Applied Surface Science, volume 456, pages 801-807
C60 layer growth on intact and Tl-modified Si(1 1 1)5 ×
1
2
Instute of Physics of Microstructures RAS, Nizhnii Novgorod 603950, Russia
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Publication type: Journal Article
Publication date: 2018-10-01
Journal:
Applied Surface Science
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 6.7
ISSN: 01694332
Surfaces, Coatings and Films
General Chemistry
General Physics and Astronomy
Condensed Matter Physics
Surfaces and Interfaces
Abstract
The Si(1 1 1)5 × 2-Au surface comprises a quasi-one-dimensional surface reconstruction consisting of Au stripes mediated by honeycomb Si chains. In the present study, using STM observations we explored adsorption of thallium (Tl) onto Si(1 1 1)5 × 2-Au surface as well as growth of C60 layers on Tl-modified and intact Si(1 1 1)5 × 2-Au surfaces. Analysis of the results was based on the recently proposed KK model of Si(1 1 1)5 × 2-Au surface [Kwon and Kang, PRL 113 (2014) 086101]. It was found that intact Si(1 1 1)5 × 2-Au surface produces a poor template effect on the overgrown C60 layers which have a close-packed-like structure without distinct ordering. In contrast, the C60 layers grown on the Tl-adsorbed Si(1 1 1)5 × 2-Au surface where Tl atoms occupy various adsorption sites on the honeycomb Si chains have a well-ordered quasi-one-dimensional structure consisting of straight C60 chains. Ordering of the C60 molecules is a result of an intricate interplay between adsorbed C60 molecules with each other and with a substrate surface. Separation between neighboring C60 chains is dictated by the periodicity of the underlying Si(1 1 1)5 × 2-Au template, while the C60-C60 spacing within the chains of ∼ 12 A that is ∼ 3.2 a 0 reflects the peculiarity of the C60-C60 intermolecular interaction on the Tl-adsorbed Si(1 1 1)5 × 2-Au surface. Structural information on (Au, Tl)/Si(1 1 1) and C60/(Au, Tl)/Si(1 1 1) systems gained in the present study can be useful for the prospective works on elucidating the ways to control electronic properties of the Si(1 1 1)5 × 2-Au surface using atomic and molecular adsorbates.
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1 publication, 20%
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Citations by publishers
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2 publications, 40%
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1 publication, 20%
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American Physical Society (APS)
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1 publication, 20%
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IOP Publishing
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IOP Publishing
1 publication, 20%
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Olyanich D. A. et al. C60 layer growth on intact and Tl-modified Si(1 1 1)5 × 2-Au surfaces // Applied Surface Science. 2018. Vol. 456. pp. 801-807.
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Olyanich D. A., Mararov V. V., Utas T. V., Aladyshkin A. Y., Mihalyuk A. N., ZOTOV A., Saranin A. C60 layer growth on intact and Tl-modified Si(1 1 1)5 × 2-Au surfaces // Applied Surface Science. 2018. Vol. 456. pp. 801-807.
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TY - JOUR
DO - 10.1016/j.apsusc.2018.06.202
UR - https://doi.org/10.1016%2Fj.apsusc.2018.06.202
TI - C60 layer growth on intact and Tl-modified Si(1 1 1)5 × 2-Au surfaces
T2 - Applied Surface Science
AU - Olyanich, Dmitry A.
AU - Mararov, Vsevolod V.
AU - Utas, Tatiana V.
AU - Aladyshkin, A. Yu.
AU - Mihalyuk, A. N.
AU - ZOTOV, A.V.
AU - Saranin, A.A.
PY - 2018
DA - 2018/10/01 00:00:00
PB - Elsevier
SP - 801-807
VL - 456
SN - 0169-4332
ER -
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@article{2018_Olyanich,
author = {Dmitry A. Olyanich and Vsevolod V. Mararov and Tatiana V. Utas and A. Yu. Aladyshkin and A. N. Mihalyuk and A.V. ZOTOV and A.A. Saranin},
title = {C60 layer growth on intact and Tl-modified Si(1 1 1)5 × 2-Au surfaces},
journal = {Applied Surface Science},
year = {2018},
volume = {456},
publisher = {Elsevier},
month = {oct},
url = {https://doi.org/10.1016%2Fj.apsusc.2018.06.202},
pages = {801--807},
doi = {10.1016/j.apsusc.2018.06.202}
}