Electrochimica Acta, volume 48, issue 2, pages 197-204
The inclusion of Mo, Nb and Ta in Pt and PtRu carbon supported electrocatalysts in the quest for improved CO tolerant PEMFC anodes
1
ECN Clean Fossil Fuels, P.O. Box 1, 1755 ZG, Petten, The Netherlands
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Publication type: Journal Article
Publication date: 2002-11-11
General Chemical Engineering
Electrochemistry
Abstract
The effect of the inclusion of Mo, Nb and Ta in Pt and PtRu carbon supported anode electrocatalysts on CO tolerance in proton exchange membrane fuel cells (PEMFC) has been investigated by cyclic voltammetry and fuel cell tests. CO stripping voltammetry on binary PtxM/C (M: Mo, Nb, Ta) reveals partial oxidation of the CO adlayer at low potential, with PtMo (4:1)/C exhibiting the lowest value. At 80 °C, the operating temperature of the fuel cell, CO oxidation was observed at potentials close to 0 V versus the reversible hydrogen electrode (RHE). No significant difference for CO electro-oxidation at the lower potential limit, compared to PtRu/C, was observed for PtRuMy/C (M: Mo, Nb). Fuel cell tests demonstrated that while all the prepared catalysts exhibited enhanced performance compared to Pt/C, only the addition of a relatively small amount of Mo to PtRu results in an electrocatalyst with a higher activity, in the presence of carbon monoxide, to PtRu/C, the current catalyst of choice for PEM fuel cell applications.
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Papageorgopoulos D. C., Keijzer M., de Bruijn F. A. The inclusion of Mo, Nb and Ta in Pt and PtRu carbon supported electrocatalysts in the quest for improved CO tolerant PEMFC anodes // Electrochimica Acta. 2002. Vol. 48. No. 2. pp. 197-204.
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Papageorgopoulos D. C., Keijzer M., de Bruijn F. A. The inclusion of Mo, Nb and Ta in Pt and PtRu carbon supported electrocatalysts in the quest for improved CO tolerant PEMFC anodes // Electrochimica Acta. 2002. Vol. 48. No. 2. pp. 197-204.
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TY - JOUR
DO - 10.1016/S0013-4686(02)00602-3
UR - https://doi.org/10.1016/S0013-4686(02)00602-3
TI - The inclusion of Mo, Nb and Ta in Pt and PtRu carbon supported electrocatalysts in the quest for improved CO tolerant PEMFC anodes
T2 - Electrochimica Acta
AU - Papageorgopoulos, D. C.
AU - Keijzer, M.
AU - de Bruijn, F. A.
PY - 2002
DA - 2002/11/11 00:00:00
PB - Elsevier
SP - 197-204
IS - 2
VL - 48
SN - 0013-4686
ER -
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@article{2002_Papageorgopoulos,
author = {D. C. Papageorgopoulos and M. Keijzer and F. A. de Bruijn},
title = {The inclusion of Mo, Nb and Ta in Pt and PtRu carbon supported electrocatalysts in the quest for improved CO tolerant PEMFC anodes},
journal = {Electrochimica Acta},
year = {2002},
volume = {48},
publisher = {Elsevier},
month = {nov},
url = {https://doi.org/10.1016/S0013-4686(02)00602-3},
number = {2},
pages = {197--204},
doi = {10.1016/S0013-4686(02)00602-3}
}
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Papageorgopoulos, D. C., et al. “The inclusion of Mo, Nb and Ta in Pt and PtRu carbon supported electrocatalysts in the quest for improved CO tolerant PEMFC anodes.” Electrochimica Acta, vol. 48, no. 2, Nov. 2002, pp. 197-204. https://doi.org/10.1016/S0013-4686(02)00602-3.