Open Access
Journal of Colloid and Interface Science, volume 564, pages 406-417
Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance
2
Chinese Research Academy of Environmental Sciences, Beijing 100012, PR China.
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Publication type: Journal Article
Publication date: 2020-03-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.9
ISSN: 00219797, 10957103
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Colloid and Surface Chemistry
Biomaterials
Abstract
Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti3C2) was used as a noble metal-free co-catalyst by simply mixing graphitic carbon nitride (g-C3N4) and alkalized Ti3C2. The carbon monoxide evolution rate of the optimized composite (5%TCOH-CN) from photocatalytic reduction of CO2 was 5.9 times higher than that of pure g-C3N4. Alkalized Ti3C2 was responsible for the superior photocatalytic activity due to its excellent electrical conductivity and large CO2 adsorption capacity. Furthermore, the separation of the photo-induced electron-hole pairs was greatly enhanced because of the large Fermi level difference between alkalized Ti3C2 and pure g-C3N4. This work demonstrates the potential of MXenes as noble metal-free co-catalyst for photocatalysis processes such as carbon dioxide reduction reaction and nitrogen reduction reaction.
Top-30
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Citations by publishers
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Tang Q. et al. Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance // Journal of Colloid and Interface Science. 2020. Vol. 564. pp. 406-417.
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Tang Q., Sun Z., Deng S., Wang H., Wu Z. Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance // Journal of Colloid and Interface Science. 2020. Vol. 564. pp. 406-417.
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TY - JOUR
DO - 10.1016/j.jcis.2019.12.091
UR - https://doi.org/10.1016/j.jcis.2019.12.091
TI - Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance
T2 - Journal of Colloid and Interface Science
AU - Tang, Qijun
AU - Sun, Zhuxing
AU - Deng, Shuang
AU - Wang, Haiqiang
AU - Wu, Zhongbiao
PY - 2020
DA - 2020/03/01 00:00:00
PB - Elsevier
SP - 406-417
VL - 564
SN - 0021-9797
SN - 1095-7103
ER -
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@article{2020_Tang,
author = {Qijun Tang and Zhuxing Sun and Shuang Deng and Haiqiang Wang and Zhongbiao Wu},
title = {Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance},
journal = {Journal of Colloid and Interface Science},
year = {2020},
volume = {564},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/j.jcis.2019.12.091},
pages = {406--417},
doi = {10.1016/j.jcis.2019.12.091}
}