Catalytic oxidative conversion of methane and ethane over polyoxometalate-derived catalysts in electric field at low temperature
Тип публикации: Journal Article
Дата публикации: 2018-01-01
scimago Q1
wos Q1
БС1
SJR: 1.05
CiteScore: 11.2
Impact factor: 5.3
ISSN: 09205861, 18734308
General Chemistry
Catalysis
Краткое описание
We examined oxidative coupling of methane (OCM) and oxidative dehydrogenation of ethane (ODE) over various polyoxometalate supported CeO 2 catalysts at 423 K in an electric field. Tetrabutylammonium (TBA) salt of Keggin-type phosphotungstate (PW 12 O 40 ) supported CeO 2 catalysts ((TBA) 3 PW 12 O 40 /CeO 2 ) showed high activities for OCM and ODE in the electric field (3 mA) at 423 K, although the catalyst without the electric field showed extremely low activities at such low temperature. FT-IR spectra and XRD patterns confirmed that the structure of (TBA) 3 PW 12 O 40 /CeO 2 was changed to Ce 2 (WO 4 ) 3 /CeO 2 after reactions with the electric field, and it acted as an active site structure for OCM and ODE with the electric field. Results of activity tests revealed that the C 2 H 6 production was a main reaction in OCM with the electric field, and C 2 H 4 was formed through a successive oxidative dehydrogenation of the formed C 2 H 6 . Periodic operation tests demonstrated that reactive oxygen species suitable for ODE were formed on the catalyst surface of Ce 2 (WO 4 ) 3 in the electric field.
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Ogo S. et al. Catalytic oxidative conversion of methane and ethane over polyoxometalate-derived catalysts in electric field at low temperature // Catalysis Today. 2018. Vol. 299. pp. 80-85.
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Ogo S., Iwasaki K., Sugiura K., Sato A., YABE T., Sekine Y. Catalytic oxidative conversion of methane and ethane over polyoxometalate-derived catalysts in electric field at low temperature // Catalysis Today. 2018. Vol. 299. pp. 80-85.
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TY - JOUR
DO - 10.1016/j.cattod.2017.05.013
UR - https://doi.org/10.1016/j.cattod.2017.05.013
TI - Catalytic oxidative conversion of methane and ethane over polyoxometalate-derived catalysts in electric field at low temperature
T2 - Catalysis Today
AU - Ogo, Shuhei
AU - Iwasaki, Kousei
AU - Sugiura, Kei
AU - Sato, Ayaka
AU - YABE, Tomohiro
AU - Sekine, Yasushi
PY - 2018
DA - 2018/01/01
PB - Elsevier
SP - 80-85
VL - 299
SN - 0920-5861
SN - 1873-4308
ER -
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@article{2018_Ogo,
author = {Shuhei Ogo and Kousei Iwasaki and Kei Sugiura and Ayaka Sato and Tomohiro YABE and Yasushi Sekine},
title = {Catalytic oxidative conversion of methane and ethane over polyoxometalate-derived catalysts in electric field at low temperature},
journal = {Catalysis Today},
year = {2018},
volume = {299},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/j.cattod.2017.05.013},
pages = {80--85},
doi = {10.1016/j.cattod.2017.05.013}
}