Applied Surface Science, volume 441, pages 12-22

Self-assembled hierarchical direct Z-scheme g-C3N4/ZnO microspheres with enhanced photocatalytic CO2 reduction performance

Ning Nie ¹

Liu-Yang Zhang ¹

Junwei Fu ¹

BEI CHENG ²

Hide authors affiliations Show authors affiliations: 2 affiliations

State Key Laboratory of Advanced Technology for Material Synthesis and Processing, Wuhan University of Technology, Wuhan, 430070, PR China |

Faculty of Science, King Abdulaziz University, Jeddah 21589, Saudi Arabia |

Publication type: Journal Article

Publication date: 2018-05-01

Elsevier

Journal: Applied Surface Science

Quartile SCImago

Quartile WOS

Impact factor: 6.7

ISSN: 01694332

DOI: 10.1016/j.apsusc.2018.01.193

Copy DOI

Surfaces, Coatings and Films

General Chemistry

General Physics and Astronomy

Condensed Matter Physics

Surfaces and Interfaces

Abstract

Photocatalytic reduction of CO2 into hydrocarbon fuels has been regarded as a promising approach to ease the greenhouse effect and the energy shortage. Herein, an electrostatic self-assembly method was exploited to prepare g-C3N4/ZnO composite microsphere. This method simply utilized the opposite surface charge of each component, achieving a hierarchical structure with intimate contact between them. A much improved photocatalytic CO2 reduction activity was attained. The CH3OH production rate was 1.32 μmol h−1 g−1, which was 2.1 and 4.1 times more than that of the pristine ZnO and g-C3N4, respectively. This facile design bestowed the g-C3N4/ZnO composite an extended light adsorption caused by multi-light scattering effect. It also guaranteed the uniform distribution of g-C3N4 nanosheets on the surface of ZnO microspheres, maximizing their advantage and synergistic effect. Most importantly, the preeminent performance was proposed and validated based on the direct Z-scheme. The recombination rate was considerably suppressed. This work features the meliority of constructing hierarchical direct Z-scheme structures in photocatalytic CO2 reduction reactions.

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Citations by publishers

	50 100 150 200 250
Elsevier	Elsevier, 237, 65.65% Elsevier 237 publications, 65.65%
Wiley	Wiley, 30, 8.31% Wiley 30 publications, 8.31%
Springer Nature	Springer Nature, 23, 6.37% Springer Nature 23 publications, 6.37%
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King Saud University	King Saud University, 2, 0.55% King Saud University 2 publications, 0.55%
World Scientific	World Scientific, 1, 0.28% World Scientific 1 publication, 0.28%
The Electrochemical Society	The Electrochemical Society, 1, 0.28% The Electrochemical Society 1 publication, 0.28%
Scrivener Publishing	Scrivener Publishing, 1, 0.28% Scrivener Publishing 1 publication, 0.28%
Tianjin Daxue/Tianjin University	Tianjin Daxue/Tianjin University, 1, 0.28% Tianjin Daxue/Tianjin University 1 publication, 0.28%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.28% Taiwan Institute of Chemical Engineers 1 publication, 0.28%
Taylor & Francis	Taylor & Francis, 1, 0.28% Taylor & Francis 1 publication, 0.28%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.28% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.28%
	50 100 150 200 250

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Nie N. et al. Self-assembled hierarchical direct Z-scheme g-C3N4/ZnO microspheres with enhanced photocatalytic CO2 reduction performance // Applied Surface Science. 2018. Vol. 441. pp. 12-22.

GOST all authors (up to 50) Copy

Nie N., Zhang L., Fu J., CHENG B. Self-assembled hierarchical direct Z-scheme g-C3N4/ZnO microspheres with enhanced photocatalytic CO2 reduction performance // Applied Surface Science. 2018. Vol. 441. pp. 12-22.

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RIS Copy

TY - JOUR

DO - 10.1016/j.apsusc.2018.01.193

UR - https://doi.org/10.1016/j.apsusc.2018.01.193

TI - Self-assembled hierarchical direct Z-scheme g-C3N4/ZnO microspheres with enhanced photocatalytic CO2 reduction performance

T2 - Applied Surface Science

AU - Nie, Ning

AU - Zhang, Liu-Yang

AU - Fu, Junwei

AU - CHENG, BEI

PY - 2018

DA - 2018/05/01 00:00:00

PB - Elsevier

SP - 12-22

VL - 441

SN - 0169-4332

ER -

BibTex

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BibTex Copy

@article{2018_Nie,

author = {Ning Nie and Liu-Yang Zhang and Junwei Fu and BEI CHENG},

title = {Self-assembled hierarchical direct Z-scheme g-C3N4/ZnO microspheres with enhanced photocatalytic CO2 reduction performance},

journal = {Applied Surface Science},

year = {2018},

volume = {441},

publisher = {Elsevier},

month = {may},

url = {https://doi.org/10.1016/j.apsusc.2018.01.193},

pages = {12--22},

doi = {10.1016/j.apsusc.2018.01.193}

}

Found error?

Publisher

Elsevier

Journal

Applied Surface Science

Quartile SCImago

Quartile WOS

Impact factor

6.7

ISSN

01694332 (Print)