Solid State Ionics, volume 131, issue 1-2, pages 13-22

Point-defect thermodynamics and size effects

Joachim Maier ¹

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Max‐Planck‐Institut für Festkörperforschung Heisenbergstraße 1 70569 Stuttgart Germany |

Publication type: Journal Article

Publication date: 2000-06-01

Elsevier

Journal: Solid State Ionics

Quartile SCImago

Quartile WOS

Impact factor: 3.2

ISSN: 01672738

DOI: 10.1016/S0167-2738(00)00618-4

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General Chemistry

Condensed Matter Physics

General Materials Science

Abstract

The introductory part reviews some basic aspects of bulk point-defect thermodynamics. It makes use of the fact that for the purposes under consideration, the real structure can be decomposed in a perfect ground structure and a superimposed defect structure. Then modifications of the point-defect concentration and distribution are considered occurring if interfaces are approached. A simple treatment is possible for the abrupt core-space charge situation in which the standard chemical potentials are assumed to change in a step-like way. Evidence is given that in very many cases this is a reasonable model. There, the adjustment at interfaces occurs solely via space charge regions. ‘Trivial’ size effects are brought about by the changed surface (i.e. core plus space charge layer) to volume ratio. A mesoscale size effect is expected if the width of the space charge layers is no longer small compared with the distance of neighbouring interfaces (Debye-length λ as scaling parameter). In some situations, e.g. if extremely small clusters are treated, distinct deviations in the ground structure also occur, affecting energetic and entropic standard terms. Since such modifications usually decay steeply with increasing interfacial distance ( L ), another scaling parameter (l) defines a further mesoscopic regime. As examples, micro- and nano-sized particles, films, polycrystals and composites are discussed.

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Citations by journals

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Journal of the European Ceramic Society	Journal of the European Ceramic Society, 3, 4.23% Journal of the European Ceramic Society 3 publications, 4.23%
Ionics	Ionics, 3, 4.23% Ionics 3 publications, 4.23%
Journal of Physics Condensed Matter	Journal of Physics Condensed Matter, 3, 4.23% Journal of Physics Condensed Matter 3 publications, 4.23%
Solid State Ionics	Solid State Ionics, 3, 4.23% Solid State Ionics 3 publications, 4.23%
Journal of the American Ceramic Society	Journal of the American Ceramic Society, 3, 4.23% Journal of the American Ceramic Society 3 publications, 4.23%
Nature Materials	Nature Materials, 2, 2.82% Nature Materials 2 publications, 2.82%
Acta Materialia	Acta Materialia, 2, 2.82% Acta Materialia 2 publications, 2.82%
Advanced Materials	Advanced Materials, 2, 2.82% Advanced Materials 2 publications, 2.82%
ACS applied materials & interfaces	ACS applied materials & interfaces, 2, 2.82% ACS applied materials & interfaces 2 publications, 2.82%
Russian Journal of General Chemistry	Russian Journal of General Chemistry, 1, 1.41% Russian Journal of General Chemistry 1 publication, 1.41%
Nanotechnologies in Russia	Nanotechnologies in Russia, 1, 1.41% Nanotechnologies in Russia 1 publication, 1.41%
Journal of Applied Physics	Journal of Applied Physics, 1, 1.41% Journal of Applied Physics 1 publication, 1.41%
Journal of Chemical Physics	Journal of Chemical Physics, 1, 1.41% Journal of Chemical Physics 1 publication, 1.41%
Applied Physics Reviews	Applied Physics Reviews, 1, 1.41% Applied Physics Reviews 1 publication, 1.41%
Physical Review B	Physical Review B, 1, 1.41% Physical Review B 1 publication, 1.41%
EPJ Applied Physics	EPJ Applied Physics, 1, 1.41% EPJ Applied Physics 1 publication, 1.41%
Current Opinion in Solid State and Materials Science	Current Opinion in Solid State and Materials Science, 1, 1.41% Current Opinion in Solid State and Materials Science 1 publication, 1.41%
Electrochemical and Solid-State Letters	Electrochemical and Solid-State Letters, 1, 1.41% Electrochemical and Solid-State Letters 1 publication, 1.41%
Nature	Nature, 1, 1.41% Nature 1 publication, 1.41%
Nanoscale Research Letters	Nanoscale Research Letters, 1, 1.41% Nanoscale Research Letters 1 publication, 1.41%
European Physical Journal B	European Physical Journal B, 1, 1.41% European Physical Journal B 1 publication, 1.41%
MRS Proceedings	MRS Proceedings, 1, 1.41% MRS Proceedings 1 publication, 1.41%
Journal of Materials Research	Journal of Materials Research, 1, 1.41% Journal of Materials Research 1 publication, 1.41%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 1, 1.41% Journal of Alloys and Compounds 1 publication, 1.41%
Materials Science & Engineering A: Structural Materials: Properties, Microstructure and Processing	Materials Science & Engineering A: Structural Materials: Properties, Microstructure and Processing, 1, 1.41% Materials Science & Engineering A: Structural Materials: Properties, Microstructure and Processing 1 publication, 1.41%
Nano Energy	Nano Energy, 1, 1.41% Nano Energy 1 publication, 1.41%
Materials Research Bulletin	Materials Research Bulletin, 1, 1.41% Materials Research Bulletin 1 publication, 1.41%
Journal of Power Sources	Journal of Power Sources, 1, 1.41% Journal of Power Sources 1 publication, 1.41%
Scripta Materialia	Scripta Materialia, 1, 1.41% Scripta Materialia 1 publication, 1.41%
	1 2 3

Citations by publishers

	2 4 6 8 10 12 14 16
Elsevier	Elsevier, 16, 22.54% Elsevier 16 publications, 22.54%
Springer Nature	Springer Nature, 10, 14.08% Springer Nature 10 publications, 14.08%
Wiley	Wiley, 7, 9.86% Wiley 7 publications, 9.86%
American Chemical Society (ACS)	American Chemical Society (ACS), 5, 7.04% American Chemical Society (ACS) 5 publications, 7.04%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 4, 5.63% American Institute of Physics (AIP) 4 publications, 5.63%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 4, 5.63% Royal Society of Chemistry (RSC) 4 publications, 5.63%
Pleiades Publishing	Pleiades Publishing, 3, 4.23% Pleiades Publishing 3 publications, 4.23%
IOP Publishing	IOP Publishing, 3, 4.23% IOP Publishing 3 publications, 4.23%
Taylor & Francis	Taylor & Francis, 2, 2.82% Taylor & Francis 2 publications, 2.82%
American Physical Society (APS)	American Physical Society (APS), 1, 1.41% American Physical Society (APS) 1 publication, 1.41%
EDP Sciences	EDP Sciences, 1, 1.41% EDP Sciences 1 publication, 1.41%
The Electrochemical Society	The Electrochemical Society, 1, 1.41% The Electrochemical Society 1 publication, 1.41%
Materials Research Society	Materials Research Society, 1, 1.41% Materials Research Society 1 publication, 1.41%
Cambridge University Press	Cambridge University Press, 1, 1.41% Cambridge University Press 1 publication, 1.41%
Materials Research Society of Korea	Materials Research Society of Korea, 1, 1.41% Materials Research Society of Korea 1 publication, 1.41%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 1.41% American Association for the Advancement of Science (AAAS) 1 publication, 1.41%
Trans Tech Publications	Trans Tech Publications, 1, 1.41% Trans Tech Publications 1 publication, 1.41%
Annual Reviews	Annual Reviews, 1, 1.41% Annual Reviews 1 publication, 1.41%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 1.41% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 1.41%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.41% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.41%
	2 4 6 8 10 12 14 16

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Maier J. Point-defect thermodynamics and size effects // Solid State Ionics. 2000. Vol. 131. No. 1-2. pp. 13-22.

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Maier J. Point-defect thermodynamics and size effects // Solid State Ionics. 2000. Vol. 131. No. 1-2. pp. 13-22.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/S0167-2738(00)00618-4

UR - https://doi.org/10.1016/S0167-2738(00)00618-4

TI - Point-defect thermodynamics and size effects

T2 - Solid State Ionics

AU - Maier, Joachim

PY - 2000

DA - 2000/06/01 00:00:00

PB - Elsevier

SP - 13-22

IS - 1-2

VL - 131

SN - 0167-2738

ER -

BibTex |

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BibTex Copy

@article{2000_Maier,

author = {Joachim Maier},

title = {Point-defect thermodynamics and size effects},

journal = {Solid State Ionics},

year = {2000},

volume = {131},

publisher = {Elsevier},

month = {jun},

url = {https://doi.org/10.1016/S0167-2738(00)00618-4},

number = {1-2},

pages = {13--22},

doi = {10.1016/S0167-2738(00)00618-4}

}

MLA

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MLA Copy

Maier, Joachim. “Point-defect thermodynamics and size effects.” Solid State Ionics, vol. 131, no. 1-2, Jun. 2000, pp. 13-22. https://doi.org/10.1016/S0167-2738(00)00618-4.

Found error?

Publisher

Elsevier

Journal

Solid State Ionics

Quartile SCImago

Quartile WOS

Impact factor

3.2

ISSN

01672738 (Print)