Applied Catalysis B: Environmental, volume 268, pages 118738

2D/2D Ti3C2 MXene/g-C3N4 nanosheets heterojunction for high efficient CO2 reduction photocatalyst: Dual effects of urea

Chao Yang ¹

Qiuyan Tan ¹

Qin Li ¹

Jie Zhou ²

Jiajie Fan ³

Bing Li ⁴

Jie Sun ¹

Kangle Lv ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education College of Resources and Environmental Science South‐Central University for Nationalities Wuhan 430074 China |

Department of Urology, Hubei Provincial Hospital of Traditional Chinese Medicine, Wuhan 430061, China |

School of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001,China) |

⁴

Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang Provincial Collaborative Innovation Center for Bamboo Resources and High-efficiency Utilization, Zhejiang A & F University, Hangzhou 311300, China |

Publication type: Journal Article

Publication date: 2020-07-01

Elsevier

Journal: Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor: 22.1

ISSN: 09263373, 18733883

DOI: 10.1016/j.apcatb.2020.118738

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Catalysis

Process Chemistry and Technology

General Environmental Science

Abstract

• An ultrathin 2D/2D Ti 3 C 2 /g-C 3 N 4 heterojunction is synthesized by a one-pot strategy. • Urea works both as the gas template for exfoliating Ti 3 C 2 and the precursor of g-C 3 N 4 . • Ti 3 C 2 stimulates the transfer of photo-generated electron-hole pairs, retarding the recombination. • 2D/2D Ti 3 C 2 /g-C 3 N 4 heterojunction boosts the photoreactivity of g-C 3 N 4 for CO 2 reduction. In this paper, an ultrathin 2D/2D Ti 3 C 2 /g-C 3 N 4 heterojunction was synthesized by direct calcination the mixture of bulk Ti 3 C 2 and urea, where urea not only acts as the gas template to exfoliate Ti 3 C 2 into nanosheets, but also as the precursor of g-C 3 N 4 to craft Ti 3 C 2 /g-C 3 N 4 heterojunction. CO 2 photoreduction activity tests reveal that pure g-C 3 N 4 (UCN) exhibits very weak photoactivity. However, when Ti 3 C 2 was coupled with g-C 3 N 4 , the photocatalytic performance is soaringly enhanced. The optimal sample (10TC) shows the yields of 5.19 and 0.044 μmol h −1 g −1 for CO and CH 4 , respectively, and the total CO 2 conversion is 8.1 times higher than that of UCN. The enhanced CO 2 photoreduction activity is mainly attributed to the combined effects of (1) improved CO 2 adsorption and activation, and (2) the construction of ultrathin 2D/2D Ti 3 C 2 /g-C 3 N 4 heterojunction, where the intimate contact stimulates an efficient spatial separation of photo-excited charge carriers.

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Chemical Engineering Journal	Chemical Engineering Journal, 31, 6.89% Chemical Engineering Journal 31 publications, 6.89%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 21, 4.67% Applied Catalysis B: Environmental 21 publications, 4.67%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 18, 4% Journal of Colloid and Interface Science 18 publications, 4%
Chemosphere	Chemosphere, 13, 2.89% Chemosphere 13 publications, 2.89%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 13, 2.89% Journal of Alloys and Compounds 13 publications, 2.89%
Journal of Environmental Chemical Engineering	Journal of Environmental Chemical Engineering, 13, 2.89% Journal of Environmental Chemical Engineering 13 publications, 2.89%
Separation and Purification Technology	Separation and Purification Technology, 13, 2.89% Separation and Purification Technology 13 publications, 2.89%
Applied Surface Science	Applied Surface Science, 12, 2.67% Applied Surface Science 12 publications, 2.67%
Energy & Fuels	Energy & Fuels, 11, 2.44% Energy & Fuels 11 publications, 2.44%
Small	Small, 10, 2.22% Small 10 publications, 2.22%
ACS Symposium Series	ACS Symposium Series, 10, 2.22% ACS Symposium Series 10 publications, 2.22%
Solar RRL	Solar RRL, 9, 2% Solar RRL 9 publications, 2%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 9, 2% Journal of Materials Chemistry A 9 publications, 2%
International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 8, 1.78% International Journal of Hydrogen Energy 8 publications, 1.78%
Catalysts	Catalysts, 7, 1.56% Catalysts 7 publications, 1.56%
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Catalysis Science and Technology	Catalysis Science and Technology, 6, 1.33% Catalysis Science and Technology 6 publications, 1.33%
Nano Research	Nano Research, 5, 1.11% Nano Research 5 publications, 1.11%
Journal of CO2 Utilization	Journal of CO2 Utilization, 5, 1.11% Journal of CO2 Utilization 5 publications, 1.11%
Colloids and Surfaces A: Physicochemical and Engineering Aspects	Colloids and Surfaces A: Physicochemical and Engineering Aspects, 5, 1.11% Colloids and Surfaces A: Physicochemical and Engineering Aspects 5 publications, 1.11%
ACS Applied Nano Materials	ACS Applied Nano Materials, 4, 0.89% ACS Applied Nano Materials 4 publications, 0.89%
Materials Research Bulletin	Materials Research Bulletin, 4, 0.89% Materials Research Bulletin 4 publications, 0.89%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 4, 0.89% Coordination Chemistry Reviews 4 publications, 0.89%
ChemistrySelect	ChemistrySelect, 4, 0.89% ChemistrySelect 4 publications, 0.89%
Langmuir	Langmuir, 4, 0.89% Langmuir 4 publications, 0.89%
Inorganic Chemistry	Inorganic Chemistry, 4, 0.89% Inorganic Chemistry 4 publications, 0.89%
ACS Catalysis	ACS Catalysis, 3, 0.67% ACS Catalysis 3 publications, 0.67%
Molecules	Molecules, 3, 0.67% Molecules 3 publications, 0.67%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 3, 0.67% Journal of Materials Science: Materials in Electronics 3 publications, 0.67%
	5 10 15 20 25 30 35

Citations by publishers

	50 100 150 200 250
Elsevier	Elsevier, 231, 51.33% Elsevier 231 publications, 51.33%
Wiley	Wiley, 61, 13.56% Wiley 61 publications, 13.56%
American Chemical Society (ACS)	American Chemical Society (ACS), 57, 12.67% American Chemical Society (ACS) 57 publications, 12.67%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 39, 8.67% Royal Society of Chemistry (RSC) 39 publications, 8.67%
Springer Nature	Springer Nature, 19, 4.22% Springer Nature 19 publications, 4.22%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 15, 3.33% Multidisciplinary Digital Publishing Institute (MDPI) 15 publications, 3.33%
KeAi Communications Co.	KeAi Communications Co., 3, 0.67% KeAi Communications Co. 3 publications, 0.67%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 0.44% American Institute of Physics (AIP) 2 publications, 0.44%
Frontiers Media S.A.	Frontiers Media S.A., 2, 0.44% Frontiers Media S.A. 2 publications, 0.44%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 2, 0.44% Nonferrous Metals Society of China 2 publications, 0.44%
IOS Press	IOS Press, 2, 0.44% IOS Press 2 publications, 0.44%
IOP Publishing	IOP Publishing, 2, 0.44% IOP Publishing 2 publications, 0.44%
Bentham Science	Bentham Science, 1, 0.22% Bentham Science 1 publication, 0.22%
World Scientific	World Scientific, 1, 0.22% World Scientific 1 publication, 0.22%
Tianjin Daxue/Tianjin University	Tianjin Daxue/Tianjin University, 1, 0.22% Tianjin Daxue/Tianjin University 1 publication, 0.22%
Chemical Industry Press	Chemical Industry Press, 1, 0.22% Chemical Industry Press 1 publication, 0.22%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.22% Taiwan Institute of Chemical Engineers 1 publication, 0.22%
Walter de Gruyter	Walter de Gruyter, 1, 0.22% Walter de Gruyter 1 publication, 0.22%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.22% Korean Society of Industrial Engineering Chemistry 1 publication, 0.22%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.22% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.22%
	50 100 150 200 250

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Yang C. et al. 2D/2D Ti3C2 MXene/g-C3N4 nanosheets heterojunction for high efficient CO2 reduction photocatalyst: Dual effects of urea // Applied Catalysis B: Environmental. 2020. Vol. 268. p. 118738.

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Yang C., Tan Q., Li Q., Zhou J., Fan J., Li B., Sun J., Lv K. 2D/2D Ti3C2 MXene/g-C3N4 nanosheets heterojunction for high efficient CO2 reduction photocatalyst: Dual effects of urea // Applied Catalysis B: Environmental. 2020. Vol. 268. p. 118738.

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RIS Copy

TY - JOUR

DO - 10.1016/j.apcatb.2020.118738

UR - https://doi.org/10.1016/j.apcatb.2020.118738

TI - 2D/2D Ti3C2 MXene/g-C3N4 nanosheets heterojunction for high efficient CO2 reduction photocatalyst: Dual effects of urea

T2 - Applied Catalysis B: Environmental

AU - Yang, Chao

AU - Tan, Qiuyan

AU - Li, Qin

AU - Zhou, Jie

AU - Fan, Jiajie

AU - Li, Bing

AU - Sun, Jie

AU - Lv, Kangle

PY - 2020

DA - 2020/07/01 00:00:00

PB - Elsevier

SP - 118738

VL - 268

SN - 0926-3373

SN - 1873-3883

ER -

BibTex

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BibTex Copy

@article{2020_Yang,

author = {Chao Yang and Qiuyan Tan and Qin Li and Jie Zhou and Jiajie Fan and Bing Li and Jie Sun and Kangle Lv},

title = {2D/2D Ti3C2 MXene/g-C3N4 nanosheets heterojunction for high efficient CO2 reduction photocatalyst: Dual effects of urea},

journal = {Applied Catalysis B: Environmental},

year = {2020},

volume = {268},

publisher = {Elsevier},

month = {jul},

url = {https://doi.org/10.1016/j.apcatb.2020.118738},

pages = {118738},

doi = {10.1016/j.apcatb.2020.118738}

}

Found error?

Publisher

Elsevier

Journal

Applied Catalysis B: Environmental

Quartile SCImago

Quartile WOS

Impact factor

22.1

ISSN

09263373 (Print)
18733883 (Electronic)