Water soluble ruthenium cyclopentadienyl and aminocyclopentadienyl PTA complexes as catalysts for selective hydrogenation of α,β-unsaturated substrates (PTA=1,3,5-triaza-7-phosphaadamantane)
Sandra Bolaño
1
,
Luca Gonsalvi
1
,
Fabrizio Zanobini
1
,
Francesco Vizza
1
,
Valerio Bertolasi
2
,
Antonio Romerosa
3
,
Publication type: Journal Article
Publication date: 2004-12-16
SJR: —
CiteScore: —
Impact factor: —
ISSN: 13811169
Catalysis
Physical and Theoretical Chemistry
Process Chemistry and Technology
Abstract
A series of half-sandwich Ru-cyclopentadienyl derivatives containing the cage-like water soluble monodentate phosphine 1,3,5-triaza-7-phosphaadamantane (PTA) was synthesized and tested in aqueous phase or biphasic homogeneous hydrogenation of activated olefins via hydrogen transfer or under hydrogen pressure at mild conditions. The hydrogen transfer results show higher activity for the Cp* derivatives (Cp* = C5Me5) than for the corresponding Cp complexes (Cp = C5H5). Under H2 pressure, all complexes show high selectivity to C C double bond hydrogenation. The X-ray crystal structure featuring a protonated 2-aminoethylcyclopentadienyl Ru complex was also determined.
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70
Total citations:
70
Citations from 2024:
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(1.43%)
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Bolaño S. et al. Water soluble ruthenium cyclopentadienyl and aminocyclopentadienyl PTA complexes as catalysts for selective hydrogenation of α,β-unsaturated substrates (PTA=1,3,5-triaza-7-phosphaadamantane) // Journal of Molecular Catalysis A Chemical. 2004. Vol. 224. No. 1-2. pp. 61-70.
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Bolaño S., Gonsalvi L., Zanobini F., Vizza F., Bertolasi V., Romerosa A., Peruzzini M. Water soluble ruthenium cyclopentadienyl and aminocyclopentadienyl PTA complexes as catalysts for selective hydrogenation of α,β-unsaturated substrates (PTA=1,3,5-triaza-7-phosphaadamantane) // Journal of Molecular Catalysis A Chemical. 2004. Vol. 224. No. 1-2. pp. 61-70.
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TY - JOUR
DO - 10.1016/j.molcata.2004.06.030
UR - https://doi.org/10.1016/j.molcata.2004.06.030
TI - Water soluble ruthenium cyclopentadienyl and aminocyclopentadienyl PTA complexes as catalysts for selective hydrogenation of α,β-unsaturated substrates (PTA=1,3,5-triaza-7-phosphaadamantane)
T2 - Journal of Molecular Catalysis A Chemical
AU - Bolaño, Sandra
AU - Gonsalvi, Luca
AU - Zanobini, Fabrizio
AU - Vizza, Francesco
AU - Bertolasi, Valerio
AU - Romerosa, Antonio
AU - Peruzzini, Maurizio
PY - 2004
DA - 2004/12/16
PB - Elsevier
SP - 61-70
IS - 1-2
VL - 224
SN - 1381-1169
ER -
Cite this
BibTex (up to 50 authors)
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@article{2004_Bolaño,
author = {Sandra Bolaño and Luca Gonsalvi and Fabrizio Zanobini and Francesco Vizza and Valerio Bertolasi and Antonio Romerosa and Maurizio Peruzzini},
title = {Water soluble ruthenium cyclopentadienyl and aminocyclopentadienyl PTA complexes as catalysts for selective hydrogenation of α,β-unsaturated substrates (PTA=1,3,5-triaza-7-phosphaadamantane)},
journal = {Journal of Molecular Catalysis A Chemical},
year = {2004},
volume = {224},
publisher = {Elsevier},
month = {dec},
url = {https://doi.org/10.1016/j.molcata.2004.06.030},
number = {1-2},
pages = {61--70},
doi = {10.1016/j.molcata.2004.06.030}
}
Cite this
MLA
Copy
Bolaño, Sandra, et al. “Water soluble ruthenium cyclopentadienyl and aminocyclopentadienyl PTA complexes as catalysts for selective hydrogenation of α,β-unsaturated substrates (PTA=1,3,5-triaza-7-phosphaadamantane).” Journal of Molecular Catalysis A Chemical, vol. 224, no. 1-2, Dec. 2004, pp. 61-70. https://doi.org/10.1016/j.molcata.2004.06.030.
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