Separation and Purification Technology, volume 268, pages 118691

In situ fabrication of a novel S-scheme heterojunction photocatalyts Bi2O3/P-C3N4 to enhance levofloxacin removal from water

Xinfei Zhang ¹

Yuan Zhang ²

Xiaobo Jia ³

Nan Zhang ¹

Rui Xia ³

Xiaojiao Zhang ³

Ziwei Wang ³

Mingqiao Yu ³

Hide authors affiliations Show authors affiliations: 3 affiliations

College of Water Sciences, Beijing Normal University, Beijing 100875, China. |

Guangdong Provincial Key Laboratory of Water Quality Improvement and Ecological Restoration for Watersheds, Institute of Environmental and Ecological Engineering, Guangdong University of Technology, Guangzhou, 510006, China. |

State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China |

Publication type: Journal Article

Publication date: 2021-08-01

Elsevier

Journal: Separation and Purification Technology

Quartile SCImago

Quartile WOS

Impact factor: 8.6

ISSN: 13835866, 18733794

DOI: 10.1016/j.seppur.2021.118691

Copy DOI

Analytical Chemistry

Filtration and Separation

Abstract

• A novel S-scheme heterojunction Bi 2 O 3 /P-C 3 N 4 material. • Removal of 89.2% of the levofloxacin in water within 75 min under simulated sunlight. • The improvement of the Bi 2 O 3 /P-C 3 N 4 photocatalytic effect mechanism was proved. • Possible intermediate products and pathways for levofloxacin degradation were proposed. The removal of antibiotics from water by S-scheme heterojunction photocatalytic materials has become a research hotspot in recent years. Herein, an S -scheme heterojunction Bi 2 O 3 /P-C 3 N 4 composite photocatalytic material was prepared via in situ thermal polymerization and the degradation effect and internal mechanism of levofloxacin (LVFX) were explored under simulated sunlight. The results show that the Bi 2 O 3 /P-C 3 N 4 composite photocatalytic material can remove 89.2% of the LVFX in water within 75 min under simulated sunlight, which is greatly improved compared to the original Bi 2 O 3 and P-C 3 N 4 . The degradation effect is improved because the constructed S-scheme system helps spatially separate the electrons with higher reducing abilities generated by P-C 3 N 4 and the holes with higher oxidizing ability generated by Bi 2 O 3 ; moreover, BET specific surface area and the hydrophilicity is improved. Further through radicals capture, electron spin resonance (ESR), the density functional theory (DFT) experiments verified the mechanism of S-scheme heterojunction degradation of LVFX and revealed that holes and superoxide free radicals are the main active substances in the degradation of LVFX. Finally, liquid chromatography–tandem mass spectrometry (LC–MS) was used to determine the intermediate products in the degradation path, and the LVFX degradation pathway was proposed. This study provides a new insight into the degradation of LVFX and provides support for antibiotic removal of photocatalytic materials in real water environments.

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RSC Advances	RSC Advances, 2, 3.13% RSC Advances 2 publications, 3.13%
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Citations by publishers

	5 10 15 20 25 30 35 40 45
Elsevier	Elsevier, 44, 68.75% Elsevier 44 publications, 68.75%
Springer Nature	Springer Nature, 9, 14.06% Springer Nature 9 publications, 14.06%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 4.69% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 4.69%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 3, 4.69% Royal Society of Chemistry (RSC) 3 publications, 4.69%
Wiley	Wiley, 2, 3.13% Wiley 2 publications, 3.13%
IGI Global	IGI Global, 1, 1.56% IGI Global 1 publication, 1.56%
CSIRO Publishing	CSIRO Publishing, 1, 1.56% CSIRO Publishing 1 publication, 1.56%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.56% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.56%
	5 10 15 20 25 30 35 40 45

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Zhang X. et al. In situ fabrication of a novel S-scheme heterojunction photocatalyts Bi2O3/P-C3N4 to enhance levofloxacin removal from water // Separation and Purification Technology. 2021. Vol. 268. p. 118691.

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Zhang X., Zhang Y., Jia X., Zhang N., Xia R., Zhang X., Wang Z., Yu M. In situ fabrication of a novel S-scheme heterojunction photocatalyts Bi2O3/P-C3N4 to enhance levofloxacin removal from water // Separation and Purification Technology. 2021. Vol. 268. p. 118691.

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RIS Copy

TY - JOUR

DO - 10.1016/j.seppur.2021.118691

UR - https://doi.org/10.1016/j.seppur.2021.118691

TI - In situ fabrication of a novel S-scheme heterojunction photocatalyts Bi2O3/P-C3N4 to enhance levofloxacin removal from water

T2 - Separation and Purification Technology

AU - Zhang, Xinfei

AU - Zhang, Yuan

AU - Jia, Xiaobo

AU - Zhang, Nan

AU - Xia, Rui

AU - Zhang, Xiaojiao

AU - Wang, Ziwei

AU - Yu, Mingqiao

PY - 2021

DA - 2021/08/01 00:00:00

PB - Elsevier

SP - 118691

VL - 268

SN - 1383-5866

SN - 1873-3794

ER -

BibTex

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BibTex Copy

@article{2021_Zhang,

author = {Xinfei Zhang and Yuan Zhang and Xiaobo Jia and Nan Zhang and Rui Xia and Xiaojiao Zhang and Ziwei Wang and Mingqiao Yu},

title = {In situ fabrication of a novel S-scheme heterojunction photocatalyts Bi2O3/P-C3N4 to enhance levofloxacin removal from water},

journal = {Separation and Purification Technology},

year = {2021},

volume = {268},

publisher = {Elsevier},

month = {aug},

url = {https://doi.org/10.1016/j.seppur.2021.118691},

pages = {118691},

doi = {10.1016/j.seppur.2021.118691}

}

Found error?

Publisher

Elsevier

Journal

Separation and Purification Technology

Quartile SCImago

Quartile WOS

Impact factor

8.6

ISSN

13835866 (Print)
18733794 (Electronic)