Open Access
Ag–Ni bimetallic SiBEA zeolite as an efficient catalyst of hydrodechlorination of 1,2-dichloroethane towards ethylene
3
CNRS, UMR 7197, Laboratoire de Réactivité de Surface, F-75005, Paris, France
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Publication type: Journal Article
Publication date: 2015-09-01
scimago Q1
wos Q2
SJR: 0.811
CiteScore: 7.9
Impact factor: 4.3
ISSN: 15667367
General Chemistry
Catalysis
Process Chemistry and Technology
Abstract
Dealuminated form of BEA zeolite with Si/Al ratio of 1500 was used for the synthesis of Ag2.0SiBEA, Ni2.0SiBEA and Ag2.0Ni2.0SiBEA by two-step postsynthesis method. The calcination of zeolite samples led to the formation of well dispersed isolated mononuclear Ag(I) and Agnδ + clusters and a pseudo-tetrahedral Ni(II), incorporated in BEA framework as evidenced by DR UV–vis investigations. The treatment of samples in flowing 10% H2/Ar stream gave small (average 3.1 nm) and well dispersed metal nanoparticles. Reduced catalysts were investigated in 1,2-dichloroethane hydrodechlorination at atmospheric pressure, at low reaction temperature (523 K) with ~ 100% of selectivity to ethylene, desired product of the reaction.
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14
Total citations:
14
Citations from 2024:
1
(7.14%)
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Śrębowata A. et al. Ag–Ni bimetallic SiBEA zeolite as an efficient catalyst of hydrodechlorination of 1,2-dichloroethane towards ethylene // Catalysis Communications. 2015. Vol. 69. pp. 154-160.
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Śrębowata A., Zielińska I., Baran R., Słowik G. P., Dzwigaj S. Ag–Ni bimetallic SiBEA zeolite as an efficient catalyst of hydrodechlorination of 1,2-dichloroethane towards ethylene // Catalysis Communications. 2015. Vol. 69. pp. 154-160.
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TY - JOUR
DO - 10.1016/j.catcom.2015.06.009
UR - https://doi.org/10.1016/j.catcom.2015.06.009
TI - Ag–Ni bimetallic SiBEA zeolite as an efficient catalyst of hydrodechlorination of 1,2-dichloroethane towards ethylene
T2 - Catalysis Communications
AU - Śrębowata, A.
AU - Zielińska, I
AU - Baran, R
AU - Słowik, Grzegorz P.
AU - Dzwigaj, Stanislaw
PY - 2015
DA - 2015/09/01
PB - Elsevier
SP - 154-160
VL - 69
SN - 1566-7367
ER -
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@article{2015_Śrębowata,
author = {A. Śrębowata and I Zielińska and R Baran and Grzegorz P. Słowik and Stanislaw Dzwigaj},
title = {Ag–Ni bimetallic SiBEA zeolite as an efficient catalyst of hydrodechlorination of 1,2-dichloroethane towards ethylene},
journal = {Catalysis Communications},
year = {2015},
volume = {69},
publisher = {Elsevier},
month = {sep},
url = {https://doi.org/10.1016/j.catcom.2015.06.009},
pages = {154--160},
doi = {10.1016/j.catcom.2015.06.009}
}