Solid State Ionics, volume 131, issue 1-2, pages 13-22
Point-defect thermodynamics and size effects
Publication type: Journal Article
Publication date: 2000-06-01
General Chemistry
Condensed Matter Physics
General Materials Science
Abstract
The introductory part reviews some basic aspects of bulk point-defect thermodynamics. It makes use of the fact that for the purposes under consideration, the real structure can be decomposed in a perfect ground structure and a superimposed defect structure. Then modifications of the point-defect concentration and distribution are considered occurring if interfaces are approached. A simple treatment is possible for the abrupt core-space charge situation in which the standard chemical potentials are assumed to change in a step-like way. Evidence is given that in very many cases this is a reasonable model. There, the adjustment at interfaces occurs solely via space charge regions. ‘Trivial’ size effects are brought about by the changed surface (i.e. core plus space charge layer) to volume ratio. A mesoscale size effect is expected if the width of the space charge layers is no longer small compared with the distance of neighbouring interfaces (Debye-length λ as scaling parameter). In some situations, e.g. if extremely small clusters are treated, distinct deviations in the ground structure also occur, affecting energetic and entropic standard terms. Since such modifications usually decay steeply with increasing interfacial distance ( L ), another scaling parameter (l) defines a further mesoscopic regime. As examples, micro- and nano-sized particles, films, polycrystals and composites are discussed.
Top-30
Citations by journals
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1 publication, 1.41%
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1 publication, 1.41%
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Electrochemical and Solid-State Letters
1 publication, 1.41%
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Nature
1 publication, 1.41%
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Nanoscale Research Letters
1 publication, 1.41%
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European Physical Journal B
1 publication, 1.41%
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MRS Proceedings
1 publication, 1.41%
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1 publication, 1.41%
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1 publication, 1.41%
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1 publication, 1.41%
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1 publication, 1.41%
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1 publication, 1.41%
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Citations by publishers
2
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16
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Elsevier
16 publications, 22.54%
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Springer Nature
10 publications, 14.08%
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Wiley
7 publications, 9.86%
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American Chemical Society (ACS)
5 publications, 7.04%
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American Institute of Physics (AIP)
4 publications, 5.63%
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Royal Society of Chemistry (RSC)
4 publications, 5.63%
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Pleiades Publishing
3 publications, 4.23%
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IOP Publishing
3 publications, 4.23%
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Taylor & Francis
2 publications, 2.82%
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American Physical Society (APS)
1 publication, 1.41%
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EDP Sciences
1 publication, 1.41%
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The Electrochemical Society
1 publication, 1.41%
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Materials Research Society
1 publication, 1.41%
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Cambridge University Press
1 publication, 1.41%
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Materials Research Society of Korea
1 publication, 1.41%
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American Association for the Advancement of Science (AAAS)
1 publication, 1.41%
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Trans Tech Publications
1 publication, 1.41%
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Annual Reviews
1 publication, 1.41%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 1.41%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 1.41%
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2
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16
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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TY - JOUR
DO - 10.1016/S0167-2738(00)00618-4
UR - https://doi.org/10.1016/S0167-2738(00)00618-4
TI - Point-defect thermodynamics and size effects
T2 - Solid State Ionics
AU - Maier, Joachim
PY - 2000
DA - 2000/06/01 00:00:00
PB - Elsevier
SP - 13-22
IS - 1-2
VL - 131
SN - 0167-2738
ER -
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@article{2000_Maier,
author = {Joachim Maier},
title = {Point-defect thermodynamics and size effects},
journal = {Solid State Ionics},
year = {2000},
volume = {131},
publisher = {Elsevier},
month = {jun},
url = {https://doi.org/10.1016/S0167-2738(00)00618-4},
number = {1-2},
pages = {13--22},
doi = {10.1016/S0167-2738(00)00618-4}
}
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Maier, Joachim. “Point-defect thermodynamics and size effects.” Solid State Ionics, vol. 131, no. 1-2, Jun. 2000, pp. 13-22. https://doi.org/10.1016/S0167-2738(00)00618-4.