Catalysis Today

, том 144 , издание 3-4 , страницы 265-272

Methane aromatization on Zn-modified zeolite in the presence of a co-reactant higher alkane: How does it occur?

Тип публикации: Journal Article

Дата публикации: 2009-06-30

Elsevier

Catalysis Today

scimago Q1

wos Q1

БС1

SJR: 1.05

CiteScore: 11.2

Impact factor: 5.3

ISSN: 09205861, 18734308

DOI: 10.1016/j.cattod.2008.08.043

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General Chemistry

Catalysis

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By using 13 C solid-state NMR and GC–MS, the analysis of the 13 C-label transfer from methane- 13 C into the products of methane and propane co-aromatization on Zn/H-BEA zeolite at 823–873 K has been performed. A high degree involvement of 13 C-carbon atoms of methane into aromatic products (benzene, toluene, xylenes) has been demonstrated. The main pathway of methane conversion into aromatics has been determined to consist in the methylation of aromatics, which is produced exclusively from propane, by methane. The methoxy species formed by the dissociative adsorption of methane on ZnO species of the zeolite is responsible for the methylation.

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Luzgin M. V. et al. Methane aromatization on Zn-modified zeolite in the presence of a co-reactant higher alkane: How does it occur? // Catalysis Today. 2009. Vol. 144. No. 3-4. pp. 265-272.

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Luzgin M. V., Rogov V. V., ARZUMANOV S., Toktarev A., Stepanov A., Parmon V. N. Methane aromatization on Zn-modified zeolite in the presence of a co-reactant higher alkane: How does it occur? // Catalysis Today. 2009. Vol. 144. No. 3-4. pp. 265-272.

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