Applied Catalysis B: Environmental

, volume 243 , pages 273-282

Catalytic application of ferrierite nanocrystals in vapour-phase dehydration of methanol to dimethyl ether

Enrico Catizzone ¹

Stijn Van Daele ²

Micaela Bianco ¹

A. Di Michele ³

Alfredo Aloise ¹

Massimo Migliori ¹

Valentin Valtchev ^{4, 5}

Girolamo Giordano ¹

Hide authors affiliations Show authors affiliations: 5 affiliations

Department of Environmental and Chemical Engineering, University of Calabria, Via P. Bucci, I-87036, Rende, CS, Italy |

Normandie University, Ensicaen, Unicaen, CNRS, Laboratoire Catalyse et Spectrochimie, 14000, Caen, France |

Department of Physics and Geology, University of Perugia, Via Pascoli, 1, 06123 Perugia, Italy |

⁴

Normandie Univ., ENSICAEN, UNICAEN, CNRS, Laboratoire Catalyse et Spectrochimie, 14000, Caen, France |

⁵

State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun, 130012, China |

Publication type: Journal Article

Publication date: 2019-04-01

Elsevier

Applied Catalysis B: Environmental

scimago Q1

wos Q1

SJR: 5.180

CiteScore: 38.4

Impact factor: 21.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2018.10.060

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Catalysis

Process Chemistry and Technology

General Environmental Science

Abstract

The FER-type zeolite was found to be a reliable catalyst for DME synthesis via both direct CO2 hydrogenation or gas phase methanol dehydration. In this work, the effect of the crystal size of FER-type zeolites on the catalytic behavior during methanol-to-DME conversion is studied. A series of FER-type crystals ranging from 0.1 μm to 10 μm in size were synthesized and their physicochemical properties (e.g. crystal morphology, acidity, textural characteristics) analyzed. The catalytic performance of FER-type catalysts was studied in a wide range of reaction temperatures (120–280 °C). The set experimental data show that the catalytic effectiveness of FER-type catalysts in terms of methanol conversion, DME selectivity and coke resistance, can strongly be improved by reducing the zeolite crystal size.

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Khalil Kamal

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PhD in Chemistry, professor, professor of the Royal Society

39 publications, 995 citations, 20 reviews

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GOST Copy

Catizzone E. et al. Catalytic application of ferrierite nanocrystals in vapour-phase dehydration of methanol to dimethyl ether // Applied Catalysis B: Environmental. 2019. Vol. 243. pp. 273-282.

GOST all authors (up to 50) Copy

Catizzone E., Daele S. V., Bianco M., Michele A. D., Aloise A., Migliori M., Valtchev V., Giordano G. Catalytic application of ferrierite nanocrystals in vapour-phase dehydration of methanol to dimethyl ether // Applied Catalysis B: Environmental. 2019. Vol. 243. pp. 273-282.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.apcatb.2018.10.060

UR - https://doi.org/10.1016/j.apcatb.2018.10.060

TI - Catalytic application of ferrierite nanocrystals in vapour-phase dehydration of methanol to dimethyl ether

T2 - Applied Catalysis B: Environmental

AU - Catizzone, Enrico

AU - Daele, Stijn Van

AU - Bianco, Micaela

AU - Michele, A. Di

AU - Aloise, Alfredo

AU - Migliori, Massimo

AU - Valtchev, Valentin

AU - Giordano, Girolamo

PY - 2019

DA - 2019/04/01

PB - Elsevier

SP - 273-282

VL - 243

SN - 0926-3373

SN - 1873-3883

ER -

BibTex

Cite this

BibTex (up to 50 authors) Copy

@article{2019_Catizzone,

author = {Enrico Catizzone and Stijn Van Daele and Micaela Bianco and A. Di Michele and Alfredo Aloise and Massimo Migliori and Valentin Valtchev and Girolamo Giordano},

title = {Catalytic application of ferrierite nanocrystals in vapour-phase dehydration of methanol to dimethyl ether},

journal = {Applied Catalysis B: Environmental},

year = {2019},

volume = {243},

publisher = {Elsevier},

month = {apr},

url = {https://doi.org/10.1016/j.apcatb.2018.10.060},

pages = {273--282},

doi = {10.1016/j.apcatb.2018.10.060}

}

Publisher

Elsevier

Journal

Applied Catalysis B: Environmental

scimago Q1

wos Q1

SJR

5.180

CiteScore

38.4

Impact factor

21.1

ISSN

09263373 (Print)

18733883 (Electronic)