Dehydrogenation of ethane with carbon dioxide over supported chromium oxide catalysts
1
Department of Surface Chemistry, National Institute of Materials and Chemical Research, Tsukuba, Ibaraki 305-8565, Japan
|
Publication type: Journal Article
Publication date: 2000-03-01
scimago Q2
wos Q2
SJR: 1.000
CiteScore: 8.6
Impact factor: 4.8
ISSN: 0926860X, 18733875
Catalysis
Process Chemistry and Technology
Abstract
The oxidative dehydrogenation of ethane into ethylene by carbon dioxide over an unsupported Cr 2 O 3 and several supported Cr 2 O 3 catalysts on metal oxides such as Al 2 O 3 , SiO 2 , TiO 2 , and ZrO 2 was investigated and the effect of support on the catalytic activity was studied. The unsupported Cr 2 O 3 shows medium catalytic activity in this reaction; the support will exert a quite different effect on catalytic behavior. The catalytic activity varies with the nature of supports. Cr 2 O 3 /SiO 2 catalysts exhibit an excellent performance in this reaction. Cr 2 O 3 loading also affects the catalytic activity; 8 wt.% Cr 2 O 3 /SiO 2 catalysts can produce 55.5% ethylene yield at 61% ethane conversion at 650°C. Characterization indicates that the distribution of chromium oxide on supports and surface chromium species structure are influenced by the nature of supports. The acidity/basicity and redox property of catalysts determines the catalytic activity in the dehydrogenation of ethane by carbon dioxide.
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Total citations:
186
Citations from 2025:
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(5.92%)
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GOST
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Wang S. et al. Dehydrogenation of ethane with carbon dioxide over supported chromium oxide catalysts // Applied Catalysis A: General. 2000. Vol. 196. No. 1. pp. 1-8.
GOST all authors (up to 50)
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Wang S., Murata K., Hayakawa T., Hamakawa S., Suzuki K. Dehydrogenation of ethane with carbon dioxide over supported chromium oxide catalysts // Applied Catalysis A: General. 2000. Vol. 196. No. 1. pp. 1-8.
Cite this
RIS
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TY - JOUR
DO - 10.1016/S0926-860X(99)00450-0
UR - https://doi.org/10.1016/S0926-860X(99)00450-0
TI - Dehydrogenation of ethane with carbon dioxide over supported chromium oxide catalysts
T2 - Applied Catalysis A: General
AU - Wang, Shuaijun
AU - Murata, K.
AU - Hayakawa, T.
AU - Hamakawa, Satoshi
AU - Suzuki, K.
PY - 2000
DA - 2000/03/01
PB - Elsevier
SP - 1-8
IS - 1
VL - 196
SN - 0926-860X
SN - 1873-3875
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2000_Wang,
author = {Shuaijun Wang and K. Murata and T. Hayakawa and Satoshi Hamakawa and K. Suzuki},
title = {Dehydrogenation of ethane with carbon dioxide over supported chromium oxide catalysts},
journal = {Applied Catalysis A: General},
year = {2000},
volume = {196},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/S0926-860X(99)00450-0},
number = {1},
pages = {1--8},
doi = {10.1016/S0926-860X(99)00450-0}
}
Cite this
MLA
Copy
Wang, Shuaijun, et al. “Dehydrogenation of ethane with carbon dioxide over supported chromium oxide catalysts.” Applied Catalysis A: General, vol. 196, no. 1, Mar. 2000, pp. 1-8. https://doi.org/10.1016/S0926-860X(99)00450-0.