Applied Surface Science, volume 509, pages 144773
Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor
Qiang Guo
1, 2
,
Liming Fu
1
,
Tao Yan
1
,
Wen Tian
1
,
Danfeng Ma
1
,
Jiaming Li
1
,
Yanan Jiang
1
,
Xitao Wang
1
Publication type: Journal Article
Publication date: 2020-04-01
Journal:
Applied Surface Science
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 6.7
ISSN: 01694332
Surfaces, Coatings and Films
General Chemistry
General Physics and Astronomy
Condensed Matter Physics
Surfaces and Interfaces
Abstract
Porous ZnO nanosheets (PNS-ZnO) were prepared by calcining ZnS(en)0.5 (en = ethylenediamine) nanosheets in air, and g-C3N4 (g-CN) nanofilms were coated on the surface of PNS-ZnO by thermal deposition using bulk g-C3N4 as precursor. Experimental results showed that the graphene-like g-C3N4 could be deposited on the surface of ZnO to form nanocomposites with core/shell structure. After the loading of g-CN, the light absorption and chemical adsorption of CO2 over PNS-ZnO were improved obviously and the recombination of photogenerated electron and hole was greatly depressed due to the formation of heterojunction between PNS-ZnO and g-CN. All PNS-ZnO@g-CN nanocomposites exhibited much higher photocatalytic activity for CO2 reduction with H2O vapor when compared to pure PNS-ZnO and bulk g-CN. The loading amount of g-CN had significant influence on the light absorption and photocatalytic activity, and PNS-ZnO@g-CN-0.4 exhibited the best photocatalytic performance, for which H2, CH4 and CO production rates of 22.7, 30.5 and 16.8 μmol/gcat/h can be obtained, respectively.
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1 publication, 1.32%
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1
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Citations by publishers
5
10
15
20
25
30
35
40
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Elsevier
38 publications, 50%
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Royal Society of Chemistry (RSC)
9 publications, 11.84%
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Wiley
9 publications, 11.84%
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American Chemical Society (ACS)
9 publications, 11.84%
|
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Multidisciplinary Digital Publishing Institute (MDPI)
4 publications, 5.26%
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Springer Nature
2 publications, 2.63%
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IOP Publishing
2 publications, 2.63%
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Taylor & Francis
2 publications, 2.63%
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|
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 1.32%
|
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5
10
15
20
25
30
35
40
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Guo Q. et al. Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor // Applied Surface Science. 2020. Vol. 509. p. 144773.
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Guo Q., Fu L., Yan T., Tian W., Ma D., Li J., Jiang Y., Wang X. Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor // Applied Surface Science. 2020. Vol. 509. p. 144773.
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TY - JOUR
DO - 10.1016/j.apsusc.2019.144773
UR - https://doi.org/10.1016/j.apsusc.2019.144773
TI - Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor
T2 - Applied Surface Science
AU - Guo, Qiang
AU - Fu, Liming
AU - Yan, Tao
AU - Tian, Wen
AU - Ma, Danfeng
AU - Li, Jiaming
AU - Jiang, Yanan
AU - Wang, Xitao
PY - 2020
DA - 2020/04/01 00:00:00
PB - Elsevier
SP - 144773
VL - 509
SN - 0169-4332
ER -
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@article{2020_Guo,
author = {Qiang Guo and Liming Fu and Tao Yan and Wen Tian and Danfeng Ma and Jiaming Li and Yanan Jiang and Xitao Wang},
title = {Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor},
journal = {Applied Surface Science},
year = {2020},
volume = {509},
publisher = {Elsevier},
month = {apr},
url = {https://doi.org/10.1016/j.apsusc.2019.144773},
pages = {144773},
doi = {10.1016/j.apsusc.2019.144773}
}