volume 29 issue 12 pages 1440-1445

Synthesis and evaluation of the HIF-1α inhibitory activities of novel ursolic acid tetrazole derivatives

Lin-Hao Zhang 1
Zhi-Hong Zhang 1
Ming Yue Li 1
Zhi-Yu Wei 2
Xue-Jun Jin 1
Hu-Ri Piao 1
1
 
Key Laboratory of Natural Resources of Changbai Mountain and Functional Molecules, Ministry of Education, Yanbian University College of Pharmacy, Yanji, 133002, China.
Publication typeJournal Article
Publication date2019-06-01
scimago Q2
wos Q2
SJR0.472
CiteScore5.1
Impact factor2.2
ISSN0960894X, 14643405
Organic Chemistry
Drug Discovery
Biochemistry
Molecular Biology
Pharmaceutical Science
Clinical Biochemistry
Molecular Medicine
Abstract
The hypoxia-inducible factor-1α (HIF-1α) pathway has been implicated in tumor angiogenesis, growth, and metastasis. Therefore, the inhibition of this pathway is an important therapeutic target for the treatment of various types of cancers. Here, we designed and synthesized 31 ursolic acid (UA) derivatives containing a tetrazole moiety and evaluated them for their potential anti-tumor activities as HIF-1α transcriptional inhibitors. Of these, compound 14d (IC50 0.8 ± 0.2 µM) displayed the most potent activity and compounds 14a (IC50 4.7 ± 0.2 µM) exhibited the most promising biological profile. Analysis of the structure-activity relationships of these compounds with HIF-1α suggested that the presence of a tetrazole group located at C-28 of the UA derivatives was critical for their inhibitory activities.
Found 
Found 

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GOST |
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GOST Copy
Zhang L. et al. Synthesis and evaluation of the HIF-1α inhibitory activities of novel ursolic acid tetrazole derivatives // Bioorganic and Medicinal Chemistry Letters. 2019. Vol. 29. No. 12. pp. 1440-1445.
GOST all authors (up to 50) Copy
Zhang L., Zhang Z., Li M. Y., Wei Z., Jin X., Piao H. Synthesis and evaluation of the HIF-1α inhibitory activities of novel ursolic acid tetrazole derivatives // Bioorganic and Medicinal Chemistry Letters. 2019. Vol. 29. No. 12. pp. 1440-1445.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1016/j.bmcl.2019.04.028
UR - https://doi.org/10.1016/j.bmcl.2019.04.028
TI - Synthesis and evaluation of the HIF-1α inhibitory activities of novel ursolic acid tetrazole derivatives
T2 - Bioorganic and Medicinal Chemistry Letters
AU - Zhang, Lin-Hao
AU - Zhang, Zhi-Hong
AU - Li, Ming Yue
AU - Wei, Zhi-Yu
AU - Jin, Xue-Jun
AU - Piao, Hu-Ri
PY - 2019
DA - 2019/06/01
PB - Elsevier
SP - 1440-1445
IS - 12
VL - 29
PMID - 31006525
SN - 0960-894X
SN - 1464-3405
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2019_Zhang,
author = {Lin-Hao Zhang and Zhi-Hong Zhang and Ming Yue Li and Zhi-Yu Wei and Xue-Jun Jin and Hu-Ri Piao},
title = {Synthesis and evaluation of the HIF-1α inhibitory activities of novel ursolic acid tetrazole derivatives},
journal = {Bioorganic and Medicinal Chemistry Letters},
year = {2019},
volume = {29},
publisher = {Elsevier},
month = {jun},
url = {https://doi.org/10.1016/j.bmcl.2019.04.028},
number = {12},
pages = {1440--1445},
doi = {10.1016/j.bmcl.2019.04.028}
}
MLA
Cite this
MLA Copy
Zhang, Lin-Hao, et al. “Synthesis and evaluation of the HIF-1α inhibitory activities of novel ursolic acid tetrazole derivatives.” Bioorganic and Medicinal Chemistry Letters, vol. 29, no. 12, Jun. 2019, pp. 1440-1445. https://doi.org/10.1016/j.bmcl.2019.04.028.