Open Access
Hydrodechlorination of chlorophenols at low temperature over highly defective Pd catalyst
Publication type: Journal Article
Publication date: 2013-11-01
scimago Q1
wos Q2
SJR: 0.811
CiteScore: 7.9
Impact factor: 4.3
ISSN: 15667367
General Chemistry
Catalysis
Process Chemistry and Technology
Abstract
Hydrodechlorination of chlorophenols at lower temperature was investigated over Pd catalyst supported on mesoporous silica-carbon nanocomposites (Pd/MSC). Characterization by XRD, HRTEM and H2-TPD has shown Pd nanoparticles of 7 nm with saw-edged GB at nanocrystal joining areas and edge steps. The catalyst exhibits high activity for hydrodechlorination of chlorophenols at 258–313 K under normal hydrogen pressure. Using triethylamine as a probe combining with further theoretical calculation, it reveals that the HDC of chlorophenols at low temperature mainly occurs on Pd defects, meanwhile reactive H species plays a direct role when the reactant adsorbs on Pd via the formation of eithei π- or σ-complex.
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12
Total citations:
12
Citations from 2024:
1
(8.33%)
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GOST
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Cheng L., Jin Z., Wang X. Hydrodechlorination of chlorophenols at low temperature over highly defective Pd catalyst // Catalysis Communications. 2013. Vol. 41. pp. 60-64.
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Cheng L., Jin Z., Wang X. Hydrodechlorination of chlorophenols at low temperature over highly defective Pd catalyst // Catalysis Communications. 2013. Vol. 41. pp. 60-64.
Cite this
RIS
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TY - JOUR
DO - 10.1016/j.catcom.2013.06.014
UR - https://doi.org/10.1016/j.catcom.2013.06.014
TI - Hydrodechlorination of chlorophenols at low temperature over highly defective Pd catalyst
T2 - Catalysis Communications
AU - Cheng, Lin
AU - Jin, Zhonghao
AU - Wang, Xing-Yi
PY - 2013
DA - 2013/11/01
PB - Elsevier
SP - 60-64
VL - 41
SN - 1566-7367
ER -
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BibTex (up to 50 authors)
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@article{2013_Cheng,
author = {Lin Cheng and Zhonghao Jin and Xing-Yi Wang},
title = {Hydrodechlorination of chlorophenols at low temperature over highly defective Pd catalyst},
journal = {Catalysis Communications},
year = {2013},
volume = {41},
publisher = {Elsevier},
month = {nov},
url = {https://doi.org/10.1016/j.catcom.2013.06.014},
pages = {60--64},
doi = {10.1016/j.catcom.2013.06.014}
}