Palladium nanoparticle decorated high nitrogen-doped graphene with high catalytic activity for Suzuki–Miyaura and Ullmann-type coupling reactions in aqueous media
Тип публикации: Journal Article
Дата публикации: 2014-11-01
scimago Q2
wos Q2
БС1
SJR: 1.000
CiteScore: 8.6
Impact factor: 4.8
ISSN: 0926860X, 18733875
Catalysis
Process Chemistry and Technology
Краткое описание
Palladium nanoparticle are decorated over a highly nitrogen-doped graphene (Pd NPs-HNG) in a facile manner by reducing palladium chloride in the presence of ethylene glycol as reducing, stabilizing, and dispersing agent. The obtained catalyst can act as an efficient catalyst for the Suzuki–Miyaura and Ullmann-type coupling reactions of a broad spectrum of aryl halides in aqueous media. The remarkable reactivity of the Pd NPs-HNG nanocomposite toward Suzuki–Miyaura and Ullmann-type coupling reactions is attributed to the high degree of nitrogen loading in graphene sheets. The N-doped graphene as polycyclic heteroaromatic molecule acts as both the catalyst support and the electron source (reducing agent) for Ullmann homocoupling. The catalyst could be recovered and reused several times without a significant loss of activity.
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Movahed S. K., Dabiri M., Bazgir A. Palladium nanoparticle decorated high nitrogen-doped graphene with high catalytic activity for Suzuki–Miyaura and Ullmann-type coupling reactions in aqueous media // Applied Catalysis A: General. 2014. Vol. 488. pp. 265-274.
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Movahed S. K., Dabiri M., Bazgir A. Palladium nanoparticle decorated high nitrogen-doped graphene with high catalytic activity for Suzuki–Miyaura and Ullmann-type coupling reactions in aqueous media // Applied Catalysis A: General. 2014. Vol. 488. pp. 265-274.
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TY - JOUR
DO - 10.1016/j.apcata.2014.09.045
UR - https://doi.org/10.1016/j.apcata.2014.09.045
TI - Palladium nanoparticle decorated high nitrogen-doped graphene with high catalytic activity for Suzuki–Miyaura and Ullmann-type coupling reactions in aqueous media
T2 - Applied Catalysis A: General
AU - Movahed, Siyavash Kazemi
AU - Dabiri, Minoo
AU - Bazgir, Ayoob
PY - 2014
DA - 2014/11/01
PB - Elsevier
SP - 265-274
VL - 488
SN - 0926-860X
SN - 1873-3875
ER -
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@article{2014_Movahed,
author = {Siyavash Kazemi Movahed and Minoo Dabiri and Ayoob Bazgir},
title = {Palladium nanoparticle decorated high nitrogen-doped graphene with high catalytic activity for Suzuki–Miyaura and Ullmann-type coupling reactions in aqueous media},
journal = {Applied Catalysis A: General},
year = {2014},
volume = {488},
publisher = {Elsevier},
month = {nov},
url = {https://doi.org/10.1016/j.apcata.2014.09.045},
pages = {265--274},
doi = {10.1016/j.apcata.2014.09.045}
}