A correlation between structural changes in a Ni-Cu catalyst during decomposition of ethylene/ammonia mixture and properties of nitrogen-doped carbon nanofibers
Тип публикации: Journal Article
Дата публикации: 2013-03-01
scimago Q1
wos Q1
БС1
SJR: 3.394
CiteScore: 27.1
Impact factor: 14.9
ISSN: 20954956, 2096885X
Electrochemistry
Energy Engineering and Power Technology
Fuel Technology
Energy (miscellaneous)
Краткое описание
Changes of a 65Ni25Cu10Al 2 O 3 catalyst consisting of Ni-enriched and Cu-enriched alloys were investigated in the bulk and on the surface during the growth of nitrogen-doped carbon nanofibers (N-CNFs) by decomposition of a 50%C 2 H 4 /50%NH 3 mixture using in situ X-ray diffraction (XRD) analysis, ex situ X-ray photoelectron spectroscopy (XPS) and transmission electron microscopy (TEM) techniques. It was shown that N-CNF growth at 450–650 °C is accompanied by dissolution of carbon and nitrogen in the Ni-enriched alloy, whereas Cu-enriched alloy remains inactive. A correlation between nickel and copper surface concentrations and properties of N-CNFs in relation to the nitrogen content was found. It was demonstrated that phase composition of the catalyst during N-CNF growth determines the type of N-CNFs structure.
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Pod”yacheva O. Yu. et al. A correlation between structural changes in a Ni-Cu catalyst during decomposition of ethylene/ammonia mixture and properties of nitrogen-doped carbon nanofibers // Journal of Energy Chemistry. 2013. Vol. 22. No. 2. pp. 270-278.
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Pod”yacheva O. Yu., Shmakov A. N., Koscheev S., Boronin A., Kibis L., Prosvirin I. P., Ismagilov Z. R. A correlation between structural changes in a Ni-Cu catalyst during decomposition of ethylene/ammonia mixture and properties of nitrogen-doped carbon nanofibers // Journal of Energy Chemistry. 2013. Vol. 22. No. 2. pp. 270-278.
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TY - JOUR
DO - 10.1016/S2095-4956(13)60033-9
UR - https://doi.org/10.1016/S2095-4956(13)60033-9
TI - A correlation between structural changes in a Ni-Cu catalyst during decomposition of ethylene/ammonia mixture and properties of nitrogen-doped carbon nanofibers
T2 - Journal of Energy Chemistry
AU - Pod”yacheva, O Yu
AU - Shmakov, A N
AU - Koscheev, S.V.
AU - Boronin, Andrei
AU - Kibis, Lidiya
AU - Prosvirin, Igor P.
AU - Ismagilov, Z. R.
PY - 2013
DA - 2013/03/01
PB - Elsevier
SP - 270-278
IS - 2
VL - 22
SN - 2095-4956
SN - 2096-885X
ER -
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@article{2013_Pod”yacheva,
author = {O Yu Pod”yacheva and A N Shmakov and S.V. Koscheev and Andrei Boronin and Lidiya Kibis and Igor P. Prosvirin and Z. R. Ismagilov},
title = {A correlation between structural changes in a Ni-Cu catalyst during decomposition of ethylene/ammonia mixture and properties of nitrogen-doped carbon nanofibers},
journal = {Journal of Energy Chemistry},
year = {2013},
volume = {22},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/S2095-4956(13)60033-9},
number = {2},
pages = {270--278},
doi = {10.1016/S2095-4956(13)60033-9}
}
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MLA
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Pod”yacheva, O. Yu., et al. “A correlation between structural changes in a Ni-Cu catalyst during decomposition of ethylene/ammonia mixture and properties of nitrogen-doped carbon nanofibers.” Journal of Energy Chemistry, vol. 22, no. 2, Mar. 2013, pp. 270-278. https://doi.org/10.1016/S2095-4956(13)60033-9.
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