Open Access
Preparation of carbon nanofibres supported palladium catalysts for hydrodechlorination reactions
Publication type: Journal Article
Publication date: 2008-06-01
scimago Q1
wos Q2
SJR: 0.811
CiteScore: 7.9
Impact factor: 4.3
ISSN: 15667367
General Chemistry
Catalysis
Process Chemistry and Technology
Abstract
Palladium catalysts (0.5 and 1 wt%) supported on carbon nanofibres were prepared and tested for tetrachloroethylene (TTCE) catalytic hydrodechlorination working with high organic loadings (using TTCE/toluene mixture, 0.9 M, that simulate real chlorinated wastes). For comparison, a commercial 0.5%-Pd/activated carbon catalyst was also tested for this reaction. CNF-based catalysts showed lower initial activity than the activated carbon-supported catalyst (40% vs. 60% initial conversion) but higher stability (after 25 h on stream activated carbon-based catalyst is completely deactivated whereas CNF-based catalysts show activities of about 15%). The fresh and used catalysts were characterized by BET, TEM, SEM, XRD and XPS. Results obtained suggest that the catalyst deactivation is caused by a combination of coke formation (lower amounts than in the case of conventional supports), and chlorine-poisoning.
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16
Total citations:
16
Citations from 2024:
1
(6.25%)
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GOST
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Bueres R. F. et al. Preparation of carbon nanofibres supported palladium catalysts for hydrodechlorination reactions // Catalysis Communications. 2008. Vol. 9. No. 10. pp. 2080-2084.
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Bueres R. F., Asedegbega Nieto E., Díaz E., Ordóñez S. G., Díez F. V. Preparation of carbon nanofibres supported palladium catalysts for hydrodechlorination reactions // Catalysis Communications. 2008. Vol. 9. No. 10. pp. 2080-2084.
Cite this
RIS
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TY - JOUR
DO - 10.1016/j.catcom.2008.04.005
UR - https://doi.org/10.1016/j.catcom.2008.04.005
TI - Preparation of carbon nanofibres supported palladium catalysts for hydrodechlorination reactions
T2 - Catalysis Communications
AU - Bueres, Ruben F
AU - Asedegbega Nieto, E
AU - Díaz, Eva
AU - Ordóñez, Salvador Gutiérrez
AU - Díez, Fernando V
PY - 2008
DA - 2008/06/01
PB - Elsevier
SP - 2080-2084
IS - 10
VL - 9
SN - 1566-7367
ER -
Cite this
BibTex (up to 50 authors)
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@article{2008_Bueres,
author = {Ruben F Bueres and E Asedegbega Nieto and Eva Díaz and Salvador Gutiérrez Ordóñez and Fernando V Díez},
title = {Preparation of carbon nanofibres supported palladium catalysts for hydrodechlorination reactions},
journal = {Catalysis Communications},
year = {2008},
volume = {9},
publisher = {Elsevier},
month = {jun},
url = {https://doi.org/10.1016/j.catcom.2008.04.005},
number = {10},
pages = {2080--2084},
doi = {10.1016/j.catcom.2008.04.005}
}
Cite this
MLA
Copy
Bueres, Ruben F., et al. “Preparation of carbon nanofibres supported palladium catalysts for hydrodechlorination reactions.” Catalysis Communications, vol. 9, no. 10, Jun. 2008, pp. 2080-2084. https://doi.org/10.1016/j.catcom.2008.04.005.