Applied Catalysis A: General

, том 302 , издание 1 , страницы 32-41

The role of Fe addition on the activity of Pd-containing catalysts in multiphase hydrodechlorination

Тип публикации: Journal Article

Дата публикации: 2006-03-01

Elsevier

Applied Catalysis A: General

scimago Q2

wos Q2

БС1

SJR: 1

CiteScore: 8.6

Impact factor: 4.8

ISSN: 0926860X, 18733875

DOI: 10.1016/j.apcata.2005.12.020

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Catalysis

Process Chemistry and Technology

Краткое описание

Multiphase hydrodechlorination of 1,4-dichlorobenzene, hexachlorobenzene and 2,4,8-trichlorodibenzofurane was studied in the presence of Pd/C and Pd-Fe/C catalysts. The effect of the addition of a second metal to Pd/C was investigated. The content (1–12 wt.%) and ratio of metals were varied to determine their influence on catalytic activity, which was demonstrated to strongly depend on metal ratio in multiphase hydrodechlorination systems. Metal–metal interaction and structure of bimetallic particles were studied by magnetic measurements and TPR analysis. Bimetallic particles consisted of Pd-enriched PdFe alloy. Also Fe 2 O 3 was presented on the surface of catalyst. Based on catalytic performance, magnetic measurements, and TPR, two aspects of the influence of iron addition were considered: (1) formation of Pd-enriched PdFe alloy, which resulted in an increase of catalytic activity of bimetallic catalysts in comparison with Pd/C; (2) formation of FeCl 3 under HDC reaction condition, which prevented complete chlorination of palladium, possibly leading to its deactivation.

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Golubina E. V. et al. The role of Fe addition on the activity of Pd-containing catalysts in multiphase hydrodechlorination // Applied Catalysis A: General. 2006. Vol. 302. No. 1. pp. 32-41.

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Golubina E. V., Lokteva E. S., Lunin V. V., Telegina N. S., Stakheev A., Tundo P. The role of Fe addition on the activity of Pd-containing catalysts in multiphase hydrodechlorination // Applied Catalysis A: General. 2006. Vol. 302. No. 1. pp. 32-41.

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TY - JOUR

DO - 10.1016/j.apcata.2005.12.020

UR - https://doi.org/10.1016/j.apcata.2005.12.020

TI - The role of Fe addition on the activity of Pd-containing catalysts in multiphase hydrodechlorination

T2 - Applied Catalysis A: General

AU - Golubina, Elena V

AU - Lokteva, Ekaterina S

AU - Lunin, V. V.

AU - Telegina, N S

AU - Stakheev, A.Yu

AU - Tundo, Pietro

PY - 2006

DA - 2006/03/01

PB - Elsevier

SP - 32-41

IS - 1

VL - 302

SN - 0926-860X

SN - 1873-3875

ER -

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@article{2006_Golubina,

author = {Elena V Golubina and Ekaterina S Lokteva and V. V. Lunin and N S Telegina and A.Yu Stakheev and Pietro Tundo},

title = {The role of Fe addition on the activity of Pd-containing catalysts in multiphase hydrodechlorination},

journal = {Applied Catalysis A: General},

year = {2006},

volume = {302},

publisher = {Elsevier},

month = {mar},

url = {https://doi.org/10.1016/j.apcata.2005.12.020},

number = {1},

pages = {32--41},

doi = {10.1016/j.apcata.2005.12.020}

}

MLA

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MLA Скопировать

Golubina, Elena V., et al. “The role of Fe addition on the activity of Pd-containing catalysts in multiphase hydrodechlorination.” Applied Catalysis A: General, vol. 302, no. 1, Mar. 2006, pp. 32-41. https://doi.org/10.1016/j.apcata.2005.12.020.

Издатель

Elsevier

Журнал

Applied Catalysis A: General

scimago Q2

wos Q2

БС1

SJR

CiteScore

8.6

Impact factor

4.8

ISSN

0926860X (Print)

18733875 (Electronic)