Phosphorus-modified b-axis oriented hierarchical ZSM-5 zeolites for enhancing catalytic performance in a methanol to propylene reaction
Publication type: Journal Article
Publication date: 2020-03-01
scimago Q2
wos Q2
SJR: 1.000
CiteScore: 8.6
Impact factor: 4.8
ISSN: 0926860X, 18733875
Catalysis
Process Chemistry and Technology
Abstract
In this work, a b-axis oriented hierarchical ZSM-5 zeolite was prepared with glucose as an additive and further modified by phosphorus to improve the propylene selectivity and prolong the lifetime of the catalyst in a methanol to propylene (MTP) reaction. The physiochemical properties were characterized by XRD, low-temperature N2 sorption, SEM, TEM, XPS, solid-state NMR, FTIR, and NH3-TPD analyses. The b-axis oriented ZSM-5 (Z5-C) zeolite exhibited a microsized hexagonal lamellar structure with a thickness of approximately 220 nm. Analyzing the MTP reactions revealed that the newly prepared Z5-C catalyst exhibited a higher propylene selectivity of 53.01 % and a longer lifetime of 45 h compared to those of a conventional nanosized ZSM-5 catalyst (propylene selectivity of 43.97 % and lifetime of 10 h). In addition, the phosphorus modification remarkably increased the lifetime of the b-axis-oriented ZSM-5 catalyst to 79 h.
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Total citations:
74
Citations from 2025:
15
(20.27%)
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GOST
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Feng R. et al. Phosphorus-modified b-axis oriented hierarchical ZSM-5 zeolites for enhancing catalytic performance in a methanol to propylene reaction // Applied Catalysis A: General. 2020. Vol. 594. p. 117464.
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Feng R., Yan X., Hu X., Zhang Y., Wu J., Yan Z. Phosphorus-modified b-axis oriented hierarchical ZSM-5 zeolites for enhancing catalytic performance in a methanol to propylene reaction // Applied Catalysis A: General. 2020. Vol. 594. p. 117464.
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TY - JOUR
DO - 10.1016/j.apcata.2020.117464
UR - https://doi.org/10.1016/j.apcata.2020.117464
TI - Phosphorus-modified b-axis oriented hierarchical ZSM-5 zeolites for enhancing catalytic performance in a methanol to propylene reaction
T2 - Applied Catalysis A: General
AU - Feng, Rui
AU - Yan, Xinlong
AU - Hu, Xiaoyan
AU - Zhang, Yixin
AU - Wu, Jianjun
AU - Yan, Zifeng
PY - 2020
DA - 2020/03/01
PB - Elsevier
SP - 117464
VL - 594
SN - 0926-860X
SN - 1873-3875
ER -
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@article{2020_Feng,
author = {Rui Feng and Xinlong Yan and Xiaoyan Hu and Yixin Zhang and Jianjun Wu and Zifeng Yan},
title = {Phosphorus-modified b-axis oriented hierarchical ZSM-5 zeolites for enhancing catalytic performance in a methanol to propylene reaction},
journal = {Applied Catalysis A: General},
year = {2020},
volume = {594},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/j.apcata.2020.117464},
pages = {117464},
doi = {10.1016/j.apcata.2020.117464}
}