Open Access

Journal of CO2 Utilization, volume 38, pages 16-23

Solar-driven CO2 conversion over Co2+ doped 0D/2D TiO2/g-C3N4 heterostructure: Insights into the role of Co2+ and cocatalyst

Hainan Shi ¹

Jun Du ¹

Jungang Hou ¹

Wenjun Ni ¹

Chunshan Song ^{2, 3}

Keyan Li ¹

Gagik G. Gurzadyan ¹

Linna Gao ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

State Key Laboratory of Fine Chemicals, PSU-DUT Joint Center for Energy Research, School of Chemical Engineering, Dalian University of Technology,Dalian 116024,PR China |

EMS Energy Institute, PSU-DUT Joint Center for Energy Research and Department of Energy & Mineral Engineering, Pennsylvania State University, University Park, Pennsylvania 16802, United States |

State Key Laboratory of Fine Chemicals, PSU-DUT Joint Center for Energy Research, School of Chemical Engineering, Dalian University of Technology, Dalian, 116024, PR China |

Publication type: Journal Article

Publication date: 2020-05-01

Elsevier

Journal: Journal of CO2 Utilization

Quartile SCImago

Quartile WOS

Impact factor: 7.7

ISSN: 22129820, 22129839

DOI: 10.1016/j.jcou.2020.01.005

Copy DOI

Process Chemistry and Technology

Waste Management and Disposal

Chemical Engineering (miscellaneous)

Abstract

Low charge separation efficiency is the critical limitation for solar-driven CO2 conversion into chemicals fuels. Accelerating charge transfer in the interface of photocatalysts is an intriguing approach to suppress charge recombination. Herein, Co2+ doped 0D/2D TiO2 quantum dots confined in graphitic carbon nitride (CoTiCN) heterostructure was prepared by in-situ pyrolysis of MOFs and urea. Co2+ serves as the bridge of linking 0D TiO2 and 2D g-C3N4 in the interface, and consequently accelerates charge transfer in the interface from 2D g-C3N4 to 0D TiO2. As a result, CO evolution rate for photocatalytic CO2 reduction reached 290 μmol g−1 h−1, much higher than those of pure g-C3N4 and TiO2/g-C3N4. In addition, photocatalytic mechanism study indicates that [Co(bpy)3]Cl2 in the system functions as cocatalyst without any photocatalytic activity under visible light irradiation. Electron transfer occurs from heterogeneous photocatalyst to [Co(bpy)3]Cl2, which acts as the electron transporter as active sites to catalyze CO2 reduction into CO. This work provides an insight into the design of metal doped 0D/2D material towards visible light driven CO2 reduction from the viewpoint of promoting charge transfer in the interface and the understanding of the photocatalytic mechanism of cocatalyst in system.

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Chemical Engineering Journal	Chemical Engineering Journal, 4, 7.55% Chemical Engineering Journal 4 publications, 7.55%
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Journal of Alloys and Compounds	Journal of Alloys and Compounds, 1, 1.89% Journal of Alloys and Compounds 1 publication, 1.89%
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ChemCatChem	ChemCatChem, 1, 1.89% ChemCatChem 1 publication, 1.89%
Carbon Energy	Carbon Energy, 1, 1.89% Carbon Energy 1 publication, 1.89%
ACS Sustainable Chemistry and Engineering	ACS Sustainable Chemistry and Engineering, 1, 1.89% ACS Sustainable Chemistry and Engineering 1 publication, 1.89%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 1, 1.89% Journal of Materials Chemistry A 1 publication, 1.89%
Catalysis Science and Technology	Catalysis Science and Technology, 1, 1.89% Catalysis Science and Technology 1 publication, 1.89%
Springer Series in Materials Science	Springer Series in Materials Science, 1, 1.89% Springer Series in Materials Science 1 publication, 1.89%
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Citations by publishers

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Elsevier	Elsevier, 27, 50.94% Elsevier 27 publications, 50.94%
American Chemical Society (ACS)	American Chemical Society (ACS), 8, 15.09% American Chemical Society (ACS) 8 publications, 15.09%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 6, 11.32% Royal Society of Chemistry (RSC) 6 publications, 11.32%
Springer Nature	Springer Nature, 4, 7.55% Springer Nature 4 publications, 7.55%
Wiley	Wiley, 4, 7.55% Wiley 4 publications, 7.55%
Hindawi Limited	Hindawi Limited, 1, 1.89% Hindawi Limited 1 publication, 1.89%
Institution of Chemical Engineers	Institution of Chemical Engineers, 1, 1.89% Institution of Chemical Engineers 1 publication, 1.89%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 1.89% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 1.89%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.89% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.89%
	5 10 15 20 25 30

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Shi H. et al. Solar-driven CO2 conversion over Co2+ doped 0D/2D TiO2/g-C3N4 heterostructure: Insights into the role of Co2+ and cocatalyst // Journal of CO2 Utilization. 2020. Vol. 38. pp. 16-23.

GOST all authors (up to 50) Copy

Shi H., Du J., Hou J., Ni W., Song C., Li K., Gurzadyan G. G., Gao L. Solar-driven CO2 conversion over Co2+ doped 0D/2D TiO2/g-C3N4 heterostructure: Insights into the role of Co2+ and cocatalyst // Journal of CO2 Utilization. 2020. Vol. 38. pp. 16-23.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.jcou.2020.01.005

UR - https://doi.org/10.1016/j.jcou.2020.01.005

TI - Solar-driven CO2 conversion over Co2+ doped 0D/2D TiO2/g-C3N4 heterostructure: Insights into the role of Co2+ and cocatalyst

T2 - Journal of CO2 Utilization

AU - Shi, Hainan

AU - Du, Jun

AU - Hou, Jungang

AU - Ni, Wenjun

AU - Song, Chunshan

AU - Li, Keyan

AU - Gurzadyan, Gagik G.

AU - Gao, Linna

PY - 2020

DA - 2020/05/01 00:00:00

PB - Elsevier

SP - 16-23

VL - 38

SN - 2212-9820

SN - 2212-9839

ER -

BibTex

Cite this

BibTex Copy

@article{2020_Shi,

author = {Hainan Shi and Jun Du and Jungang Hou and Wenjun Ni and Chunshan Song and Keyan Li and Gagik G. Gurzadyan and Linna Gao},

title = {Solar-driven CO2 conversion over Co2+ doped 0D/2D TiO2/g-C3N4 heterostructure: Insights into the role of Co2+ and cocatalyst},

journal = {Journal of CO2 Utilization},

year = {2020},

volume = {38},

publisher = {Elsevier},

month = {may},

url = {https://doi.org/10.1016/j.jcou.2020.01.005},

pages = {16--23},

doi = {10.1016/j.jcou.2020.01.005}

}

Found error?

Publisher

Elsevier

Journal

Journal of CO2 Utilization

Quartile SCImago

Quartile WOS

Impact factor

7.7

ISSN

22129820 (Print)
22129839 (Electronic)