {Photocatalytic carbon dioxide reduction: Exploring the role of ultrathin 2D graphitic carbon nitride (g-C3N4)},

journal = {Chemical Engineering Journal},

year = {2021},

volume = {425},

publisher = {Elsevier},

month = {dec},

url = {https://doi.org/10.1016/j.cej.2021.131402},

pages = {131402},

doi = {10.1016/j.cej.2021.131402}

}

Found error?

Publisher

Elsevier

Journal

Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor

15.1

ISSN

13858947 (Print)
03009467 (Print)