Applied Catalysis B: Environmental

, том 89 , издание 1-2 , страницы 149-159

The effect of CeO2 on the surface and catalytic properties of Pt/CeO2–ZrO2 catalysts for methane dry reforming

Тип публикации: Journal Article

Дата публикации: 2009-07-01

Elsevier

Applied Catalysis B: Environmental

scimago Q1

wos Q1

БС1

SJR: 5.18

CiteScore: 38.4

Impact factor: 21.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2008.11.035

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Catalysis

Process Chemistry and Technology

General Environmental Science

Краткое описание

The CO 2 reforming of CH 4 over Pt catalysts supported on nanocrystalline mesoporous ZrO 2 and CeO 2 –ZrO 2 carriers was investigated at atmospheric pressure. The effect of CeO 2 content (1–12 wt%) on the surface and catalytic properties of the catalysts was studied. It was found that the pre-treatment temperature and the concentration of CeO 2 influence on the morphology of Pt particles. The calcination temperature as high as 1073 K leads to sintering of Pt particles deposited over zirconia- and CeO 2 -loaded zirconia substrates. Temperature-programmed reduction (TPR) results showed good reductive properties for Pt/CeO 2 –ZrO 2 catalysts due to both, the high surface shell reduction of zirconia and the synergetic effect between Pt and CeO 2 . X-ray photoelectron spectroscopy (XPS) of reduced catalysts revealed the presence of different Pt oxidation state depending on the catalyst composition. Stabilization of partially oxidized platinum species by ceria was detected for the reduced Pt/CeO 2 –ZrO 2 samples. An activation period was required for the stabilization of the activity of Pt/CeO 2 –ZrO 2 catalysts. The high stability of Pt/CeO 2 –ZrO 2 catalysts was related to the close contact between Pt and CeO 2 .

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Damyanova S. et al. The effect of CeO2 on the surface and catalytic properties of Pt/CeO2–ZrO2 catalysts for methane dry reforming // Applied Catalysis B: Environmental. 2009. Vol. 89. No. 1-2. pp. 149-159.

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Damyanova S., Pawelec B., Arishtirova K., Huerta M. V. M., Garcia Fierro J. L. The effect of CeO2 on the surface and catalytic properties of Pt/CeO2–ZrO2 catalysts for methane dry reforming // Applied Catalysis B: Environmental. 2009. Vol. 89. No. 1-2. pp. 149-159.

RIS |

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TY - JOUR

DO - 10.1016/j.apcatb.2008.11.035

UR - https://doi.org/10.1016/j.apcatb.2008.11.035

TI - The effect of CeO2 on the surface and catalytic properties of Pt/CeO2–ZrO2 catalysts for methane dry reforming

T2 - Applied Catalysis B: Environmental

AU - Damyanova, S

AU - Pawelec, B

AU - Arishtirova, K

AU - Huerta, M V Martínez

AU - Garcia Fierro, Jose Luis

PY - 2009

DA - 2009/07/01

PB - Elsevier

SP - 149-159

IS - 1-2

VL - 89

SN - 0926-3373

SN - 1873-3883

ER -

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@article{2009_Damyanova,

author = {S Damyanova and B Pawelec and K Arishtirova and M V Martínez Huerta and Jose Luis Garcia Fierro},

title = {The effect of CeO2 on the surface and catalytic properties of Pt/CeO2–ZrO2 catalysts for methane dry reforming},

journal = {Applied Catalysis B: Environmental},

year = {2009},

volume = {89},

publisher = {Elsevier},

month = {jul},

url = {https://doi.org/10.1016/j.apcatb.2008.11.035},

number = {1-2},

pages = {149--159},

doi = {10.1016/j.apcatb.2008.11.035}

}

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MLA Скопировать

Damyanova, S., et al. “The effect of CeO2 on the surface and catalytic properties of Pt/CeO2–ZrO2 catalysts for methane dry reforming.” Applied Catalysis B: Environmental, vol. 89, no. 1-2, Jul. 2009, pp. 149-159. https://doi.org/10.1016/j.apcatb.2008.11.035.

Издатель

Elsevier

Журнал

Applied Catalysis B: Environmental

scimago Q1

wos Q1

БС1

SJR

5.18

CiteScore

38.4

Impact factor

21.1

ISSN

09263373 (Print)

18733883 (Electronic)