Bimetallic Ni-Co/SBA-15 catalysts prepared by urea co-precipitation for dry reforming of methane
Publication type: Journal Article
Publication date: 2018-03-01
scimago Q2
wos Q2
SJR: 1.000
CiteScore: 8.6
Impact factor: 4.8
ISSN: 0926860X, 18733875
Catalysis
Process Chemistry and Technology
Abstract
A series of NixCo(10-x)/SBA-15 catalysts with constant metal loading (10 wt%) and different Co/Ni mass ratios (0/10–10/0) were prepared by urea co-precipitation and applied to the dry reforming of methane (DRM). The physicochemical properties of the catalysts were characterized in detail by various techniques (N2 physisorption, H2 chemisorption, XRD, TPR, ICP-OES, TGA, HRTEM and XPS), revealing that Ni and Co particles were embedded into the channel of SBA-15 and Ni was alloyed with Co. In addition, the bimetallic catalysts with a Co/Ni ratio (RCo/Ni) lower than 1 had relatively high metal dispersion (ca. 17–20%) and small metal particle sizes (ca. 4–5 nm). The DRM activity and stability of NixCo(10-x)/SBA-15 in terms of coke- and sintering- resistance were systematically examined and compared, which showed that the activity and stability of the catalysts depended strongly on the metal particle size, indicating the structure-sensitive character of the DRM reaction. Compared to monometallic Ni10/SBA-15 and Co10/SBA-15, bimetallic NixCo(10-x)/SBA-15 with RCo/Ni
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Citations from 2025:
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Xin J. et al. Bimetallic Ni-Co/SBA-15 catalysts prepared by urea co-precipitation for dry reforming of methane // Applied Catalysis A: General. 2018. Vol. 554. pp. 95-104.
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Xin J., Cui H., Cheng Z., Zhou Z. Bimetallic Ni-Co/SBA-15 catalysts prepared by urea co-precipitation for dry reforming of methane // Applied Catalysis A: General. 2018. Vol. 554. pp. 95-104.
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TY - JOUR
DO - 10.1016/j.apcata.2018.01.033
UR - https://doi.org/10.1016/j.apcata.2018.01.033
TI - Bimetallic Ni-Co/SBA-15 catalysts prepared by urea co-precipitation for dry reforming of methane
T2 - Applied Catalysis A: General
AU - Xin, Jinni
AU - Cui, Hongjie
AU - Cheng, Zhen-Min
AU - Zhou, Zhiming
PY - 2018
DA - 2018/03/01
PB - Elsevier
SP - 95-104
VL - 554
SN - 0926-860X
SN - 1873-3875
ER -
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BibTex (up to 50 authors)
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@article{2018_Xin,
author = {Jinni Xin and Hongjie Cui and Zhen-Min Cheng and Zhiming Zhou},
title = {Bimetallic Ni-Co/SBA-15 catalysts prepared by urea co-precipitation for dry reforming of methane},
journal = {Applied Catalysis A: General},
year = {2018},
volume = {554},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/j.apcata.2018.01.033},
pages = {95--104},
doi = {10.1016/j.apcata.2018.01.033}
}